An experimental study is carried out to investigate the three-dimensional instantaneous structure of an incident shock wave/turbulent boundary layer interaction at Mach 2.1 using tomographic particle image velocimetry. Large-scale coherent motions within the incoming boundary layer are observed, in the form of three-dimensional streamwise-elongated regions of relatively low- and high-speed fluid, similar to what has been reported in other supersonic boundary layers. Three-dimensional vortical structures are found to be associated with the low-speed regions, in a way that can be explained by the hairpin packet model. The instantaneous reflected shock wave pattern is observed to conform to the low- and high-speed regions as they enter the interaction, and its organization may be qualitatively decomposed into streamwise translation and spanwise rippling patterns, in agreement with what has been observed in direct numerical simulations. The results are used to construct a conceptual model of the three-dimensional unsteady flow organization of the interaction.