VERIFICATION OF SUBCRITICAL LIMITS IN ANSI/ANS-8.1-2014

The ANSI/ANS-8.1 standard, “Safety Standard for Operations with Fissionable Materials Outside Reactors,” has been available since 1964 as ASA N6.1-1964. In 1969, this standard was revised as ANSI N16.1-1969, “Nuclear Criticality Safety in Operations with Fissionable Materials Outside Reactors.” This version of the standard includes a variety of subcritical limits (SCLs) for uniform aqueous solutions and metals containing fissile nuclides for 233U, 235U, and 239Pu. Furthermore, SCLs are also included for uranium-water lattices. In the 1983 version of ANSI/ANS-8.1 (a revision of ANSI N16.1-1975), the suite of SCLs in the standard expanded to include 235U enrichment limits for homogeneous uranium-water mixtures and dry/damp oxides, uniform aqueous solutions of low-enriched uranium, and uniform aqueous mixtures of Pu(NO3)4 containing 240Pu, in addition to the SCLs included in ANSI N16.1-1969. The SCLs have changed little in subsequent revisions (ANSI/ANS-8.1-1998 and ANSI/ANS-8.1-2014). The ANSI/ANS-8.1-2014 standard is currently being revised to include new SCLs (uranium metal and compounds with enrichments up to 20 wt. % 235U) and possible updates to the current SCLs already in the standard, although these SCLs will not be available to the nuclear criticality safety community for a number of years. The bases for these SCLs were documented in journal articles such as Nuclear Science and Engineering, and the American Nuclear Society’s meeting transactions; however, the bases were ambiguous enough that sites and regulators in the United States are reluctant to endorse them for safety purposes. The purpose of this paper is to present the results of a comparison study for the SCLs in the ANSI/ANS-8.1-2014 standard using modern codes and cross sections (SCALE/ENDF/B-VIII) to provide some assurance about their quality (bias and bias uncertainty) for use in nuclear criticality safety applications.

ENDF/B-VIII.0 CROSS SECTION TESTING FOR COPPER NUCLEAR CRITICALITY SAFETY APPLICATIONS

In the update from ENDF/B-VII.1 to ENDF/B-VIII.0, copper cross sections were significantly altered in the intermediate and fast spectrum of the ENDF-VIII.0 library. Performance of this ENDF data requires validation to determine whether recent evaluation has proven beneficial. To examine the performance of the new library, particularly new copper data, critical benchmarks from the ICSBEP handbook were chosen for their sensitivity to copper cross section changes and modeled using SCALE continuous energy Monte Carlo simulations. Selected benchmarks were modeled in ENDF-VII.1 and ENDF-VIII.0 to compute keff within a statistical uncertainty of 10 pcm and compared in reference to the benchmark experimental criticality. Due to spectrum choices in selection based on the changes to cross section data, the set of benchmarks consist of intermediately enriched uranium, highly enriched uranium, or plutonium systems. 11 separate benchmark evaluations containing 32 individual configurations highly sensitive to copper were selected, modelled, and compared to benchmark experimental criticality. This work demonstrates a significant decrease in the deviation between calculated and experimental criticality as a result of the ENDF-VIII.0 library; a decrease in absolute mean deviation from 522.5±39.3 to 249.6±39.3, and a decrease in root mean square deviation from 630.8±46.1 to 338.1±74.9. Additionally, the role of recently evaluated copper data in this improved agreement is presented, confirming the benefit of reaffirming cross section data.