Simultaneous removal of NO x and SO2 by low-temperature selective catalytic reduction over modified activated carbon catalysts

2017 ◽  
Vol 91 (3) ◽  
pp. 490-499 ◽  
Author(s):  
Ye Liu ◽  
Ping Ning ◽  
Kai Li ◽  
Lihong Tang ◽  
Jiming Hao ◽  
...  
Keyword(s):  
Activated Carbon ◽  
Low Temperature ◽  
Selective Catalytic Reduction ◽  
Catalytic Reduction ◽  
Simultaneous Removal ◽  
Modified Activated Carbon ◽  
Carbon Catalysts

scholarly journals The Enhanced Performance of N-Modified Activated Carbon Promoted with Ce in Selective Catalytic Reduction of NOx with NH3

Catalysts ◽  
2020 ◽  
Vol 10 (12) ◽  
pp. 1423
Author(s):  
Marwa Saad ◽  
Agnieszka Szymaszek ◽  
Anna Białas ◽  
Bogdan Samojeden ◽  
Monika Motak
Keyword(s):  
Catalytic Activity ◽  
Activated Carbon ◽  
Low Temperature ◽  
Selective Catalytic Reduction ◽  
Catalytic Reduction ◽  
Catalytic Performance ◽  
Reduction Mechanism ◽  
Modified Activated Carbon ◽  
Oxidation Reduction ◽  
Reduction Of Nox

The goal of the study was to modify activated carbon (AC) with nitrogen groups and ceria and to test the obtained materials in low temperature selective catalytic reduction of nitrogen oxides. For that purpose, the starting AC was oxidized with HNO3 of various concentrations, modified with urea and doped with 0.5 wt.% of Ce. It was observed that the increased concentration of acid influenced the catalytic activity, since textural and surface chemistry of activated carbon was changed. The most active sample was that modified with 14 M HNO3 and it reached 96% of NO conversion at 300 °C. Additionally, the addition of Ce improved the catalytic performance of modified AC, and NO was reduced according to oxidation–reduction mechanism, characteristic for supported metal oxides. Nevertheless, the samples promoted with Ce emitted significantly higher amount of CO2 comparing to the non-promoted ones.

Regeneration of field-spent activated carbon catalysts for low-temperature selective catalytic reduction of NOx with NH3

2011 ◽  
Vol 174 (1) ◽  
pp. 242-248 ◽  
Author(s):  
Jong-Ki Jeon ◽  
Hyeonjoo Kim ◽  
Young-Kwon Park ◽  
Charles H.F. Peden ◽  
Do Heui Kim
Keyword(s):  
Activated Carbon ◽  
Low Temperature ◽  
Selective Catalytic Reduction ◽  
Catalytic Reduction ◽  
Reduction Of Nox ◽  
Carbon Catalysts

scholarly journals SO2 Poisoning and Recovery of Copper-Based Activated Carbon Catalysts for Selective Catalytic Reduction of NO with NH3 at Low Temperature

Catalysts ◽  
2020 ◽  
Vol 10 (12) ◽  
pp. 1426
Author(s):  
Marwa Saad ◽  
Agnieszka Szymaszek ◽  
Anna Białas ◽  
Bogdan Samojeden ◽  
Monika Motak
Keyword(s):  
Activated Carbon ◽  
Selective Catalytic Reduction ◽  
Active Sites ◽  
Catalytic Reduction ◽  
Incipient Wetness Impregnation ◽  
Exhaust Gas ◽  
Impregnation Method ◽  
No Conversion ◽  
So2 Poisoning ◽  
Carbon Catalysts

A series of materials based on activated carbon (AC) with copper deposited in various amounts were prepared using an incipient wetness impregnation method and tested as catalysts for selective catalytic reduction of nitrogen oxides with ammonia. The samples were poisoned with SO2 and regenerated in order to analyze their susceptibility to deactivation by the harmful component of exhaust gas. NO conversion over the fresh catalyst doped with 10 wt.% of Cu reached 81% of NO conversion at 140 °C and about 90% in the temperature range of 260–300 °C. The rate of poisoning with SO2 was dependent on Cu loading, but in general, it lowered NO conversion due to the formation of (NH4)2SO4 deposits that blocked the active sites of the catalysts. After regeneration, the catalytic activity of the materials was restored and NO conversion exceeded 70% for all of the samples.

Selective catalytic reduction of NO with NH3 over activated carbon impregnated with melamine at low temperature

2014 ◽  
Vol 42 (4) ◽  
pp. 487-493 ◽  
Author(s):  
Qiao-yan LI ◽  
Ya-qin HOU ◽  
Xiao-jin HAN ◽  
Zhang-gen HUANG ◽  
Qian-qian GUO ◽  
...  
Keyword(s):  
Activated Carbon ◽  
Low Temperature ◽  
Selective Catalytic Reduction ◽  
Catalytic Reduction ◽  
Reduction Of No
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