scholarly journals Intense exact resonance enhancement of single-high-harmonic from an antimony ion by using Ti:Sapphire laser at 37 nm

2007 ◽  
Vol 15 (3) ◽  
pp. 1161 ◽  
Author(s):  
Masayuki Suzuki ◽  
Motoyoshi Baba ◽  
Hiroto Kuroda ◽  
Rashid A. Ganeev ◽  
Tsuneyuki Ozaki
Mathematics ◽  
2020 ◽  
Vol 8 (3) ◽  
pp. 450
Author(s):  
Denys Dutykh ◽  
Elena Tobisch

The theory of exact resonances (kinematics and dynamics) is well developed while even the very concept of detuned resonance is ambiguous and only studies of their kinematic characteristics (that is, those not depending on time) are available in the literature. In this paper, we report novel effects enforced by the resonance detuning on solutions of the dynamical system describing interactions of three spherical planetary waves. We establish that the energy variation range can significantly exceed the range of the exact resonance for suitably chosen values of the detuning. The asymmetry of system’s solutions with respect to the sign of the detuning parameter is demonstrated. Finally, a non-monotonic dependence of the energy oscillation period with respect to detuning magnitude is discovered. These results have direct implications in physics of atmosphere, e.g., for prediction of weather extremes in the Northern Hemisphere midlatitudes (Proc. Nat. Acad. Sci. USA 2016, 133(25), 6862–6867). Moreover, similar study can be conducted for a generic three-wave system taken in the Hamiltonian form which makes our results applicable for an arbitrary Hamiltonian three-wave system met in climate prediction theory, geophysical fluid dynamics, plasma physics, etc.


Author(s):  
Denys Dutykh ◽  
Elena Tobisch

In this manuscript we report new effects of resonance detuning on various dynamical parameters of a generic 3-wave system. Namely, for suitably chosen values of detuning the variation range of amplitudes can be significantly wider than for exact resonance. Moreover, the range of energy variation is not symmetric with respect to the sign of the detuning. Finally, the period of the energy oscillation exhibits non-monotonic dependency on the magnitude of detuning. These results have important theoretical implications where nonlinear resonance analysis is involved, such as geophysics, plasma physics, fluid dynamics. Numerous practical applications are envisageable e.g. in energy harvesting systems.


2003 ◽  
Vol 104 ◽  
pp. 149-152 ◽  
Author(s):  
M. Wieland ◽  
R. Früke ◽  
T. Wilhein ◽  
U. Kleineberg ◽  
M. Pohl ◽  
...  

2020 ◽  
Author(s):  
Marta L. Vidal ◽  
Michael Epshtein ◽  
Valeriu Scutelnic ◽  
Zheyue Yang ◽  
Tian Xue ◽  
...  

We report a theoretical investigation and elucidation of the x-ray absorption spectra of neutral benzene and of the benzene cation. The generation of the cation by multiphoton ultraviolet (UV) ionization as well as the measurement of<br>the carbon K-edge spectra of both species using a table-top high-harmonic generation (HHG) source are described in the companion experimental paper [M. Epshtein et al., J. Phys.<br>Chem. A., submitted. Available on ChemRxiv]. We show that the 1sC -> pi transition serves as a sensitive signature of the transient cation formation, as it occurs outside of the spectral window of the parent neutral species. Moreover, the presence<br>of the unpaired (spectator) electron in the pi-subshell of the cation and the high symmetry of the system result in significant differences relative to neutral benzene in the spectral features associated with the 1sC ->pi* transitions. High-level calculations using equation-of-motion coupled-cluster theory provide the interpretation of the experimental spectra and insight into the electronic structure of benzene and its cation.<br>The prominent split structure of the 1sC -> pi* band of the cation is attributed to the interplay between the coupling of the core -> pi* excitation with the unpaired electron<br>in the pi-subshell and the Jahn-Teller distortion. The calculations attribute most of<br>the splitting (~1-1.2 eV) to the spin coupling, which is visible already at the Franck-Condon structure, and estimate the additional splitting due to structural relaxation to<br>be around ~0.1-0.2 eV. These results suggest that x-ray absorption with increased resolution might be able to disentangle electronic and structural aspects of the Jahn-Teller<br>effect in benzene cation.<br>


2019 ◽  
Author(s):  
Le Wang ◽  
Devon Jakob ◽  
Haomin Wang ◽  
Alexis Apostolos ◽  
Marcos M. Pires ◽  
...  

<div>Infrared chemical microscopy through mechanical probing of light-matter interactions by atomic force microscopy (AFM) bypasses the diffraction limit. One increasingly popular technique is photo-induced force microscopy (PiFM), which utilizes the mechanical heterodyne signal detection between cantilever mechanical resonant oscillations and the photo induced force from light-matter interaction. So far, photo induced force microscopy has been operated in only one heterodyne configuration. In this article, we generalize heterodyne configurations of photoinduced force microscopy by introducing two new schemes: harmonic heterodyne detection and sequential heterodyne detection. In harmonic heterodyne detection, the laser repetition rate matches integer fractions of the difference between the two mechanical resonant modes of the AFM cantilever. The high harmonic of the beating from the photothermal expansion mixes with the AFM cantilever oscillation to provide PiFM signal. In sequential heterodyne detection, the combination of the repetition rate of laser pulses and polarization modulation frequency matches the difference between two AFM mechanical modes, leading to detectable PiFM signals. These two generalized heterodyne configurations for photo induced force microscopy deliver new avenues for chemical imaging and broadband spectroscopy at ~10 nm spatial resolution. They are suitable for a wide range of heterogeneous materials across various disciplines: from structured polymer film, polaritonic boron nitride materials, to isolated bacterial peptidoglycan cell walls. The generalized heterodyne configurations introduce flexibility for the implementation of PiFM and related tapping mode AFM-IR, and provide possibilities for additional modulation channel in PiFM for targeted signal extraction with nanoscale spatial resolution.</div>


1979 ◽  
Vol 7 (3) ◽  
pp. 166-170 ◽  
Author(s):  
P. A. Jaanimagi ◽  
G. D. Enright ◽  
M. C. Richardson

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