Large second harmonic generation from hollow gold nanoprisms: role of plasmon hybridization and structural effects

2017 ◽  
Vol 19 (28) ◽  
pp. 18394-18399 ◽  
Author(s):  
Bidhan Hazra ◽  
Kamalika Das ◽  
Manabendra Chandra
Keyword(s):  
Optical Properties ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Plasmon Hybridization ◽  
Structural Effects ◽  
Structure And Morphology ◽  
Gold Nanoprisms

The structure and morphology of nanomateials strongly influence their nonlinear optical properties.

K2Sn2ZnSe6, Na2Ge2ZnSe6, and Na2In2GeSe6: a new series of quaternary selenides with intriguing structural diversity and nonlinear optical properties

2016 ◽  
Vol 45 (18) ◽  
pp. 7627-7633 ◽  
Author(s):  
Molin Zhou ◽  
Chao Li ◽  
Xiaoshuang Li ◽  
Jiyong Yao ◽  
Yicheng Wu
Keyword(s):  
Optical Properties ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Structural Diversity ◽  
Nonlinear Optical Properties

New selenides K2Sn2ZnSe6, Na2Ge2ZnSe6, and Na2In2GeSe6 exhibit diverse structures and Na2In2GeSe6 possesses a moderate second harmonic generation response.

Second harmonic generation from alternate-layer LB films: quadratic enhancement with film thickness

1994 ◽  
Vol 445 (1924) ◽  
pp. 385-398 ◽  
Keyword(s):  
Optical Properties ◽  
Second Harmonic Generation ◽  
Film Thickness ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Lb Films ◽  
Langmuir Blodgett ◽  
Alternate Layer ◽  
Order Susceptibility

The second harmonic generation (SHG) from alternate-layer Langmuir-Blodgett (LB) films of stilbazolium dyes and 4, 4'-dioctadecyl-3, 5, 3', 5'-tetramethyldipyrryl-methene hydrobromide increases as I 2ω(N) = l 2ω(1) N 2 for N ≥ 2 bilayers, but the equivalent monolayer signal ( I 2ω(1) ) is significantly less than the intensity from LB monolayers of the corresponding dye on glass. This is attributed, in part, to the different molecular tilts and, in part, to the position of the anion which influences the charge distribution within the chromophore. For alternate-layer films of E-N-octadecyl-4-[2-(4-dimethylaminophenyl)ethenyl]pyridinium octadecylsulphate (dye I) the second-order susceptibility and chromophore tilt angle are χ (2) zzz = 45 pm V -1 and ϕ = 30° respectively, whereas the methoxy congener, E-N-octadecyl-4-[2-(4-methoxyphenyl)ethenyl]pyridinium octadecylsulphate (dye II), has χ (2) zzz = 11 Pm V -1 and ϕ = 35°. The nonlinear optical properties of such films are dependent upon the compatibility of the dye and spacer.

Investigation of the nonlinear optical properties of metamaterials by second harmonic generation

2011 ◽  
Vol 105 (1) ◽  
pp. 149-162 ◽  
Author(s):  
M. Gentile ◽  
M. Hentschel ◽  
R. Taubert ◽  
H. Guo ◽  
H. Giessen ◽  
...  
Keyword(s):  
Optical Properties ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Nonlinear Optical Properties

Polar potassium rare earth nitrates K2[RE(NO3)5(H2O)2] (RE = La, Ce, Pr and Nd). II. Linear and nonlinear optical properties

2000 ◽  
Vol 33 (2) ◽  
pp. 380-386 ◽  
Author(s):  
H. Hellwig ◽  
S. Rühle ◽  
P. Held ◽  
L. Bohatý
Keyword(s):  
Optical Properties ◽  
Rare Earth ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Point Group ◽  
Nonlinear Optical Properties ◽  
Rare Earth Nitrates ◽  
Linear And Nonlinear

Linear and nonlinear optical properties of the four isomorphic orthorhombic (point groupmm2) potassium rare earth nitrates K2[RE(NO3)5(H2O)2], with RE = La, Ce, Pr or Nd, have been investigated. Refractive indices in a wavelength range from 0.35 to 2.5 µm and the transmission spectra between 0.25 to 3.0 µm were measured. Using the Maker fringe technique, the d_{ijk}^{\rm\, SHG} coefficients of second-harmonic generation for a fundamental of the Nd–YAP laser (λ = 1079.5 nm) were determined for all four compounds. The d_{ijk}^{\rm\, SHG} coefficients of all four substances are about three times larger than those of KDP, as was first published by Ebberset al.[IEEE J. Quantum Electron.(1993),29, 497–507] for K2[La(NO3)5(H2O)2]. These nitrates are promising materials for application to nonlinear optics (e.g.second-harmonic generation of Nd laser radiation). The nonlinear optical properties of these compounds seem to have their origin mainly in the nitrate groups, as indicated by a simple model (summing the molecular hyperpolarizabilities of the NO3group). Neglecting local field effects, the hyperpolarizability of the NO3group was calculated as β222= 2.52 × 10−40 m4 V−1.

scholarly journals The Role of Surface Plasmon Resonance of Gold Nanoparticles for the Enhancement of Second Harmonic Generation of Nonlinear Chromophores

Inorganics ◽  
2019 ◽  
Vol 7 (5) ◽  
pp. 64 ◽  
Author(s):  
Anu Singh Bisht ◽  
Khuyen Hoang-Thi ◽  
Isabelle Ledoux-Rak ◽  
Hynd Remita ◽  
Frédéric Dumur ◽  
...  
Keyword(s):  
Gold Nanoparticles ◽  
Surface Plasmon Resonance ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Phenyl Ring ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Nlo Response ◽  
Spherical Gold Nanoparticles

A significant enhancement of the second harmonic generation (SHG) from second-order nonlinear optical (NLO) dyes in solution has been evidenced when these dyes were grafted onto the surface of spherical gold nanoparticles (AuNPs), as compared to their NLO response without AuNPs. The length, as well as the nature of the spacers between the gold particle and the chromophore, is shown to play an important role, a benzene linker being more favorable to AuNP-4-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) interactions, as illustrated by a higher exaltation of the NLO response for DAST molecules linked to AuNP via a phenyl ring as compared to their equivalent with a CH2–CH2 link.

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