Suppression of external quantum efficiency roll-off of nanopatterned organic-light emitting diodes at high current densities

2015 ◽  
Vol 118 (15) ◽  
pp. 155501 ◽  
Author(s):  
Hiroyuki Kuwae ◽  
Atsushi Nitta ◽  
Kou Yoshida ◽  
Takashi Kasahara ◽  
Toshinori Matsushima ◽  
...  
2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Buddhika S. B. Karunathilaka ◽  
Umamahesh Balijapalli ◽  
Chathuranganie A. M. Senevirathne ◽  
Seiya Yoshida ◽  
Yu Esaki ◽  
...  

Abstract Large external quantum efficiency rolloff at high current densities in organic light-emitting diodes (OLEDs) is frequently caused by the quenching of radiative singlet excitons by long-lived triplet excitons [singlet–triplet annihilation (STA)]. In this study, we adopted a triplet scavenging strategy to overcome the aforementioned STA issue. To construct a model system for the triplet scavenging, we selected 2,6-dicyano-1,1-diphenyl-λ5σ4-phosphinine (DCNP) as the emitter and 4,4′-bis[(N-carbazole)styryl]biphenyl (BSBCz) as the host material by considering their singlet and triplet energy levels. In this system, the DCNP’s triplets are effectively scavenged by BSBCz while the DCNP’s singlets are intact, resulting in the suppressed STA under electrical excitation. Therefore, OLEDs with a 1 wt.%-DCNP-doped BSBCz emitting layer demonstrated the greatly suppressed efficiency rolloff even at higher current densities. This finding favourably provides the advanced light-emitting performance for OLEDs and organic semiconductor laser diodes from the aspect of the suppressed efficiency rolloff.


2001 ◽  
Vol 665 ◽  
Author(s):  
Masamichi Ikai ◽  
Yasunori Taga

ABSTRACTWe present our recent findings on the development of organic light emitting diodes (OLEDs). One of the keys to highly efficient phosphorescent emission in organic light-emitting diodes is to confine triplet excitons generated within the emitting layer. To confine triplet excitons, we employ perfluorinated phenylene dendrimers (C60F42) as a both hole- and exciton-block layer, and a hole-transport material (4,4',4”-tris(N-carbazolyl) triphenylamine [TCTA]) as a host for the phosphorescent dopant, Ir(ppy)3, in the emitting layer. The maximum external quantum efficiency reaches to 19.2%, and is over 15% even at high injection current densities of 10 to 20 mA/cm2, where the brightness of the device reaches to approximately 10,000 cd/m2.


2017 ◽  
Vol 5 (23) ◽  
pp. 5749-5756 ◽  
Author(s):  
Lingcheng Chen ◽  
Shumeng Wang ◽  
Zhimin Yan ◽  
Junqiao Ding ◽  
Lixiang Wang

By fully encapsulating the heteroleptic red Ir complex with carbazole dendrons, solution-processed nondoped electrophosphorescent devices reveal over 10% EQE.


2018 ◽  
Vol 2 (1) ◽  
Author(s):  
Fatemeh Maasoumi ◽  
Ross D. Jansen-van Vuuren ◽  
Paul E. Shaw ◽  
Emma V. Puttock ◽  
Ravi Chandra Raju Nagiri ◽  
...  

2013 ◽  
Vol 23 (31) ◽  
pp. 3896-3900 ◽  
Author(s):  
Sei-Yong Kim ◽  
Won-Ik Jeong ◽  
Christian Mayr ◽  
Young-Seo Park ◽  
Kwon-Hyeon Kim ◽  
...  

2018 ◽  
Vol 47 (22) ◽  
pp. 7587-7593 ◽  
Author(s):  
Ning Su ◽  
Zheng-Guang Wu ◽  
You-Xuan Zheng

Two efficient bluish green iridium(iii) complexes were applied as emitters in the organic light-emitting diodes, which showing high current efficiency of 58.17 cd A−1 and external quantum efficiency of 25.33% with low efficiency roll-off.


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