Time-resolved imaging of CaF2 poly-crystal response following 355 nm nanosecond laser irradiation

Author(s):  
Jiuling Meng ◽  
Tao Lü ◽  
Yong Jiang ◽  
Rong Qiu
2016 ◽  
Vol 108 (21) ◽  
pp. 211602 ◽  
Author(s):  
Dongfeng Qi ◽  
Dongwoo Paeng ◽  
Junyeob Yeo ◽  
Eunpa Kim ◽  
Letian Wang ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Yao Lu ◽  
Qi Zhang ◽  
Qiang Wu ◽  
Zhigang Chen ◽  
Xueming Liu ◽  
...  

AbstractThe field of nonlinear optics has grown substantially in past decades, leading to tremendous progress in fundamental research and revolutionized applications. Traditionally, the optical nonlinearity for a light wave at frequencies beyond near-infrared is observed with very high peak intensity, as in most materials only the electronic nonlinearity dominates while ionic contribution is negligible. However, it was shown that the ionic contribution to nonlinearity can be much larger than the electronic one in microwave experiments. In the terahertz (THz) regime, phonon polariton may assist to substantially trigger the ionic nonlinearity of the crystals, so as to enhance even more the nonlinear optical susceptibility. Here, we experimentally demonstrate a giant second-order optical nonlinearity at THz frequency, orders of magnitude higher than that in the visible and microwave regimes. Different from previous work, the phonon-light coupling is achieved under a phase-matching setting, and the dynamic process of nonlinear THz generation is directly observed in a thin-film waveguide using a time-resolved imaging technique. Furthermore, a nonlinear modification to the Huang equations is proposed to explain the observed nonlinearity enhancement. This work brings about an effective approach to achieve high nonlinearity in ionic crystals, promising for applications in THz nonlinear technologies.


Nanoscale ◽  
2018 ◽  
Vol 10 (43) ◽  
pp. 20108-20112 ◽  
Author(s):  
Tae-Hyeon Park ◽  
Du-Jeon Jang

Hollow and porous gold nanoshells with high surface-enhanced Raman scattering efficiency have been fabricated through utilizing nanosecond laser irradiation.


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