scholarly journals Insights from Transient Absorption Spectroscopy into Electron Dynamics Along the Ga‐Gradient in Cu(In,Ga)Se 2 Solar Cells

2021 ◽  
Vol 11 (8) ◽  
pp. 2003446
Author(s):  
Yu‐Han Chang ◽  
Romain Carron ◽  
Mario Ochoa ◽  
Carlota Bozal‐Ginesta ◽  
Ayodhya N. Tiwari ◽  
...  
2019 ◽  
Vol 9 (7) ◽  
pp. 1350
Author(s):  
Daria Kolbasova ◽  
Robin Santra

A theoretical description of attosecond transient absorption spectroscopy for temporally and spatially overlapping XUV and optical pulses is developed, explaining the signals one can obtain in such an experiment. To this end, we employ a two-stage approach based on perturbation theory, which allows us to give an analytical expression for the transient absorption signal. We focus on the situation in which the attosecond XUV pulse is used to create a coherent superposition of electronic states. As we explain, the resulting dynamics can be detected in the spectrum of the transmitted XUV pulse by manipulating the electronic wave packet using a carrier-envelope-phase-stabilized optical dressing pulse. In addition to coherent electron dynamics triggered by the attosecond pulse, the transmitted XUV spectrum encodes information on electronic states made accessible by the optical dressing pulse. We illustrate these concepts through calculations performed for a few-level model.


2020 ◽  
Vol 22 (5) ◽  
pp. 2704-2712 ◽  
Author(s):  
Taran Driver ◽  
Siqi Li ◽  
Elio G. Champenois ◽  
Joseph Duris ◽  
Daniel Ratner ◽  
...  

Recently demonstrated isolated attosecond XFEL pulses should allow the probing of ultrafast electron dynamics at X-ray wavelengths. The authors use ghost imaging to enable high-resolution transient absorption spectroscopy at fluctuating XFEL sources.


2016 ◽  
Vol 18 (13) ◽  
pp. 8938-8944 ◽  
Author(s):  
Iulia Minda ◽  
Essraa Ahmed ◽  
Vivien Sleziona ◽  
Christoph Richter ◽  
Max Beu ◽  
...  

Charge transfer dynamics in fully operational dye sensitised solar cells as observed using ultrafast transient absorption spectroscopy.


2015 ◽  
Vol 17 (22) ◽  
pp. 14674-14684 ◽  
Author(s):  
Piotr Piatkowski ◽  
Boiko Cohen ◽  
Francisco Javier Ramos ◽  
Maria Di Nunzio ◽  
Mohammad Khaja Nazeeruddin ◽  
...  

Electron and hole dynamics, and internal and surface trap states in perovskite-based solar cells are explored by fs transient absorption spectroscopy.


2002 ◽  
Vol 106 (31) ◽  
pp. 7605-7613 ◽  
Author(s):  
Richard L. Willis ◽  
Carol Olson ◽  
Brian O'Regan ◽  
Thierry Lutz ◽  
Jenny Nelson ◽  
...  

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