Integrating Chemical Mass Balance and the Community Multiscale Air Quality models for source identification and apportionment of PM2.5

Author(s):  
Cheng Zhang ◽  
Deji Jing ◽  
Chengzhi Wu ◽  
Sujing Li ◽  
Nana Cheng ◽  
...  
2014 ◽  
Vol 14 (15) ◽  
pp. 8043-8054 ◽  
Author(s):  
G. Engling ◽  
J. He ◽  
R. Betha ◽  
R. Balasubramanian

Abstract. Biomass burning activities commonly occur in Southeast Asia (SEA), and are particularly intense in Indonesia during the dry seasons. The effect of biomass smoke emissions on air quality in the city state of Singapore was investigated during a haze episode in October 2006. Substantially increased levels of airborne particulate matter (PM) and associated chemical species were observed during the haze period. Specifically, the enhancement in the concentration of molecular tracers for biomass combustion such as levoglucosan by as much as two orders of magnitude and the diagnostic ratios of individual organic compounds indicated that biomass burning emissions caused a regional smoke haze episode due to their long-range transport by prevailing winds. With the aid of air mass backward trajectories and chemical mass balance modeling, large-scale forest and peat fires in Sumatra and Kalimantan were identified as the sources of the smoke aerosol, exerting a significant impact on air quality in downwind areas, such as Singapore.


2014 ◽  
Vol 140 (3) ◽  
pp. 04013015 ◽  
Author(s):  
Soroosh Sharifi ◽  
Mohammad Masoud Haghshenas ◽  
Tolessa Deksissa ◽  
Peter Green ◽  
William Hare ◽  
...  

2014 ◽  
Vol 14 (2) ◽  
pp. 2773-2798 ◽  
Author(s):  
G. Engling ◽  
J. He ◽  
R. Betha ◽  
R. Balasubramanian

Abstract. Biomass burning activities commonly occur in Southeast Asia (SEA), and are particularly intense in Indonesia during dry seasons. The effect of biomass smoke emissions on air quality in the city state of Singapore was investigated during a haze episode in October 2006. Substantially increased levels of airborne particulate matter (PM) and associated chemical species were observed during the haze period. Specifically, the enhancement in the concentration of molecular tracers for biomass combustion such as levoglucosan by as much as two orders of magnitude and diagnostic ratios of individual organic compounds indicated that biomass burning emissions caused a regional smoke haze episode due to their long-range transport by prevailing winds. With the aid of air mass back trajectories and chemical mass balance modeling, large-scale forest and peat fires in Sumatra and Kalimantan were identified as the sources of the smoke aerosol, exerting a significant impact on air quality in downwind areas, such as Singapore.


1998 ◽  
Vol 37 (6-7) ◽  
pp. 199-206 ◽  
Author(s):  
P. Rachdawong ◽  
E. R. Christensen ◽  
S. Chi

This work focuses on the determination of PCB source profiles and their contributions to sediments in the Milwaukee Harbor Estuary by a principal component analysis (PCA) model. The model was recently developed and, for the first time, applied to apportion pollutant sources in sediments. Factor loadings and scores were computed, rotated via nonnegative constraints, and matched with candidate Aroclor profiles. Contamination by Aroclors 1016, 1242, 1254, and 1260 were identified for cores VC 6, 9, and 12 based on a log Q2 criterion. The majority of PCB contribution was from a combination of Aroclors 1016 and 1242. Similarity between Aroclors 1016 and 1242 obscured resolution between the two profiles. Results from a chemical mass balance (CMB) model with known Aroclor profiles were in good agreement with the prediction from the PCA model.


1994 ◽  
Vol 21 (1) ◽  
pp. 1-36 ◽  
Author(s):  
John G. Watson ◽  
Judith C. Chow ◽  
Zhiqiang Lu ◽  
Eric M. Fujita ◽  
Douglas H. Lowenthal ◽  
...  

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