A novel ligand with –NH2 and –COOH-decorated Co/Fe-based oxide for an efficient overall water splitting: dual modulation roles of active sites and local electronic structure

2020 ◽  
Vol 10 (18) ◽  
pp. 6266-6273
Author(s):  
Yalan Zhang ◽  
Zebin Yu ◽  
Ronghua Jiang ◽  
Jung Huang ◽  
Yanping Hou ◽  
...  
Keyword(s):  
Electronic Structure ◽  
Water Splitting ◽  
Energy Demand ◽  
Active Sites ◽  
Electrode Materials ◽  
Global Energy ◽  
Overall Water Splitting ◽  
Local Electronic Structure ◽  
Electrochemical Water Splitting

Excellent electrochemical water splitting with remarkable durability can provide a solution to satisfy the increasing global energy demand in which the electrode materials play an important role.

Achieving electronic structure reconfiguration in metallic carbides for robust electrochemical water splitting

2020 ◽  
Vol 8 (5) ◽  
pp. 2453-2462 ◽  
Author(s):  
Lulu Qiao ◽  
Anquan Zhu ◽  
Weixuan Zeng ◽  
Rui Dong ◽  
Pengfei Tan ◽  
...  
Keyword(s):  
Electronic Structure ◽  
Water Splitting ◽  
Active Sites ◽  
Metallic Copper ◽  
Structure Modification ◽  
Dual Source ◽  
Electrochemical Water Splitting

The electronic structure modification of metallic carbide is achieved by introducing dual-source transition metallic copper and cobalt atoms, thus contributing abundant active sites to afford decent water splitting performances.

scholarly journals Fe(III) Ions-Assisted Aniline Polymerization Strategy to Nitrogen-Doped Carbon-Supported Bimetallic CoFeP Nanospheres as Efficient Bifunctional Electrocatalysts toward Overall Water Splitting

Materials ◽  
2021 ◽  
Vol 14 (6) ◽  
pp. 1473
Author(s):  
Changhao Zhao ◽  
Fen Wei ◽  
Haolin Lv ◽  
Dengke Zhao ◽  
Nan Wang ◽  
...  
Keyword(s):  
Water Splitting ◽  
Water Oxidation ◽  
Active Sites ◽  
Alkaline Media ◽  
Alkaline Electrolyte ◽  
Nitrogen Doped ◽  
Overall Water Splitting ◽  
Electrochemical Water Splitting ◽  
Acidic And Alkaline Media ◽  
Aniline Polymerization

It remains an urgent demand and challenging task to design and fabricate efficient, stable, and inexpensive catalysts toward sustainable electrochemical water splitting for hydrogen production. Herein, we explored the use of Fe(III) ion-assisted aniline polymerization strategy to embed bimetallic CoFeP nanospheres into the nitrogen-doped porous carbon framework (referred CoFeP-NC). The as-prepared CoFeP-NC possesses excellent hydrogen evolution reaction (HER) performance with the small overpotential (η10) of 81 mV and 173 mV generated at a current density of 10 mA cm−2 in acidic and alkaline media, respectively. Additionally, it can also efficiently catalyze water oxidation (OER), which shows an ideal overpotential (η10) of 283 mV in alkaline electrolyte (pH = 14). The remarkable catalytic property of CoFeP-NC mainly stems from the strong synergetic effects of CoFeP nanospheres and carbon network. On the one hand, the interaction between the two can make better contact between the electrolyte and the catalyst, thereby providing a large number of available active sites. On the other hand, it can also form a network to offer better durability and electrical conductivity (8.64 × 10−1 S cm−1). This work demonstrates an efficient method to fabricate non-noble electrocatalyst towards overall water splitting, with great application prospect.

Construction of Fe-doped CoP with hybrid nanostructures as a bifunctional catalyst for overall water splitting

2021 ◽  
Author(s):  
Qinghua Yang ◽  
Jiang Dai ◽  
Wenhao Liao ◽  
Xianfeng Tong ◽  
Yan Fu ◽  
...  
Keyword(s):  
Water Splitting ◽  
Active Sites ◽  
Bifunctional Catalyst ◽  
Hybrid Nanostructures ◽  
Overall Water Splitting ◽  
Electrochemical Water Splitting

With the open skeleton structures, adjustable active sites and homogeneous catalytic centers, PBA-based materials had promising applications in electrochemical water splitting. Herein, we reported a PBA derived Fe0.25-CoP electrocatalyst with...

Construction of hierarchical IrTe nanotubes with assembled nanosheets for overall water splitting electrocatalysis

2021 ◽  
Author(s):  
Ziqiang Wang ◽  
Peng Wang ◽  
Hugang Zhang ◽  
Wenjing Tian ◽  
You Xu ◽  
...  
Keyword(s):  
Water Splitting ◽  
Oxygen Evolution ◽  
Bifunctional Catalysts ◽  
Overall Water Splitting ◽  
Electrochemical Water Splitting

The design of efficient bifunctional catalysts for hydrogen and oxygen evolution reactions is significant for electrochemical water splitting. Here, hierarchical IrTe nanotubes (NTs) with assembled nanosheets have been prepared through...

Amine-functionalized multi-walled carbon nanotubes (EDA-MWCNTs) for electrochemical water splitting reactions

2021 ◽  
Author(s):  
Shankar S. Narwade ◽  
Shivsharan M. Mali ◽  
Bhaskar R. Sathe
Keyword(s):  
Carbon Nanotubes ◽  
Water Splitting ◽  
Metal Free ◽  
Overall Water Splitting ◽  
Amine Functionalized ◽  
Multi Walled Carbon Nanotubes ◽  
Electrochemical Water Splitting ◽  
Walled Carbon Nanotubes

A study on the in situ decoration of ethylenediamine (EDA) on acid functionalized multi-walled carbon nanotubes (O-MWCNTs) for overall water splitting reactions at all pH as an efficient and inexpensive metal-free multifunctional electrocatalyst.

Electronic Structure Basis for Enhanced Overall Water Splitting Photocatalysis of Doped Strontium Titanate in Direct Sunlight

2018 ◽  
Author(s):  
Frank Osterloh ◽  
Zeqiong Zhao ◽  
Renato Gonçalves ◽  
Muhammad Huda ◽  
Sajib Barman ◽  
...  
Keyword(s):  
Electronic Structure ◽  
Water Splitting ◽  
Strontium Titanate ◽  
Direct Sunlight ◽  
Overall Water Splitting

Tuning the electronic structure of NiCoVOx nanosheets through S doping for enhanced oxygen evolution

Nanoscale ◽  
2021 ◽  
Author(s):  
Haibin Ma ◽  
ChangNing SUN ◽  
Zhili Wang ◽  
Qing Jiang
Keyword(s):  
Electronic Structure ◽  
Water Splitting ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Low Cost ◽  
Ni Foam ◽  
Electrochemical Water Splitting

It is of great importance to develop efficient and low-cost oxygen evolution reaction (OER) electrocatalysts for electrochemical water splitting. Herein, S doped NiCoVOx nanosheets grown on Ni-Foam (S-NiCoVOx/NF) with modified...

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