A green route to a novel hyperbranched electrolyte interlayer for nonfullerene polymer solar cells with over 11% efficiency

2018 ◽  
Vol 54 (5) ◽  
pp. 563-566 ◽  
Author(s):  
Dan Zhou ◽  
Sixing Xiong ◽  
Lie Chen ◽  
Xiaofang Cheng ◽  
Haitao Xu ◽  
...  

A PNSO3Na organic interfacial layer can induce the active layer to form a bi-continuous nano-micro phase separation face-on orientation.

2020 ◽  
Vol 8 (16) ◽  
pp. 5613-5619 ◽  
Author(s):  
Lu Zhang ◽  
Zicheng Ding ◽  
Ruyan Zhao ◽  
Feng Jirui ◽  
Wei Ma ◽  
...  

The aggregation tendency in solution of polymer donors is the dominant factor in the phase separation of semi-crystalline polymer donor/amorphous polymer acceptor blends in all-PSCs.


2021 ◽  
Vol 3 (4) ◽  
pp. 1923-1931
Author(s):  
Dong Chen ◽  
Siqi Liu ◽  
Jinliang Liu ◽  
Jihui Han ◽  
Lie Chen ◽  
...  

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Zahra Arefinia ◽  
Dip Prakash Samajdar

AbstractNumerical-based simulations of plasmonic polymer solar cells (PSCs) incorporating a disordered array of non-uniform sized plasmonic nanoparticles (NPs) impose a prohibitively long-time and complex computational demand. To surmount this limitation, we present a novel semi-analytical modeling, which dramatically reduces computational time and resource consumption and yet is acceptably accurate. For this purpose, the optical modeling of active layer-incorporated plasmonic metal NPs, which is described by a homogenization theory based on a modified Maxwell–Garnett-Mie theory, is inputted in the electrical modeling based on the coupled equations of Poisson, continuity, and drift–diffusion. Besides, our modeling considers the effects of absorption in the non-active layers, interference induced by electrodes, and scattered light escaping from the PSC. The modeling results satisfactorily reproduce a series of experimental data for photovoltaic parameters of plasmonic PSCs, demonstrating the validity of our modeling approach. According to this, we implement the semi-analytical modeling to propose a new high-efficiency plasmonic PSC based on the PM6:Y6 PSC, having the highest reported power conversion efficiency (PCE) to date. The results show that the incorporation of plasmonic NPs into PM6:Y6 active layer leads to the PCE over 18%.


2021 ◽  
Vol 113 ◽  
pp. 110909 ◽  
Author(s):  
Can Chen ◽  
Chunlin Zhang ◽  
Yichun Peng ◽  
Ningning Wang ◽  
Xingpeng Liu ◽  
...  

2010 ◽  
Vol 11 (4) ◽  
pp. 599-603 ◽  
Author(s):  
Dong Hwan Wang ◽  
Dae Geun Choi ◽  
Ki-Joong Lee ◽  
O. Ok Park ◽  
Jong Hyeok Park

2021 ◽  
Author(s):  
Yanming Sun ◽  
Yunhao Cai ◽  
Qian Li ◽  
Guanyu Lu ◽  
Hwa Sook Ryu ◽  
...  

Abstract The development of high-performance organic solar cells (OSCs) with thick active layers is of crucial importance for the roll-to-roll printing of large-area solar panels. Unfortunately, increasing the active layer thickness usually results in a significant reduction in efficiency. Herein, we fabricated efficient thick-film OSCs with an active layer consisting of one polymer donor and two non-fullerene acceptors. The two acceptors were found to possess enlarged exciton diffusion length in the mixed phase, which is beneficial to exciton generation and dissociation. Additionally, layer by layer approach was employed to optimize the vertical phase separation. Benefiting from the synergetic effects of enlarged exciton diffusion length and graded vertical phase separation, a record high efficiency of 17.31% (certified value of 16.9%) was obtained for the 300 nm-thick OSC, with an unprecedented short-circuit current density of 28.36 mA cm−2, and a high fill factor of 73.0%. Moreover, the device with an active layer thickness of 500 nm also shows a record efficiency of 15.21%. This work provides new insights into the fabrication of high-efficiency OSCs with thick active layers.


RSC Advances ◽  
2017 ◽  
Vol 7 (50) ◽  
pp. 31158-31163 ◽  
Author(s):  
Mingguang Li ◽  
Wen Zhang ◽  
Honglei Wang ◽  
Lingfeng Chen ◽  
Chao Zheng ◽  
...  

Simultaneously enhanced efficiency and stability can be achieved by using an organic cathode interfacial layer with high mobility and coarse morphology.


2008 ◽  
Vol 92 (10) ◽  
pp. 103306 ◽  
Author(s):  
Chih-Wei Chu ◽  
Hoichang Yang ◽  
Wei-Jen Hou ◽  
Jinsong Huang ◽  
Gang Li ◽  
...  

2018 ◽  
Vol 62 (1) ◽  
pp. 67-73 ◽  
Author(s):  
Sheng Dong ◽  
Kai Zhang ◽  
Xiang Liu ◽  
Qingwu Yin ◽  
Hin-Lap Yip ◽  
...  

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