Enhanced morphology and stability of high-performance perovskite solar cells with ultra-smooth surface and high fill factor via crystal growth engineering

2017 ◽  
Vol 1 (4) ◽  
pp. 907-914 ◽  
Author(s):  
Jiajiu Ye ◽  
Xuhui Zhang ◽  
Liangzheng Zhu ◽  
Haiying Zheng ◽  
Guozhen Liu ◽  
...  

We report a highly reproducible method for controlling perovskite crystal growth by a spraying anti-solvent process. A PCE of 19.21% was obtained, with a fill factor as high as 80.84%.

2020 ◽  
Vol 13 (7) ◽  
pp. 1971-1996 ◽  
Author(s):  
Weijie Chen ◽  
Xinqi Li ◽  
Yaowen Li ◽  
Yongfang Li

The key factors for high-quality all-inorganic perovskite crystal growth.


2018 ◽  
Vol 63 ◽  
pp. 207-215 ◽  
Author(s):  
Shao Jin ◽  
Yuelin Wei ◽  
Xiaomin Yang ◽  
Dan Luo ◽  
Yu Fang ◽  
...  

2017 ◽  
Vol 4 (12) ◽  
pp. 170980 ◽  
Author(s):  
Ya-Qiong Wang ◽  
Shou-Bin Xu ◽  
Jian-Guo Deng ◽  
Li-Zhen Gao

The interfacial compatibility between compact TiO 2 and perovskite layers is critical for the performance of planar heterojunction perovskite solar cells (PSCs). A compact TiO 2 film employed as an electron-transport layer (ETL) was modified using 3-aminopropyl trimethoxy silane (APMS) hydrolysate. The power conversion efficiency (PCE) of PSCs composed of an APMS-hydrolysate-modified TiO 2 layer increased from 13.45 to 15.79%, which was associated with a significant enhancement in the fill factor (FF) from 62.23 to 68.04%. The results indicate that APMS hydrolysate can enhance the wettability of γ-butyrolactone (GBL) on the TiO 2 surface, form a perfect CH 3 NH 3 PbI 3 film, and increase the recombination resistance at the interface. This work demonstrates a simple but efficient method to improve the TiO 2 /perovskite interface that can be greatly beneficial for developing high-performance PSCs.


2017 ◽  
Vol 9 (50) ◽  
pp. 43902-43909 ◽  
Author(s):  
Lijun Hu ◽  
Kuan Sun ◽  
Ming Wang ◽  
Wei Chen ◽  
Bo Yang ◽  
...  

2018 ◽  
Vol 6 (21) ◽  
pp. 9930-9937 ◽  
Author(s):  
Haiying Zheng ◽  
Liangzheng Zhu ◽  
Linhua Hu ◽  
Shangfeng Yang ◽  
Shuanghong Chen ◽  
...  

By introducing CH3CONH2 as an additive, perovskite solar cells showed an improved PCE of 19.01%, with high humidity and heat stability.


Author(s):  
Peng Gao ◽  
Lusheng Liang ◽  
Naoyuki Shibayama ◽  
Haiying Jiang ◽  
Zilong Zhang ◽  
...  

Developing high-performance dopant-free hole transport material (DF-HTM) is critical to realizing stable perovskite solar cells (PSCs). Herein, a class of siloxane-terminated polymers (PBZ-Si) with low surface energy were studied as...


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