scholarly journals Second Harmonic Revisited: An Analytic Quantum Approach

2019 ◽  
Vol 9 (8) ◽  
pp. 1690
Author(s):  
Giovanni Chesi ◽  
Matteo M. Wauters ◽  
Nadir Fasola ◽  
Alessia Allevi ◽  
Maria Bondani

We address the second-harmonic generation process in a quantum frame. Starting with a perturbative approach, we show that it is possible to achieve a number of analytic results, ranging from the up-conversion probability to the statistical properties of the generated light. In particular, the moments and the correlations of the photon-number distribution of the second-harmonic light generated by any initial state are retrieved. When possible, a comparison with the results achieved with the classical regime is successfully provided. The nonclassicality of some benchmark states is investigated by inspecting the corresponding autocorrelation function.

2011 ◽  
Vol 284 (5) ◽  
pp. 1401-1404 ◽  
Author(s):  
Michaël Delqué ◽  
Gil Fanjoux ◽  
Simon-Pierre Gorza ◽  
Marc Haelterman

2018 ◽  
Vol 43 (14) ◽  
pp. 3236 ◽  
Author(s):  
Haigang Liu ◽  
Xiaohui Zhao ◽  
Hui Li ◽  
Yuanlin Zheng ◽  
Xianfeng Chen

2008 ◽  
Vol 16 (19) ◽  
pp. 14496 ◽  
Author(s):  
A. Massaro ◽  
V. Tasco ◽  
M. T. Todaro ◽  
R. Cingolani ◽  
M. De Vittorio ◽  
...  

2020 ◽  
Author(s):  
Guan Gui ◽  
Nathan Brooks ◽  
Henry Kapteyn ◽  
Margaret Murnane ◽  
Chen-Ting Liao

Abstract Light with spatiotemporal orbital angular momentum (ST-OAM) is a recently discovered type of structured electromagnetic field with characteristic space-time spiral phase structure and transverse OAM. In this work, we present the first generation and characterization of the second-harmonic of ST-OAM pulses. By uncovering the conservation of transverse OAM in a second-harmonic generation process, where the space-time topological charge of the fundamental field is doubled along with the optical frequency, we establish a general nonlinear scaling rule— analogous to that describing the spatial topological charges associated with the conventional longitudinal OAM of light. Furthermore, we observe that the topology of a second-harmonic ST-OAM pulse can be modified by complex spatiotemporal astigmatism, giving rise to multiple phase singularities separated in space and time. Our finding thus confirms that a spatiotemporal phase winding, surrounding one or many phase singularities in space and time, can be interpreted as a new class of topological charge. Our study opens a new route for nonlinear conversion and scaling of light carrying ST-OAM with the potential for driving other secondary ST-OAM sources of electromagnetic fields, electron pulses, and beyond.


1999 ◽  
Vol 571 ◽  
Author(s):  
M. Jacobsohn ◽  
U. Banin

ABSTRACTSecond Harmonic Generation in CdSe nanocrystal quantum dots is observed by Hyper-Rayleigh scattering. We use a Ti-Sapphire femtosecond laser at 820 nm to induce the nonlinear optical response of the nanocrystals in solution. The unit cell normalized second harmonic coefficient βn, shows a substantial systematic enhancement in small sizes. The observed size dependence of the second harmonic generation process, is explained assuming two contributions. The first is a bulk-like contribution, from the non-centrosymmetric nanocrystal core, and the second, a contribution from the particle surface. The latter contribution is most significant in small nanocrystals with a substantial proportion of surface atoms.


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