Integrated Radionuclide Transport Model for a High-Level Waste Repository in Water-Saturated Geologic Formations

1998 ◽  
Vol 121 (1) ◽  
pp. 24-39 ◽  
Author(s):  
Joonhong Ahn
1984 ◽  
Vol 44 ◽  
Author(s):  
C. Pescatore ◽  
T. Sullivan

AbstractRadionuclides breakthrough times as calculated through constant retardation factors obtained in dilute solutions are non-conservative. The constant retardation approach regards the solid as having infinite sorption capacity throughout the solid. However, as the solid becomes locally saturated, such as in the proximity of the waste form-packing materials interface, it will exhibit no retardation properties, and transport will take place as if the radionuclides were locally non-reactive. The magnitude of the effect of finite sorption capacity of the packing materials on radionuclide transport is discussed with reference to high-level waste package performance. An example based on literature sorption data indicates that the breakthrough time may be overpredicted by orders of magnitude using a constant retardation factor as compared to using the entire sorption isotherm to obtain a concentrationdependent retardation factor.


1992 ◽  
Vol 294 ◽  
Author(s):  
A. Saotome ◽  
K. Hara ◽  
J. Okamoto

ABSTRACTShaft sealing in a high-level waste(HLW) disposal system functions to minimize the water flow passage, and retard the radionuclide transport from the repository to the accessible environment. It is important to estimate the radionuclide migration along the sealed shaft from the viewpoint of the design and the performance assessment of the sealing system.This study presents the results of sensitivity analyses on the radionuclide migration in the vicinity of the access shaft of a repository in order to evaluate the effects of the length of a plug, as well as the number of plugs, and curtain grouts.In this study, the upward hydraulic gradient of the groundwater flow along shafts was used, based on transient coupled thermo-hydraulic analyses around a repository. Hydraulic conductivities of the backfill material and the disturbed zones around the shaft tunnels were also assumed to be one order and two orders of magnitude higher than that of the host rock, respectively.The results show that the velocity of the groundwater within the shaft and the disturbed zone is reduced by a factor of one third by installing a few plugs into the shaft filled with backfill material. The curtain grouts have the effect of retarding the radionuclide migration from the repository to the ground surface at a factor of approximately five. A few plug installations have the same effect. The sealing system properly constituted with backfill, plugs, and grouts can provide the same performance as the original host rock.


2000 ◽  
Vol 663 ◽  
Author(s):  
D.K. Smith ◽  
A.B. Kersting ◽  
J.L. Thompson ◽  
D.L. Finnegan

ABSTRACTUnderground nuclear test sites offer an unprecedented opportunity to evaluate processes relevant to high-level waste repository performance in the absence of engineered barriers. Radionuclide migration programs at the Nevada Test Site represent a twenty-five year systematic investigation of the diverse radiologic source terms residual from weapons testing and the evolution of the hydrologic source term which comprises those radionuclides dissolved in or otherwise available for transport by groundwater. The Nevada Test Site shares actinide source terms, correlative geology, an identical tectonic setting, similar climate, and a thick unsaturated zone with the adjacent potential Yucca Mountain high-level waste repository and provides a natural laboratory to assess long-term radionuclide transport in the near field. Analog studies may ultimately help validate predictions of radionuclide transport from the potential Yucca Mountain repository.


1995 ◽  
Vol 412 ◽  
Author(s):  
C. Oda ◽  
H. Yoshikawa ◽  
M. Yui

AbstractPalladium solubility was measured in a dilute aqueous solution at room temperature in the pH range from 3 to 13 under anaerobic conditions. Crystalline Pd metal was clearly visible and the concentration of palladium in solution decreased gradually with aging time. The palladium concentrations in solution were less than 9.4×10-10M in the pH range from 4 to 10 and increased to 10-7M in the pH range greater than 10. This study suggests that palladium concentrations in certain high-level waste repository environments may be limited by Pd metal and may be less than 10-9M.


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