For the sake of improving the agility and super-static performance of spacecraft, this paper puts forward an idea for using single gimbal magnetically suspended control moment gyroscope pyramid configuration to realize dual control of attitude maneuver and micro-vibration suppression of spacecraft, in which gyro gimbal rotation is used to realize fast attitude maneuver and magnetic suspension rotor deflection is used to realize high-precision micro-vibration suppression of spacecraft; the switching design of spacecraft attitude/vibration controller realizes the coordinated operation of gyro gimbal and magnetic suspension motor, showing the control advantage of dual actuators. This strategy not only speeds up the attitude maneuver process of spacecraft, improving the dynamic response, but also reduces the attitude stabilization adjustment time as well as improves the stabilization precision, ensuring the fast vibration suppression after attitude maneuver. In addition, this method has strong robustness ensuring the smooth implementation of spacecraft attitude control and vibration suppression integration in the case of parameter change. The simulation results show the effectiveness and superiority of this strategy.