This paper presents space-time kriging within a multi-Gaussian framework for time-series mapping of particulate matter less than 10 μm in aerodynamic diameter (PM10) concentration. To account for the spatiotemporal autocorrelation structures of monitoring data and to model the uncertainties attached to the prediction, conventional multi-Gaussian kriging is extended to the space-time domain. Multi-Gaussian space-time kriging presented in this paper is based on decomposition of the PM10concentrations into deterministic trend and stochastic residual components. The deterministic trend component is modelled and regionalized using the temporal elementary functions. For the residual component which is the main target for space-time kriging, spatiotemporal autocorrelation information is modeled and used for space-time mapping of the residual. The conditional cumulative distribution functions (ccdfs) are constructed by using the trend and residual components and space-time kriging variance. Then, the PM10concentration estimate and conditional variance are empirically obtained from the ccdfs at all locations in the study area. A case study using the monthly PM10concentrations from 2007 to 2011 in the Seoul metropolitan area, Korea, illustrates the applicability of the presented method. The presented method generated time-series PM10concentration mapping results as well as supporting information for interpretations, and led to better prediction performance, compared to conventional spatial kriging.
Case study of ozone photochemistry in the Seoul metropolitan area during the summer 2003