scholarly journals Impact of El Niño–Southern Oscillation on the interannual variability of methane and tropospheric ozone

2019 ◽  
Vol 19 (13) ◽  
pp. 8669-8686 ◽  
Author(s):  
Matthew J. Rowlinson ◽  
Alexandru Rap ◽  
Stephen R. Arnold ◽  
Richard J. Pope ◽  
Martyn P. Chipperfield ◽  
...  
Keyword(s):  
Growth Rate ◽  
Interannual Variability ◽  
Biomass Burning ◽  
El Niño ◽  
Tropospheric Ozone ◽  
El Nino ◽  
Southern Oscillation ◽  
Fire Emissions ◽  
Tropospheric O3 ◽  
Global Mean

Abstract. The interannual variability of the greenhouse gases methane (CH4) and tropospheric ozone (O3) is largely driven by natural variations in global emissions and meteorology. The El Niño–Southern Oscillation (ENSO) is known to influence fire occurrence, wetland emission and atmospheric circulation, affecting sources and sinks of CH4 and tropospheric O3, but there are still important uncertainties associated with the exact mechanism and magnitude of this effect. Here we use a modelling approach to investigate how fires and meteorology control the interannual variability of global carbon monoxide (CO), CH4 and O3 concentrations, particularly during large El Niño events. Using a three-dimensional chemical transport model (TOMCAT) coupled to a sophisticated aerosol microphysics scheme (GLOMAP) we simulate changes to CO, hydroxyl radical (OH) and O3 for the period 1997–2014. We then use an offline radiative transfer model to quantify the climate impact of changes to atmospheric composition as a result of specific drivers. During the El Niño event of 1997–1998, there were increased emissions from biomass burning globally, causing global CO concentrations to increase by more than 40 %. This resulted in decreased global mass-weighted tropospheric OH concentrations of up to 9 % and a consequent 4 % increase in the CH4 atmospheric lifetime. The change in CH4 lifetime led to a 7.5 ppb yr−1 increase in the global mean CH4 growth rate in 1998. Therefore, biomass burning emission of CO could account for 72 % of the total effect of fire emissions on CH4 growth rate in 1998. Our simulations indicate that variations in fire emissions and meteorology associated with El Niño have opposing impacts on tropospheric O3 burden. El Niño-related changes in atmospheric transport and humidity decrease global tropospheric O3 concentrations leading to a −0.03 W m−2 change in the O3 radiative effect (RE). However, enhanced fire emission of precursors such as nitrogen oxides (NOx) and CO increase O3 and lead to an O3 RE of 0.03 W m−2. While globally the two mechanisms nearly cancel out, causing only a small change in global mean O3 RE, the regional changes are large – up to −0.33 W m−2 with potentially important consequences for atmospheric heating and dynamics.

scholarly journals Impact of El Niño Southern Oscillation on the interannual variability of methane and tropospheric ozone

2019 ◽  
Author(s):  
Matthew J. Rowlinson ◽  
Alexandru Rap ◽  
Stephen R. Arnold ◽  
Richard J. Pope ◽  
Martyn P. Chipperfield ◽  
...  
Keyword(s):  
Growth Rate ◽  
Interannual Variability ◽  
Biomass Burning ◽  
El Niño ◽  
Atmospheric Transport ◽  
El Nino ◽  
Southern Oscillation ◽  
Fire Emissions ◽  
Tropospheric O3 ◽  
Global Mean

Abstract. The growth rate of global methane (CH4) concentrations has a strong interannual variability which is believed to be driven largely by fluctuations in CH4 emissions from wetlands and wildfires, as well as changes to the atmospheric sink. The El Niño Southern Oscillation (ENSO) is known to influence fire occurrence, wetland emission and atmospheric transport, but there are still important uncertainties associated with the exact mechanism and magnitude of this influence. Here we use a modelling approach to investigate how fires and meteorology control the interannual variability of global carbon monoxide (CO), CH4 and ozone (O3) concentrations, particularly during large El Niño events. Using a three-dimensional chemical transport model (TOMCAT) coupled to a sophisticated aerosol microphysics scheme (GLOMAP) we simulate changes to CO, hydroxyl radical (OH) and O3 for the period 1997–2014. We then use an offline radiative transfer model to quantify the impact of changes to atmospheric composition as a result of specific drivers. During the El Niño event of 1997–1998, there were increased emissions from biomass burning globally. As a result, global CO concentrations increased by more than 40 %. This resulted in decreased global mass-weighted tropospheric OH concentrations of up to 9 % and a resulting 4 % increase in the CH4 atmospheric lifetime. The change in CH4 lifetime led to a 7.5 ppb yr−1 increase in global mean CH4 growth rate in 1998. Therefore biomass burning emission of CO could account for 72 % of the total effect of fire emissions on CH4 growth rate in 1998. Our simulations indicate variations in fire emissions and meteorology associated with El Niño have opposing impacts on tropospheric O3 burden. El Niño-related atmospheric transport changes decrease global tropospheric O3 concentrations leading to a −0.03 Wm−2 change in O3 radiative effect (RE). However, enhanced fire emission of precursors such as nitrous oxides (NOx) and CO increase O3 RE by 0.03 Wm−2. While globally the two mechanisms nearly cancel out, causing only a small change in global mean O3 RE, the regional changes are large   up to −0.33 Wm−2 with potentially important consequences for atmospheric heating and dynamics.

scholarly journals Limited impact of El Niño–Southern Oscillation on variability and growth rate of atmospheric methane

