scholarly journals Cooperative enhancement versus additivity of two-photon-absorption cross sections in linear and branched squaraine superchromophores

2016 ◽  
Vol 18 (24) ◽  
pp. 16404-16413 ◽  
Author(s):  
Harald Ceymann ◽  
Arnulf Rosspeintner ◽  
Maximilian H. Schreck ◽  
Carina Mützel ◽  
Andreas Stoy ◽  
...  

Our investigation of the nonlinear optical properties of a series of oligomeric squaraine dyes showed enhanced cross sections for linear oligomers but only additivity for branched systems.

2008 ◽  
Vol 17 (03) ◽  
pp. 275-283 ◽  
Author(s):  
YING HU ◽  
EVGENY O. DANILOV ◽  
BRIGITTE WEX ◽  
DOUGLAS C. NECKERS

The nonlinear optical properties of heterocyclic compounds (1-7) were investigated. π-Centers benzo[1,2-b:4,3-b']dithiophene (1) and trithia[5]helicene (5) were studied. Compounds 2-4, 6 and 7 possess either donor-π (D-π) or donor-π-acceptor (D-π-A) structures. The optimized geometry of 7 shows a 3D helical structure. Two-photon absorption cross-sections related to the third-order nonlinear susceptibility were measured using open-aperture Z-scan techniques. Compound 7 has a two-photon absorption cross-section of 103 GM when excited at 720 nm. Important molecular structure-nonlinear optical property relationships are formulated.


2002 ◽  
Vol 209 (4-6) ◽  
pp. 461-466 ◽  
Author(s):  
I. Fuks-Janczarek ◽  
J-M. Nunzi ◽  
B. Sahraoui ◽  
I.V. Kityk ◽  
J. Berdowski ◽  
...  

2001 ◽  
Vol 190 (1-6) ◽  
pp. 345-349 ◽  
Author(s):  
Guangyong Zhou ◽  
Xiaomei Wang ◽  
Dong Wang ◽  
Chun Wang ◽  
Zongshu Shao ◽  
...  

2008 ◽  
Vol 108 (5) ◽  
pp. 3218-3224 ◽  
Author(s):  
Seetharam Shettigar ◽  
G. Umesh ◽  
K. Chandrasekharan ◽  
Ganesh Rai ◽  
B. Kalluraya

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