Flicker noise in two-dimensional electron gas

Using the method developed in a recent paper (Euro. Phys. J. B 92.8 (2019): 1-28) we consider 1/f noise in two-dimensional electron gas (2DEG). The electron coherence length of the system is considered as a basic parameter for discretizing the space, inside which the dynamics of electrons is described by quantum mechanics, while for length scales much larger than it the dynamics is semi-classical. For our model, which is based on the Thomas-Fermi-Dirac approximation, there are two control parameters: temperature T and the disorder strength (∆). Our Monte Carlo studies show that the system exhibits 1/f noise related to the electronic avalanche size, which can serve as a model for describing the experimentally observed flicker noise in 2DEG. The power spectrum of our model scales with frequency with an exponent in the interval 0.3 < αPS < 0.6. We numerically show that the electronic avalanches are scale invariant with power-law behaviors in and out of the metal-insulator transition line.

Probing Attosecond Electron Coherence in Molecular Charge Migration by Ultrafast X-Ray Photoelectron Imaging

Electron coherence is a fundamental quantum phenomenon in today’s ultrafast physics and chemistry research. Based on attosecond pump–probe schemes, ultrafast X-ray photoelectron imaging of molecules was used to monitor the coherent electron dynamics which is created by an XUV pulse. We performed simulations on the molecular ion H 2 + by numerically solving time-dependent Schrödinger equations. It was found that the X-ray photoelectron angular and momentum distributions depend on the time delay between the XUV pump and soft X-ray probe pulses. Varying the polarization and helicity of the soft X-ray probe pulse gave rise to a modulation of the time-resolved photoelectron distributions. The present results provide a new approach for exploring ultrafast coherent electron dynamics and charge migration in reactions of molecules on the attosecond time scale.

Emergence of electron coherence and two-color all-optical switching in MoS2 based on spatial self-phase modulation

Generating electron coherence in quantum materials is essential in optimal control of many-body interactions and correlations. In a multidomain system this signifies nonlocal coherence and emergence of collective phenomena, particularly in layered 2D quantum materials possessing novel electronic structures and high carrier mobilities. Here we report nonlocal ac electron coherence induced in dispersed MoS2 flake domains, using coherent spatial self-phase modulation (SSPM). The gap-dependent nonlinear dielectric susceptibility χ(3) measured is surprisingly large, where direct interband transition and two-photon SSPM are responsible for excitations above and below the bandgap, respectively. A wind-chime model is proposed to account for the emergence of the ac electron coherence. Furthermore, all-optical switching is achieved based on SSPM, especially with two-color intraband coherence, demonstrating that electron coherence generation is a ubiquitous property of layered quantum materials.