Simulations of Steam Methane Reforming/Sorption-Enhanced Steam Methane Reforming Bubbling Fluidized Bed Reactors by a Dynamic One-Dimensional Two-Fluid Model: Implementation Issues and Model Validation

2013 ◽  
Vol 52 (11) ◽  
pp. 4202-4220 ◽  
Author(s):  
Jannike Solsvik ◽  
Rafael A. Sánchez ◽  
Zhongxi Chao ◽  
Hugo A. Jakobsen
2016 ◽  
Vol 55 (17) ◽  
pp. 5063-5077 ◽  
Author(s):  
Musango Lungu ◽  
Haotong Wang ◽  
Jingdai Wang ◽  
Yongrong Yang ◽  
Fengqiu Chen

Author(s):  
Meltem Dogan ◽  
Dusko Posarac ◽  
John Grace ◽  
Alaa-Eldin M. Adris ◽  
C. Jim Lim

Fluidized bed reactors for steam methane reforming, with and without immersed membrane surfaces for withdrawal of hydrogen, are modeled with oxygen added in order to provide the endothermic heat required by the reforming reactions. Porous alumina, palladium and palladium-coated high-flux tubes are investigated as separation materials, the latter two being permselective. Hydrogen yield and permeate hydrogen molar flow are predicted to decrease with increasing oxygen flow, and to increase with temperature. When the steam-to-carbon ratio increases, permeate hydrogen yield decreases slightly, while the total hydrogen yield increases for all configurations. The flow of oxygen required to achieve autothermal conditions depends on such factors as the reactor temperature, steam-to-carbon ratio and preheating of the feed.


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