Effects of local matrix environment on the spectroscopic properties of ensemble to single-particle level carbon dots

2021 ◽  
Author(s):  
Zhihong Wei ◽  
Boyang Wang ◽  
Mingcai Xie ◽  
Daocheng Hong ◽  
Xin Yang ◽  
...  
Keyword(s):  
Single Particle ◽  
Carbon Dots ◽  
Spectroscopic Properties ◽  
Single Particle Level ◽  
Particle Level

Synthesis of single-particle level white-light-emitting carbon dots via a one-step microwave method

2018 ◽  
Vol 6 (25) ◽  
pp. 6691-6697 ◽  
Author(s):  
Kafeel Ahmad ◽  
Ayan Pal ◽  
Uday Narayan Pan ◽  
Arun Chattopadhyay ◽  
Anumita Paul
Keyword(s):  
White Light ◽  
Single Particle ◽  
Microwave Synthesis ◽  
Carbon Dots ◽  
Microwave Method ◽  
Light Emitting ◽  
Single Particle Level ◽  
Particle Level ◽  
One Step

Single-particle level white-light-emitting carbon dots via a one-step microwave synthesis.

Carbon dots with induced surface oxidation permits imaging at single-particle level for intracellular studies

Nanoscale ◽  
2018 ◽  
Vol 10 (39) ◽  
pp. 18510-18519 ◽  
Author(s):  
Santosh K. Misra ◽  
Indrajit Srivastava ◽  
John S. Khamo ◽  
Vishnu V. Krishnamurthy ◽  
Dinabandhu Sar ◽  
...  
Keyword(s):  
Single Particle ◽  
Carbon Dots ◽  
Surface Oxidation ◽  
Single Particle Level ◽  
Particle Level

Separated fractions of carbon dots having induced surface oxidation allows imaging at single-particle level and can be used for intracellular studies.

scholarly journals Role of Single-Particle Energies in Microscopic Interacting Boson Model Double Beta Decay Calculations

Universe ◽  
2021 ◽  
Vol 7 (3) ◽  
pp. 66
Author(s):  
Jenni Kotila
Keyword(s):  
Beta Decay ◽  
Single Particle ◽  
Field Potential ◽  
Double Beta Decay ◽  
Interacting Boson Model ◽  
Model Calculations ◽  
Single Particle Level ◽  
Particle Level ◽  
Boson Model

Single-particle level energies form a significant input in nuclear physics calculations where single-particle degrees of freedom are taken into account, including microscopic interacting boson model investigations. The single-particle energies may be treated as input parameters that are fitted to reach an optimal fit to the data. Alternatively, they can be calculated using a mean field potential, or they can be extracted from available experimental data, as is done in the current study. The role of single-particle level energies in the microscopic interacting boson model calculations is discussed with special emphasis on recent double beta decay calculations.

The influence of diffusion phenomena on catalysis: A study at the single particle level using fluorescence microscopy

2010 ◽  
Vol 157 (1-4) ◽  
pp. 236-242 ◽  
Author(s):  
Gert De Cremer ◽  
Evelyne Bartholomeeusen ◽  
Paolo P. Pescarmona ◽  
Kaifeng Lin ◽  
Dirk E. De Vos ◽  
...  
Keyword(s):  
Fluorescence Microscopy ◽  
Single Particle ◽  
Single Particle Level ◽  
Particle Level ◽  
Diffusion Phenomena

scholarly journals Local Substrate Heterogeneity Influences Electrochemical Activity of TEM Grid-Supported Battery Particles

2021 ◽  
Vol 9 ◽  
Author(s):  
Christina Cashen ◽  
R. Colby Evans ◽  
Zach N. Nilsson ◽  
Justin B. Sambur
Keyword(s):  
Single Particle ◽  
Electrochemical Behavior ◽  
Electrochemical Activity ◽  
Ex Situ ◽  
Structure Property ◽  
Structure Property Relationships ◽  
Single Particle Level ◽  
Particle Level ◽  
Tem Grid ◽  
Ion Insertion

Understanding how particle size and morphology influence ion insertion dynamics is critical for a wide range of electrochemical applications including energy storage and electrochromic smart windows. One strategy to reveal such structure–property relationships is to perform ex situ transmission electron microscopy (TEM) of nanoparticles that have been cycled on TEM grid electrodes. One drawback of this approach is that images of some particles are correlated with the electrochemical response of the entire TEM grid electrode. The lack of one-to-one electrochemical-to-structural information complicates interpretation of genuine structure/property relationships. Developing high-throughput ex situ single particle-level analytical techniques that effectively link electrochemical behavior with structural properties could accelerate the discovery of critical structure-property relationships. Here, using Li-ion insertion in WO3 nanorods as a model system, we demonstrate a correlated optically-detected electrochemistry and TEM technique that measures electrochemical behavior of via many particles simultaneously without having to make electrical contacts to single particles on the TEM grid. This correlated optical-TEM approach can link particle structure with electrochemical behavior at the single particle-level. Our measurements revealed significant electrochemical activity heterogeneity among particles. Single particle activity correlated with distinct local mechanical or electrical properties of the amorphous carbon film of the TEM grid, leading to active and inactive particles. The results are significant for correlated electrochemical/TEM imaging studies that aim to reveal structure-property relationships using single particle-level imaging and ensemble-level electrochemistry.

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