Facile fabrication and enhanced photosensitized degradation performance of the g-C3N4–Bi2O2CO3 composite

2014 ◽  
Vol 43 (22) ◽  
pp. 8331-8337 ◽  
Author(s):  
Miao Xiong ◽  
Lang Chen ◽  
Qing Yuan ◽  
Jie He ◽  
Sheng-Lian Luo ◽  
...  

Flower-like Bi2O2CO3 and g-C3N4–Bi2O2CO3 microspheres with a high adsorption ability were synthesized using a facile method, and their dye-induced photosensitized degradation activity under visible light irradiation was evaluated.

2016 ◽  
Vol 193 ◽  
pp. 22-35 ◽  
Author(s):  
Xiaolong Yang ◽  
Fangfang Qian ◽  
Guojun Zou ◽  
Mengli Li ◽  
Jinren Lu ◽  
...  

2020 ◽  
Vol 2020 ◽  
pp. 1-10
Author(s):  
Shuo Xu ◽  
Xiaoya Gao ◽  
Wenfeng Xu ◽  
Pengfei Jin ◽  
Yongmei Kuang

A series of ultrathin BiOCl 2D nanosheet photocatalysts were prepared by the TBAOH-assisted hydrolysis method in water. The effects of tetrabutylammonium hydroxide (TBAOH) dosages, chlorine source, preparation pH value, ultrasonic treatment, and magnetic stirring on the photocatalytic degradation dynamics of carbamazepine were examined under visible-light irradiation to optimize the preparation parameters. It was found that ultrathin BiOCl prepared with TBAOH dosages of 1 mmol and chlorine source of NaCl in the pH of 2 upon magnetic stirring of 6 h displayed the highest photocatalytic degradation rate constant (0.0038 min−1) of carbamazepine, which is 7.6 times higher than that with the ordinary BiOCl (without TBAOH). To clarify the mechanism on the outstanding photocatalytic activity of ultrathin BiOCl, the elemental composition/state, micromorphology, and separation efficiency of photogenerated electron-hole pairs were investigated by X-ray photoelectron spectroscopy (XPS), scanning electron microscope (SEM), and photoluminescence (PL). Results showed that the presence of oxygen vacancy, ultrathin nanosheet structure, and improved separation efficiency of photogenerated electron-hole pairs contributed to the excellent photocatalytic degradation activity of ultrathin BiOCl. The obtained result provides a novel method to fabricate ultrathin BiOCl with excellent photocatalytic degradation activity of carbamazepine under visible-light irradiation.


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