scholarly journals Comparison of the optical depth of total ozone and atmospheric aerosols in Poprad-Gánovce, Slovakia

2018 ◽  
Vol 18 (10) ◽  
pp. 7739-7755
Author(s):  
Peter Hrabčák

Abstract. The amount of ultraviolet solar radiation reaching the Earth's surface is significantly affected by atmospheric ozone along with aerosols. The present paper is focused on a comparison of the total ozone and atmospheric aerosol optical depth in the area of Poprad-Gánovce, which is situated at the altitude of 706 m a. s. l.  in the vicinity of the highest mountain in the Carpathian mountains. The direct solar ultraviolet radiation has been measured here continuously since August 1993 using a Brewer MKIV ozone spectrophotometer. These measurements have been used to calculate the total amount of atmospheric ozone and, subsequently, its optical depth. They have also been used to determine the atmospheric aerosol optical depth (AOD) using the Langley plot method. Results obtained by this method were verified by means of comparison with a method that is part of the Brewer operating software, as well as with measurements made by a Cimel sun photometer. Diffuse radiation, the stray-light effect and polarization corrections were applied to calculate the AOD using the Langley plot method. In this paper, two factors that substantially attenuate the flow of direct ultraviolet solar radiation to the Earth's surface are compared. The paper presents results for 23 years of measurements, namely from 1994 to 2016. Values of optical depth were determined for the wavelengths of 306.3, 310, 313.5, 316.8 and 320 nm. A statistically significant decrease in the total optical depth of the atmosphere was observed with all examined wavelengths. Its root cause is the statistically significant decline in the optical depth of aerosols.

2014 ◽  
Vol 14 (11) ◽  
pp. 16529-16589
Author(s):  
V. De Bock ◽  
H. De Backer ◽  
R. Van Malderen ◽  
A. Mangold ◽  
A. Delcloo

Abstract. At Uccle, a long time series (1991–2013) of simultaneous measurements of erythemal ultraviolet (UV) dose, global solar radiation, total ozone column (TOC) and Aerosol Optical Depth (AOD) (at 320.1 nm) is available which allows for an extensive study of the changes in the variables over time. A change-point analysis, which determines whether there is a significant change in the mean of the time series, is applied to the monthly anomalies time series of the variables. Only for erythemal UV dose and TOC, a significant change point (without any known instrumental cause) was present in the time series around February 1998 and March 1998 respectively. The change point in TOC corresponds with results found in literature, where the change in ozone levels (around 1997) is attributed to the recovery of ozone. Linear trends were determined for the different (monthly anomalies) time series. Erythemal UV dose, global solar radiation and TOC all increase with respectively 7, 4 and 3% per decade. AOD shows an (insignificant) negative trend of −8% per decade. These trends agree with results found in literature for sites with comparable latitudes. A multiple linear regression (MLR) analysis is applied to the data in order to study the influence of global solar radiation, TOC and AOD on the erythemal UV dose. Together these parameters are able to explain 94% of the variation in erythemal UV dose. Most of the variation (56%) in erythemal UV dose is explained by global solar radiation. The regression model performs well with a slight tendency to underestimate the measured erythemal UV doses and with a Mean Absolute Bias Error (MABE) of 18%. However, in winter, negative erythemal UV dose values are modeled. Applying the MLR to the individual seasons solves this issue. The seasonal models have an adjusted R2 value higher than 0.8 and the correlation between modeled and measured erythemal UV dose values is higher than 0.9 for each season. The summer model gives the best performance, with an absolute mean error of only 6%. Again, global solar radiation is the factor that contributes the most to the variation in erythemal UV dose, so there is no doubt about the necessity to include this factor in the regression models. A large part of the influence of AOD is already represented by the global solar radiation parameter. Therefore the individual contribution of AOD to erythemal UV dose is so low. For this reason, it seems unnecessary to include AOD in the MLR analysis. Including TOC however, is justified as the adjusted R2 increases and the MABE of the model decreases compared to a model where only global solar radiation is used as explanatory variable.


2000 ◽  
Vol 45 (14) ◽  
pp. 1328-1334 ◽  
Author(s):  
Yunfeng Luo ◽  
Daren Lü ◽  
Qing He ◽  
Weiliang Li ◽  
Xiuji Zhou

2012 ◽  
Vol 12 (12) ◽  
pp. 33265-33289
Author(s):  
A. V. Lindfors ◽  
N. Kouremeti ◽  
A. Arola ◽  
S. Kazadzis ◽  
A. F. Bais ◽  
...  

Abstract. Pyranometer measurements of the solar surface radiation (SSR) are available at many locations worldwide, often as long time series covering several decades into the past. These data constitute a potential source of information on the atmospheric aerosol load. Here, we present a method for estimating the aerosol optical depth (AOD) using pyranometer measurements of the SSR together with total water vapor column information. The method, which is based on radiative transfer simulations, was developed and tested using recent data from Thessaloniki, Greece. The effective AOD calculated using this method was found to agree well with co-located AERONET measurements, exhibiting a correlation coefficient of 0.9 with 2/3 of the data found within ±20% or ±0.05 of the AERONET AOD. This is similar to the performance of current satellite aerosol methods. Differences in the AOD as compared to AERONET can be explained by variations in the aerosol properties of the atmosphere that are not accounted for in the idealized settings used in the radiative transfer simulations, such as variations in the single scattering albedo and Ångström exponent. Furthermore, the method is sensitive to calibration offsets between the radiative transfer simulations and the pyranometer SSR. The method provides an opportunity of extending our knowledge of the atmospheric aerosol load to locations and times not covered by dedicated aerosol measurements.


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