Empirical model of vertical structure of the middle atmosphere: Seasonal variations and long-term changes of temperature and number density

2006 ◽  
Vol 38 (11) ◽  
pp. 2465-2469
Author(s):  
N.N. Pertsev ◽  
A.I. Semenov ◽  
N.N. Shefov
2015 ◽  
Vol 33 (6) ◽  
pp. 749-767 ◽  
Author(s):  
G. R. Sonnemann ◽  
P. Hartogh ◽  
U. Berger ◽  
M. Grygalashvyly

Abstract. The layer of vibrationally excited hydroxyl (OH*) near the mesopause in Earth's atmosphere is widely used to derive the temperature at this height and to observe dynamical processes such as gravity waves. The concentration of OH* is controlled by the product of atomic hydrogen, with ozone creating a layer of enhanced concentration in the mesopause region. However, the basic influences on the OH* layer are atomic oxygen and temperature. The long-term monitoring of this layer provides information on a changing atmosphere. It is important to know which proportion of a trend results from anthropogenic impacts on the atmosphere and which proportion reflects natural variations. In a previous paper (Grygalashvyly et al., 2014), the trend of the height of the layer and the trend in temperature were investigated particularly in midlatitudes on the basis of our coupled dynamic and chemical transport model LIMA (Leibniz Institute Middle Atmosphere). In this paper we consider the trend for the number density between the years 1961 and 2009 and analyze the reason of the trends on a global scale. Further, we consider intra-annual variations. Temperature and wind have the strongest impacts on the trend. Surprisingly, the increase in greenhouse gases (GHGs) has no clear influence on the chemistry of OH*. The main reason for this lies in the fact that, in the production term of OH*, if atomic hydrogen increases due to increasing humidity of the middle atmosphere by methane oxidation, ozone decreases. The maximum of the OH* layer is found in the mesopause region and is very variable. The mesopause region is a very intricate domain marked by changeable dynamics and strong gradients of all chemically active minor constituents determining the OH* chemistry. The OH* concentration responds, in part, very sensitively to small changes in these parameters. The cause for this behavior is given by nonlinear reactions of the photochemical system being a nonlinear enforced chemical oscillator driven by the diurnal-periodic solar insolation. At the height of the OH* layer the system operates in the vicinity of chemical resonance. The solar cycle is mirrored in the data, but the long-term behavior due to the trend in the Lyman-α radiation is very small. The number density shows distinct hemispheric differences. The calculated OH* values show sometimes a step around a certain year. We introduce a method to find out the date of this step and discuss a possible reason for such behavior.


2003 ◽  
Vol 32 (9) ◽  
pp. 1675-1684 ◽  
Author(s):  
D. Offermannl ◽  
M. Donner ◽  
P. Knieling ◽  
K. Hamilton ◽  
A. Menzel ◽  
...  

2022 ◽  
Vol 22 (1) ◽  
pp. 561-575
Author(s):  
Jiaxing Sun ◽  
Zhe Wang ◽  
Wei Zhou ◽  
Conghui Xie ◽  
Cheng Wu ◽  
...  

Abstract. Atmospheric aerosols play an important role in the radiation balance of the earth–atmosphere system. However, our knowledge of the long-term changes in equivalent black carbon (eBC) and aerosol optical properties in China is very limited. Here we analyze the 9-year measurements of eBC and aerosol optical properties from 2012 to 2020 in Beijing, China. Our results showed large reductions in eBC by 71 % from 6.25 ± 5.73 µg m−3 in 2012 to 1.80 ± 1.54 µg m−3 in 2020 and 47 % decreases in the light extinction coefficient (bext, λ = 630 nm) of fine particles due to the Clean Air Action Plan that was implemented in 2013. The seasonal and diurnal variations of eBC illustrated the most significant reductions in the fall and at nighttime, respectively. ΔeBC / ΔCO also showed an annual decrease from ∼ 7 to 4 ng m−3 ppbv−1 and presented strong seasonal variations with high values in spring and fall, indicating that primary emissions in Beijing have changed significantly. As a response to the Clean Air Action Plan, single-scattering albedo (SSA) showed a considerable increase from 0.79 ± 0.11 to 0.88 ± 0.06, and mass extinction efficiency (MEE) increased from 3.2 to 3.8 m2 g−1. These results highlight the increasing importance of scattering aerosols in radiative forcing and a future challenge in visibility improvement due to enhanced MEE. Brown carbon (BrC) showed similar changes and seasonal variations to eBC during 2018–2020. However, we found a large increase of secondary BrC in the total BrC in most seasons, particularly in summer with the contribution up to 50 %, demonstrating an enhanced role of secondary formation in BrC in recent years. The long-term changes in eBC and BrC have also affected the radiative forcing effect. The direct radiative forcing (ΔFR) of BC decreased by 67 % from +3.36 W m−2 in 2012 to +1.09 W m−2 in 2020, and that of BrC decreased from +0.30 to +0.17 W m−2 during 2018–2020. Such changes might have important implications for affecting aerosol–boundary layer interactions and the improvement of future air quality.


2021 ◽  
Author(s):  
Ales Kuchar ◽  
Gunter Stober ◽  
Christoph Jacobi ◽  
Dimitry Pokhotelov ◽  
Huxin Liu ◽  
...  

