Helium release from the uranium–plutonium mixed oxide (MOX) fuel irradiated to high burn-up in a fast breeder reactor (FBR)

2010 ◽  
Vol 401 (1-3) ◽  
pp. 86-90 ◽  
Author(s):  
Kozo Katsuyama ◽  
Akihiro Ishimi ◽  
Koji Maeda ◽  
Tsuyoshi Nagamine ◽  
Takeo Asaga
2009 ◽  
Vol 1215 ◽  
Author(s):  
Kosuke Tanaka ◽  
Masahiko Osaka ◽  
Ken Kurosaki ◽  
Hiroaki Muta ◽  
Masayoshi Uno ◽  
...  

AbstractThe oxygen potentials at 1273 K of mixed oxide (MOX) fuels with Am and 26 kinds of fission product elements (FPs), simulating low-decontaminated MOX fuel and high burn-up of up to 250 GWd/t, have been measured by using thermogravimetric analysis (TGA). The oxygen potentials for simulated low-decontaminated MOX fuels were higher than the fuels without FPs and increased with increasing simulated burn-up.


2014 ◽  
Vol 2014 ◽  
pp. 1-10 ◽  
Author(s):  
Cheuk Wah Lau ◽  
Henrik Nylén ◽  
Klara Insulander Björk ◽  
Urban Sandberg

Thorium-plutonium mixed oxide (Th-MOX) fuel has become one of the most promising solutions to reduce a large and increasing plutonium stockpile. Compared with traditional uranium-plutonium mixed oxide (U-MOX) fuels, Th-MOX fuel has higher consumption rate of plutonium in LWRs. Besides, thorium based fuels have improved thermomechanical material properties compared with traditional U-MOX fuels. Previous studies on a full Th-MOX core have shown reduced efficiency in reactivity control mechanisms, stronger reactivity feedback, and a significantly lower fraction of delayed neutrons compared with a traditional uranium oxide (UOX) core. These problems complicate the implementation of a full Th-MOX core in a similar way as for a traditional U-MOX core. In order to reduce and avoid some of these issues, the introduction of a lower fraction of Th-MOX fuel in the core is proposed. In this study, one-third of the assemblies are Th-MOX fuel, and the rest are traditional UOX fuel. The feasibility study is based on the Swedish Ringhals-3 PWR. The results show that the core characteristics are more similar to a traditional UOX core, and the fraction of delayed neutrons is within acceptable limits. Moreover, the damping of axial xenon oscillations induced by control rod insertions is almost 5 times more effective for the 1/3 Th-MOX core compared with the standard core.


2020 ◽  
Vol 86 (12) ◽  
pp. 15-22
Author(s):  
N. A. Bulayev ◽  
E. V. Chukhlantseva ◽  
O. V. Starovoytova ◽  
A. A. Tarasenko

The content of uranium and plutonium is the main characteristic of mixed uranium-plutonium oxide fuel, which is strictly controlled and has a very narrow range of the permissible values. We focused on developing a technique for measuring mass fractions of uranium and plutonium by controlled potential coulometry using a coulometric unit UPK-19 in set with a R-40Kh potentiostat-galvanostat. Under conditions of sealed enclosures, a special design of the support stand which minimized the effect of fluctuations in ambient conditions on the signal stability was developed. Optimal conditions for coulometric determination of plutonium and uranium mass fractions were specified. The sulfuric acid solution with a molar concentration of 0.5 mol/dm3 was used as a medium. Lead ions were introduced into the background electrolyte to decrease the minimum voltage of hydrogen reduction to –190 mV. The addition of aluminum nitride reduced the effect of fluoride ions participating as a catalyst in dissolving MOX fuel samples, and the interfering effect of nitrite ions was eliminated by introducing a sulfamic acid solution into the cell. The total content of uranium and plutonium was determined by evaluation of the amount of electricity consumed at the stage of uranium and plutonium co-oxidation. Plutonium content was measured at the potentials, at which uranium remains in the stable state, which makes it possible to subtract the contribution of plutonium oxidation current from the total oxidation current. The error characteristics of the developed measurement technique were evaluated using the standard sample method and the real MOX fuel pellets. The error limits match the requirements set out in the specifications for MOX fuel. The technique for measuring mass fractions of uranium and plutonium in uranium-plutonium oxide nuclear fuel was certified. The relative measurement error of the mass fraction of plutonium and uranium was ±0.0070 and ±0.0095, respectively. The relative error of the ratio of the plutonium mass fraction to the sum of mass fractions of uranium and plutonium was ±0.0085.


2020 ◽  
Vol 148 ◽  
pp. 105588 ◽  
Author(s):  
Jean-Yves Colle ◽  
Sarah Stohr ◽  
Bert Cremer ◽  
Stefaan Van Winckel ◽  
Gert Rasmussen ◽  
...  

1985 ◽  
Vol 22 (2) ◽  
pp. 155-157 ◽  
Author(s):  
Toshimichi TACHIBANA ◽  
Tsuyoshi OHMORI ◽  
Sadamu YAMANOUCHI ◽  
Toshiyuki ITAKI

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