Steady-State Modeling of Pt-Catalyzed H2 Combustion in a Monolithic Reactor: From Micro- to Macro-kinetics
2016 ◽
Vol 14
(1)
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pp. 373-381
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AbstractMicro-kinetic modeling of Pt-catalyzed hydrogen oxidation in a monolithic reactor was carried out for various feed temperatures. The monolith behavior was described by a simplified steady-state model that avoids surface species enthalpy evaluation and does not have temperatures as unknowns. A simplified pseudoarch length method was used to obtain the multiple solution branches for this typical exothermic reaction system. Based on parametric sensitivity and surface species distribution analyses of the micro-kinetic modeling results, macro-kinetic models that involve only gas concentrations were derived and were used to explain the composition effects on ignition temperature.
2006 ◽
Vol 320
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pp. 99-102
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1994 ◽
Vol 269
(42)
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pp. 26034-26039
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1973 ◽
Vol 37
(5)
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pp. 1141-1162
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2015 ◽
Vol 9
(16)
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pp. 2534-2543
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