scholarly journals Supplementary material to "Compositions and mixing states of aerosol particles by aircraft observations in the Arctic springtime, 2018"

Author(s):  
Kouji Adachi ◽  
Naga Oshima ◽  
Sho Ohata ◽  
Atsushi Yoshida ◽  
Nobuhiro Moteki ◽  
...  
Author(s):  
Peter K. Peterson ◽  
Denis Pöhler ◽  
Holger Sihler ◽  
Johannes Zielcke ◽  
Stephan General ◽  
...  

2005 ◽  
Vol 5 (3) ◽  
pp. 767-779 ◽  
Author(s):  
T. Petäjä ◽  
V.-M. Kerminen ◽  
K. Hämeri ◽  
P. Vaattovaara ◽  
J. Joutsensaari ◽  
...  

Abstract. Hygroscopicity (i.e. water vapour affinity) of atmospheric aerosol particles is one of the key factors in defining their impacts on climate. Condensation of sulphuric acid onto less hygroscopic particles is expected to increase their hygrocopicity and hence their cloud condensation nuclei formation potential. In this study, differences in the hygroscopic and ethanol uptake properties of ultrafine aerosol particles in the Arctic air masses with a different exposure to anthropogenic sulfur pollution were examined. The main discovery was that Aitken mode particles having been exposed to polluted air were more hygroscopic and less soluble to ethanol than after transport in clean air. This aging process was attributed to sulphur dioxide oxidation and subsequent condensation during the transport of these particle to our measurement site. The hygroscopicity of nucleation mode aerosol particles, on the other hand, was approximately the same in all the cases, being indicative of a relatively similar chemical composition despite the differences in air mass transport routes. These particles had also been produced closer to the observation site typically 3–8 h prior to sampling. Apparently, these particles did not have an opportunity to accumulate sulphuric acid on their way to the site, but instead their chemical composition (hygroscopicity and ethanol solubility) resembled that of particles produced in the local or semi-regional ambient conditions.


2019 ◽  
Author(s):  
Jutta E. Wollenburg ◽  
Morten Iversen ◽  
Christian Katlein ◽  
Thomas Krumpen ◽  
Marcel Nicolaus ◽  
...  

2011 ◽  
Vol 11 (4) ◽  
pp. 12411-12440 ◽  
Author(s):  
A. R. Russell ◽  
A. E. Perring ◽  
L. C. Valin ◽  
E. Bucsela ◽  
E. C. Browne ◽  
...  

Abstract. We present a new retrieval of tropospheric NO2 vertical column density from the Ozone Monitoring Instrument (OMI) based on high spatial and temporal resolution terrain and profile inputs. We find non-negligible impacts on the retrieved NO2 column for terrain pressure (±20%), albedo (±40%), and NO2 vertical profile (−75%–+10%). We compare our NO2 product, the Berkeley High-Resolution (BEHR) product, with operational retrievals and find that the operational retrievals are biased high (30%) over remote areas and biased low (8%) over urban regions. We validate the operational and BEHR products using boundary layer aircraft observations from the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS-CA) field campaign which occurred in June 2008 in California. Results indicate that columns derived using our boundary layer extrapolation method show good agreement with satellite observations (R2 = 0.65–0.83; N = 68) and provide a more robust validation of satellite-observed NO2 column than those determined using full vertical spirals (R2 = 0.26; N = 5) as in previous work. Agreement between aircraft observations and the BEHR product (R2 = 0.83) is better than agreement with the operational products (R2 = 0.65–0.72). We also show that agreement between satellite and aircraft observations for all products can be further improved (e.g. BEHR: R2 = 0.91) using cloud information from the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument instead of the OMI cloud product. These results indicate that much of the variance in the operational products can be attributed to coarse resolution terrain and profile parameters.


2019 ◽  
Author(s):  
Xiaoli Shen ◽  
Heike Vogel ◽  
Bernhard Vogel ◽  
Wei Huang ◽  
Claudia Mohr ◽  
...  

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