222Rn Exhalation Rates from Some Granite and Marble Used in Korea: Preliminary Study

The objective of this study was to establish a test method for assessing radon exhalation rates from building materials considering radon related environmental policy and research in Korea. This method was established in consideration of cost-effectiveness based on the International Standards Organization (ISO) method and the closed chamber method, which is an evaluation method for the emission of hazardous chemical substances from building materials in Korea. The assessment of radon exhalation rates from five types each of granite and marble used in the construction industry in Korea gave mean radon exhalation rates of 0.497 ± 0.467 Bq/m2∙h from granite and 0.193 ± 0.113 Bq/m2∙h from marble, indicating higher radon exhalation rates from granite. These results are consistent with those of a previous study, indicating that granites are more likely to show higher radon exhalation rates than marbles.

Influence of the accumulation chamber insertion depth to measure surface radon exhalation rates

<p>A common method to measure radon exhalation rates relies on the accumulation chamber technique. Usually, this approach only considers one-dimensional gas transport within the soil that neglects lateral diffusion. However, this lateral transport could reduce the reliability of the method. In this work, several cylindrical- shaped accumulation chambers were built with different heights to test if the insertion depth of the chamber into the soil improves the reliability of the method and, in that case, if it could limit the radon lateral diffusion effects. To check this hypothesis in laboratory, two reference exhalation boxes were manufactured using phospho- gypsum from a repository located nearby the city of Huelva, in the southwest of Spain. Laboratory experiments showed that insertion depth had a deep impact in reducing the effective decay constant of the system, extending the interval where the linear fitting can be applied, and consistently obtaining reliable exhalation measurements once a minimum insertion depth is employed. Field experiments carried out in the phosphogypsum repository showed that increasing the insertion depth could reduce the influence of external effects, increasing the re- peatability of the method. These experiments provided a method to obtain consistent radon exhalation mea- surements over the phosphogypsum repository.</p>

Long-Term Measurements of Radon and Thoron Exhalation Rates from the Ground Using the Vertical Distributions of Their Activity Concentrations

A long-term measurement technique of radon exhalation rate was previously developed using a passive type radon and thoron discriminative monitor and a ventilated type accumulation chamber. In the present study, this technique was applied to evaluate the thoron exhalation rate as well, and long-term measurements of radon and thoron exhalation rates were conducted for four years in Gifu Prefecture. The ventilated type accumulation chamber (0.8 × 0.8 × 1.0 m3) with an open bottom was embedded 15 cm into the ground. The vertical distributions of radon and thoron activity concentrations from the ground were obtained using passive type radon-thoron discriminative monitors (RADUETs). The RADUETs were placed at 1, 3, 10, 30, and 80 cm above the ground inside the accumulation chamber. The measurements were conducted from autumn 2014 to autumn 2018. These long-term results were found to be in good agreement with the values obtained by another methodology. The radon exhalation rates from the ground showed a clearly seasonal variation. Similar to findings of previous studies, radon exhalation rates from summer to autumn were relatively higher than those from winter to spring. In contrast, thoron exhalation rates were not found to show seasonal variation.

Measurements of radon exhalation from a South African gold mine tailings using sealed tube method

To date, approximately 6000 tons of uranium has been disposed of onto tailings dams per year by gold mining activities in South Africa. These uranium bearing tailings dumps contain significant amounts of radium and are therefore possible sources of substantial amounts of radon gas. Due to the large sizes of these dams, measurements of the radon exhalation for the whole dam using established and conventional methods become time consuming and labour intensive. In this study, radon exhalation rates from a gold mine tailings dam around mining area of Odendalsrus were measured using passive “sealed tube” method and CR-39 gas etched track monitors known as Radon Gas Monitors (RGMs). Twenty samples were collected at the depths ranging from 90 cm to 1 m from the tailings for exhalation rate measurements. Radon exhalation rates from these samples were found to vary from 0.0410 ± 0.0042 Bq/m2 · s to 0.440 ± 0.045 Bq/m2 · s with a mean value of 0.102 ± 0.021 Bq/m2 · s and a standard deviation of 0.087 Bq/m2 · s. The results of these measurements show very high radon exhalation rate and radium content from one particular sample which requires further investigations.