<p class="western">Several studies (Banerjee et al. (2020) and before that Sun et al. (2014)) found a trend reversal between winter and summer circulation in the southern hemisphere around 2000 in the middle atmosphere. One may argue that the negative trend after 2000 is due to the CO<sub>2</sub>-induced change in stratospheric dynamics. However, Ramesh et al. (2020), using the newest WACCM6 simulation and a multiple linear regression model, confirmed that the negative trend in the stratosphere after 2000 can be attributed to ozone recovery. Here we investigate how stratospheric trends relate to trends in the mesosphere and lower thermosphere (MLT) dynamics. Using the adaptive spectral filtering (ASF) method (Stober et al., 2021), we study long-term changes in mesospheric wind and planetary and gravity wave estimates<span lang="en-GB"> of meteor radar stations in the northern (NH: Collm, Kiruna, Sodankyla, CM</span><span lang="en-GB">OR</span><span lang="en-GB">) and southern (SH: Rio Grande, Davis, Rothera) hemisphere, respectively, for the altitude range of 80–100 km. </span>Linear trends have been estimated (from monthly means calculated from the preprocessed original data using ASF) by the Theil–Sen estimator (Theil, 1950; Sen, 1968). The robustness of our fitting method is assessed in terms of spurious trends due to, e.g., high autocorrelation of relatively short time series. The long-term changes are validated in two whole-atmosphere models, namely, GAIA and WACCMX-SD (both nudged in the stratosphere). While both models reveal issues reproducing basic climatology in the mesosphere, GAIA fairly reproduces the trends captured by the meteor radars. Finally, we conclude that the ozone recovery effects in the SH stratosphere influence the dynamics in MLT via gravity wave coupling.</p>


2017 ◽  
Vol 31 (1) ◽  
pp. 423-448 ◽  
Author(s):  
Gloria L. Manney ◽  
Michaela I. Hegglin

Abstract Long-term changes in upper-tropospheric jet latitude, altitude, and strength are assessed for 1980–2014 using five modern reanalyses: MERRA, MERRA-2, ERA-Interim, JRA-55, and NCEP CFSR. Changes are computed from jet locations evaluated daily at each longitude to analyze regional and seasonal variations. The changes in subtropical and polar (eddy driven) jets are evaluated separately. Good agreement among the reanalyses in many regions and seasons provides confidence in the robustness of the diagnosed trends. Jet shifts show strong regional and seasonal variations, resulting in changes that are not robust in zonal or annual means. Robust changes in the subtropical jet indicate tropical widening over Africa except during Northern Hemisphere (NH) spring, and tropical narrowing over the eastern Pacific in NH winter. The Southern Hemisphere (SH) polar jet shows a robust poleward shift, while the NH polar jet shifts equatorward in most regions/seasons. Both subtropical and polar jet altitudes typically increase; these changes are more robust in the NH than in the SH. Subtropical jet wind speeds have generally increased in winter and decreased in summer, whereas polar jet wind speeds have weakened (strengthened) over Africa and eastern Asia (elsewhere) during winter in both hemispheres. The Asian monsoon has increased in area and appears to have shifted slightly westward toward Africa. The results herein highlight the importance of understanding regional and seasonal variations when quantifying long-term changes in jet locations, the mechanisms for those changes, and their potential human impacts. Comparison of multiple reanalyses is a valuable tool for assessing the robustness of jet changes.


2021 ◽  
Author(s):  
Jiaxing Sun ◽  
Zhe Wang ◽  
Wei Zhou ◽  
Conghui Xie ◽  
Cheng Wu ◽  
...  

Abstract. Atmospheric aerosols play an important role in radiation balance of the earth-atmosphere system. However, our knowledge of the long-term changes in black carbon (BC) and aerosol optical properties in China are very limited. Here we analyze the nine-year measurements of BC and aerosol optical properties from 2012 to 2020 in Beijing, China. Our results showed large reductions in eBC by 67 % from 5.54 ± 5.25 µg m−3 in 2012 to 1.80 ± 1.54 µg m−3 in 2020, and 47 % decreases in light extinction coefficient (bext, λ = 630 nm) of fine particles due to clean air action plan since 2013. The seasonal and diurnal variations of eBC illustrated the most significant reductions in the fall and night time, respectively. ΔeBC/ΔCO also showed an annual decrease from ~6 to 4 ng m−3 ppbv−1 and presented strong seasonal variations with high values in spring and fall, indicating that primary emissions in Beijing have changed significantly. As a response to clean air action, single scattering albedo (SSA) showed a considerable increase from 0.79 ± 0.11 to 0.88 ± 0.06, and mass extinction efficiency (MEE) increased from 3.2 to 3.8 m2 g−1. These results highlight an increasing importance of scattering aerosols in radiative forcing, and a future challenge in visibility improvement due to enhanced MEE. Brown carbon (BrC) showed similar changes and seasonal variations to eBC during 2018–2020. However, we found a large increase of secondary BrC in the total BrC in most seasons, particularly in summer with the contribution up to 50 %, demonstrating an enhanced role of secondary formation in BrC in recent years. The long-term changes in eBC and BrC have also affected the radiative forcing effect. The direct radiative forcing (ΔFR) of BC decreased by 64 % from +3.00 W m−2 in 2012 to +1.09 W m−2 in 2020, and that of BrC decreased from +0.30 to +0.17 W m−2 during 2018–2020. Such changes might have important implications in affecting aerosol and boundary-layer interactions and the future air quality improvement.


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