2018 ◽  
Vol 15 (21) ◽  
pp. 6371-6386 ◽  
Author(s):  
Hinrich Schaefer ◽  
Dan Smale ◽  
Sylvia E. Nichol ◽  
Tony M. Bromley ◽  
Gordon W. Brailsford ◽  
...  
Keyword(s):  
Climate Change ◽  
Growth Rate ◽  
Biomass Burning ◽  
El Niño ◽  
El Nino ◽  
Southern Oscillation ◽  
El Nino Southern Oscillation ◽  
Atmospheric Methane ◽  
Ch4 Production ◽  
A Minor

Abstract. The El Niño–Southern Oscillation (ENSO) has been suggested as a strong forcing in the methane cycle and as a driver of recent trends in global atmospheric methane mole fractions [CH4]. Such a sensitivity of the global CH4 budget to climate events would have important repercussions for climate change mitigation strategies and the accuracy of projections for future greenhouse forcing. Here, we test the impact of ENSO on atmospheric CH4 in a correlation analysis. We use local and global records of [CH4], as well as stable carbon isotopic records of atmospheric CH4 (δ13CH4), which are particularly sensitive to the combined ENSO effects on CH4 production from wetlands and biomass burning. We use a variety of nominal, smoothed, and detrended time series including growth rate records. We find that at most 36 % of the variability in [CH4] and δ13CH4 is attributable to ENSO, but only for detrended records in the southern tropics. Trend-bearing records from the southern tropics, as well as all studied hemispheric and global records, show a minor impact of ENSO, i.e. < 24 % of variability explained. Additional analyses using hydrogen cyanide (HCN) records show a detectable ENSO influence on biomass burning (up to 51 %–55 %), suggesting that it is wetland CH4 production that responds less to ENSO than previously suggested. Dynamics of the removal by hydroxyl likely counteract the variation in emissions, but the expected isotope signal is not evident. It is possible that other processes obscure the ENSO signal, which itself indicates a minor influence of the latter on global CH4 emissions. Trends like the recent rise in atmospheric [CH4] can therefore not be attributed to ENSO. This leaves anthropogenic methane sources as the likely driver, which must be mitigated to reduce anthropogenic climate change.

scholarly journals Effects of the 2006 El Niño on tropospheric ozone and carbon monoxide: implications for dynamics and biomass burning

2009 ◽  
Vol 9 (13) ◽  
pp. 4239-4249 ◽  
Author(s):  
S. Chandra ◽  
J. R. Ziemke ◽  
B. N. Duncan ◽  
T. L. Diehl ◽  
N. J. Livesey ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Atmospheric Chemistry ◽  
Forest Fires ◽  
El Niño ◽  
Tropospheric Ozone ◽  
Large Scale ◽  
El Nino ◽  
Global Burden ◽  
The North ◽  
Tropospheric O3

Abstract. We have studied the effects of the 2006 El Niño on tropospheric O3 and CO at tropical and sub-tropical latitudes measured from the OMI and MLS instruments on the Aura satellite. The 2006 El Niño-induced drought caused forest fires (largely set to clear land) to burn out of control during October and November in the Indonesian region. The effects of these fires are clearly seen in the enhancement of CO concentration measured from the MLS instrument. We have used a global model of atmospheric chemistry and transport (GMI CTM) to quantify the relative importance of biomass burning and large scale transport in producing observed changes in tropospheric O3 and CO. The model results show that during October and November biomass burning and meteorological changes contributed almost equally to the observed increase in tropospheric O3 in the Indonesian region. The biomass component was 4–6 DU but it was limited to the Indonesian region where the fires were most intense. The dynamical component was 4–8 DU but it covered a much larger area in the Indian Ocean extending from South East Asia in the north to western Australia in the south. By December 2006, the effect of biomass burning was reduced to zero and the observed changes in tropospheric O3 were mostly due to dynamical effects. The model results show an increase of 2–3% in the global burden of tropospheric ozone. In comparison, the global burden of CO increased by 8–12%.

scholarly journals Effects of the 2006 El Niño on tropospheric ozone and carbon monoxide: implications for dynamics and biomass burning

2009 ◽  
Vol 9 (1) ◽  
pp. 2735-2761
Author(s):  
S. Chandra ◽  
J. R. Ziemke ◽  
B. N. Duncan ◽  
T. L. Diehl ◽  
N. J. Livesey ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Atmospheric Chemistry ◽  
Forest Fires ◽  
El Niño ◽  
Tropospheric Ozone ◽  
Large Scale ◽  
El Nino ◽  
Global Burden ◽  
The North ◽  
Tropospheric O3

Abstract. We have studied the effects of the 2006 El Niño on tropospheric O3 and CO at tropical and sub-tropical latitudes measured from the OMI and MLS instruments on the Aura satellite. The 2006 El Niño-induced drought allowed forest fires set to clear land to burn out of control during October and November in the Indonesian region. The effects of these fires are clearly seen in the enhancement of CO concentration measured from the MLS instrument. We have used a global model of atmospheric chemistry and transport (GMI CTM) to quantify the relative importance of biomass burning and large scale transport in producing observed changes in tropospheric O3 and CO. The model results show that during October and November both biomass burning and meteorological changes contributed almost equally to the observed increase in tropospheric O3 in the Indonesian region. The biomass component was 4–6 DU but it was limited to the Indonesian region where the fires were most intense. The dynamical component was 4–8 DU but it covered a much larger area in the Indian Ocean extending from South East Asia in the north to western Australia in the south. By December 2006, the effect of biomass burning was reduced to zero and the observed changes in tropospheric O3 were mostly due to dynamical effects. The model results show an increase of 2–3% in the global burden of tropospheric ozone. In comparison, the global burden of CO increased by 8–12%.

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