Engineering active sites of two-dimensional MoS2 nanosheets for improving hydrogen evolution

2016 ◽  
Vol 3 (11) ◽  
pp. 1376-1380 ◽  
Author(s):  
Xiangkai Kong ◽  
Xiaochen Shen ◽  
Changlin Zhang ◽  
Shirin Norooz Oliaee ◽  
Zhenmeng Peng
Keyword(s):  
Hydrogen Evolution ◽  
Active Sites ◽  
Two Dimensional ◽  
Mos2 Nanosheets

S edges were peeled off to disclose inner S as new under-coordinated atoms, which exposed more fresh active sites.

In-Plane Heterojunctions Enable Multiphasic Two-Dimensional (2D) MoS2 Nanosheets As Efficient Photocatalysts for Hydrogen Evolution from Water Reduction

ACS Catalysis ◽  
2016 ◽  
Vol 6 (10) ◽  
pp. 6723-6729 ◽  
Author(s):  
Rui Peng ◽  
Liangbo Liang ◽  
Zachary D. Hood ◽  
Abdelaziz Boulesbaa ◽  
Alexander Puretzky ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Two Dimensional ◽  
Mos2 Nanosheets ◽  
Water Reduction

Two-Dimensional Confined Synthesis of Metastable 1T-Phase MoS2 Nanosheets for the Hydrogen Evolution Reaction

2022 ◽  
Author(s):  
Shize Geng ◽  
Yujin Ji ◽  
Binbin Jiang ◽  
Wenxiang Zhu ◽  
Kui Yin ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
Two Dimensional ◽  
Mos2 Nanosheets

Hydrazine-assisted formation of ultrathin MoS2 nanosheets for enhancing their co-catalytic activity in photocatalytic hydrogen evolution

2017 ◽  
Vol 5 (15) ◽  
pp. 6981-6991 ◽  
Author(s):  
D. Amaranatha Reddy ◽  
Hanbit Park ◽  
Sangyeob Hong ◽  
D. Praveen Kumar ◽  
Tae Kyu Kim
Keyword(s):  
Electrical Conductivity ◽  
Catalytic Activity ◽  
Hydrogen Evolution ◽  
Active Sites ◽  
Mos2 Nanosheets ◽  
Photocatalytic Hydrogen Evolution ◽  
Ultrathin Mos2 Nanosheets

This work demonstrates a simple and effective approach using hydrazine to modulate the active sites and electrical conductivity of MoS2 with the aid of ultrasonication.

Synthesized ultrathin MoS2 nanosheets perpendicular to graphene for catalysis of hydrogen evolution reaction

2015 ◽  
Vol 51 (10) ◽  
pp. 1893-1896 ◽  
Author(s):  
Z. H. Deng ◽  
L. Li ◽  
W. Ding ◽  
K. Xiong ◽  
Z. D. Wei
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
Active Sites ◽  
Mos2 Nanosheets ◽  
Subsequent Growth ◽  
Ultrathin Mos2 Nanosheets

The S atoms bind to active sites of RGO for the nucleation of MoS2 and its subsequent growth perpendicular to RGO.

Unveiling active sites by structural tailoring of two‐dimensional niobium disulfide for improved electrocatalytic hydrogen evolution reaction

2020 ◽  
Vol 44 (13) ◽  
pp. 10551-10561
Author(s):  
Hitanshu Kumar ◽  
Ke Wang ◽  
Fei Tang ◽  
Xierong Zeng ◽  
Lin Gan ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
Active Sites ◽  
Two Dimensional ◽  
Niobium Disulfide

Self-limited conversion of MoO2 into ultramicro MoS2 nanosheets on graphene/CNTs matrix for hydrogen evolution with excellent stability

2020 ◽  
Vol 4 (6) ◽  
pp. 2869-2874 ◽  
Author(s):  
Jingyang Tian ◽  
Jiaxin Li ◽  
Anlin Feng ◽  
Xinran Han ◽  
Yuancai Lv ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Active Sites ◽  
Mos2 Nanosheets ◽  
Excellent Stability

Ultramicro MoS2 nanosheets with abundant active sites were uniformly dispersed in rGO, which can be effectively separated by CNTs.

scholarly journals Ultra-Thin SnS2-Pt Nanocatalyst for Efficient Hydrogen Evolution Reaction

Nanomaterials ◽  
2020 ◽  
Vol 10 (12) ◽  
pp. 2337
Author(s):  
Yanying Yu ◽  
Jie Xu ◽  
Jianwei Zhang ◽  
Fan Li ◽  
Jiantao Fu ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
Active Sites ◽  
Transition Metal Dichalcogenides ◽  
Two Dimensional ◽  
Pt Nanoclusters ◽  
Two Dimensional Materials ◽  
Low Load ◽  
Metal Dichalcogenides ◽  
Poor Stability

Transition-metal dichalcogenides (TMDs) materials have attracted much attention for hydrogen evolution reaction (HER) as a new catalyst, but they still have challenges in poor stability and high reaction over-potential. In this study, Ultra-thin SnS2 nanocatalysts were synthesized by simple hydrothermal method, and low load of Pt was added to form stable SnS2-Pt-3 (the content of platinum is 0.5 wt %). The synergistic effect between ultra-thin SnS2 rich in active sites and individual dispersed Pt nanoclusters can significantly reduce the reaction barrier and further accelerate HER reaction kinetics. Hence, SnS2-Pt-3 exhibits a low overpotential of 210 mV at the current density of 10 mA cm−2. It is worth noting that SnS2-Pt-3 has a small Tafel slope (126 mV dec−1) in 0.5 M H2SO4, as well as stability. This work provides a new option for the application of TMDs materials in efficient hydrogen evolution reaction. Moreover, this method can be easily extended to other catalysts with desired two-dimensional materials.

Fluorination Activates the Basal Plane HER Activity of ReS2: A Combined Experimental and Theoretical Study

2021 ◽  
Author(s):  
Yonggang Liu ◽  
Haijing Li ◽  
Junfu Li ◽  
Xiaoshuang Ma ◽  
Zhiming Cui ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
Basal Plane ◽  
Active Sites ◽  
Theoretical Study ◽  
Two Dimensional ◽  
Catalytic Active Sites

Two-dimensional (2D) rhenium disulfide (ReS2) has been attracting immense interests as highly promising hydrogen evolution reaction (HER) electrocatalyst recently. However, the HER catalytic active sites of ReS2 are still limited...

Constructing tunable dual active sites on two-dimensional C3N4@MoN hybrid for electrocatalytic hydrogen evolution

Nano Energy ◽  
2018 ◽  
Vol 53 ◽  
pp. 690-697 ◽  
Author(s):  
Huanyu Jin ◽  
Xin Liu ◽  
Yan Jiao ◽  
Anthony Vasileff ◽  
Yao Zheng ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Active Sites ◽  
Two Dimensional
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