Highly Efficient Solution-Processed Thermally Activated Delayed Fluorescence Bluish-Green and Hybrid White Organic Light-Emitting Diodes Using Novel Bipolar Host Materials

2019 ◽  
Vol 11 (49) ◽  
pp. 45939-45948 ◽  
Author(s):  
Phu Si Ngo ◽  
Miao-Ken Hung ◽  
Kuen-Wei Tsai ◽  
Sunil Sharma ◽  
Show-An Chen
2020 ◽  
Vol 20 (11) ◽  
pp. 7191-7195
Author(s):  
JaMin Lee ◽  
Sae Won Lee ◽  
Young Sik Kim

Novel thermally activated delayed fluorescence (TADF) host materials for blue electrophosphores-cence were designed by combining the electron acceptor dibenzothiophene (DBT) unit and the electron donor acridine derivatives into a single molecular unit by density functional theory (DFT). Depending on the optimal charge transfer, DFT and time-dependent DFT (TD-DFT) calculations for the ground state were performed to obtain the energy of the singlet (S1) and triplet (T1) excited states of the TADF material for Hartree-Fock percentage of TD-DFT. The sufficiently large separation between the HOMO and LUMO resulted in a small difference in energy (ΔEST) between the S1 and T1 states using DFT and TD-DFT calculations. The host molecules retained high triplet energy and showed great potential for use in blue organic light-emitting diodes (OLED). The results showed that these molecules are a good TADF host materials because they have a low barrier to hole and electron injection with a balanced charge transporting property for both holes and electrons, and a small ΔEST.


2021 ◽  
Author(s):  
Gyana Prakash Nanda ◽  
Bahadur Sk ◽  
Nisha Yadav ◽  
Suresh Rajamanickam ◽  
Upasana Deori ◽  
...  

We report highly efficient, ultrathin non-doped green and bluish-green organic light-emitting diodes (OLEDs) using a thermally activated delayed fluorescence (TADF) emitter. The green OLED with an ultrathin (~1 nm) EML...


2018 ◽  
Vol 6 (34) ◽  
pp. 9152-9157 ◽  
Author(s):  
Xing Li ◽  
Kai Wang ◽  
Yi-Zhong Shi ◽  
Ming Zhang ◽  
Gao-Le Dai ◽  
...  

A novel thermally activated delayed fluorescence (TADF) emitter was designed and synthesized for solution-processed red organic light-emitting diodes (OLEDs).


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