scholarly journals Influence of size polydispersity on magnetic field tunable structures in magnetic nanofluids containing superparamagnetic nanoparticles.

2021 ◽  
Author(s):  
Dillip Kumar Mohapatra ◽  
Philip James Camp ◽  
John Philip
Keyword(s):  
Magnetic Field ◽  
Particle Size ◽  
Light Scattering ◽  
Optical Microscopy ◽  
Brownian Dynamics ◽  
Phase Contrast ◽  
Superparamagnetic Nanoparticles ◽  
Magnetic Nanofluids ◽  
Dynamics Simulations ◽  
Brownian Dynamics Simulations

We probe the influence of particle size polydispersity on field-induced structures and structural transitions in magnetic fluids (ferrofluids) using phase contrast optical microscopy, light scattering and Brownian dynamics simulations. Three...

scholarly journals Structure evolution of suspensions under time-dependent electric or magnetic field

2021 ◽  
Author(s):  
Konstantinos Manikas ◽  
Markus Hütter ◽  
Patrick D. Anderson
Keyword(s):  
Magnetic Field ◽  
Field Strength ◽  
Brownian Dynamics ◽  
Thermal Fluctuations ◽  
Time Dependent ◽  
Structure Evolution ◽  
Strength Increase ◽  
Large Rotation ◽  
Dynamics Simulations ◽  
Brownian Dynamics Simulations

AbstractThe effect of time-dependent external fields on the structures formed by particles with induced dipoles dispersed in a viscous fluid is investigated by means of Brownian Dynamics simulations. The physical effects accounted for are thermal fluctuations, dipole-dipole and excluded volume interactions. The emerging structures are characterised in terms of particle clusters (orientation, size, anisotropy and percolation) and network structure. The strength of the external field is increased in one direction and then kept constant for a certain amount of time, with the structure formation being influenced by the slope of the field-strength increase. This effect can be partially rationalized by inhomogeneous time re-scaling with respect to the field strength, however, the presence of thermal fluctuations makes the scaling at low field strength inappropriate. After the re-scaling, one can observe that the lower the slope of the field increase, the more network-like and the thicker the structure is. In the second part of the study the field is also rotated instantaneously by a certain angle, and the effect of this transition on the structure is studied. For small rotation angles ($$\theta \le 20^{{\circ }}$$ θ ≤ 20 ∘ ) the clusters rotate but stay largely intact, while for large rotation angles ($$\theta \ge 80^{{\circ }}$$ θ ≥ 80 ∘ ) the structure disintegrates and then reforms, due to the nature of the interactions (parallel dipoles with perpendicular inter-particle vector repel each other). For intermediate angles ($$20<\theta <80^{{\circ }}$$ 20 < θ < 80 ∘ ), it seems that, during rotation, the structure is altered towards a more network-like state, as a result of cluster fusion (larger clusters). The details provided in this paper concern an electric field, however, all results can be projected into the case of a magnetic field and paramagnetic particles.

Brownian Dynamics Simulations of Aggregation Phenomena in a Magnetic Particle Suspension With an Alternating Magnetic Field (Relationship Between the Aggregate Structure and the Heat Production)

2018 ◽  
Author(s):  
Seiya Suzuki ◽  
Akira Satoh ◽  
Muneo Futamura
Keyword(s):  
Magnetic Field ◽  
Heat Production ◽  
Brownian Dynamics ◽  
Magnetic Particle ◽  
Particle Interaction ◽  
Alternating Magnetic Field ◽  
Dynamics Simulations ◽  
Brownian Dynamics Simulations ◽  
The Magnetic Field ◽  
Aggregation Phenomena

The present study addresses physical phenomena of a suspension composed of magnetic spherical particles in an alternating magnetic field in order to elucidate particle aggregation phenomena and their influence on heat production. For this objective, we have performed Brownian dynamics simulations in a variety of circumstances of the magnetic field strength and frequency of an alternating magnetic field, and the magnetic dipole-dipole interaction strength. As in a time-independent uniform external magnetic field, large aggregates are formed in the case of strong magnetic particle-particle interactions. However, these clusters exhibit completely different behaviors that are dependent on the frequency of an alternating magnetic field. If the frequency is significantly high, then the viscous torque is the dominant factor, so that the formation of the clusters is not significantly influenced by the time-dependent magnetic field. If the frequency is significantly low, the magnetic field have a significant effect on the rotational motion of the particles, so that the formation of the cluster is dependent on which factor dominates the particle motion between the applied magnetic field and the magnetic particle-particle interaction. If the magnetic interaction is more dominant than the external field, stable chain-like clusters are formed in the field direction, and the magnetic particle-particle interaction induces a significant delay for the moments inclining in the alternating magnetic field direction. This behavior gives rise to a hysteresis loop with a larger area and therefore a large heating effect is obtained.

Brownian Dynamics Simulations of Colloidal Dispersion Composed of Ferromagnetic Spherocylinder Particles in a Simple Shear Flow (For the Case of an Applied Magnetic Field Normal to the Shear Plane)

2009 ◽  
Author(s):  
Ryo Hayasaka ◽  
Yasuhiro Sakuda ◽  
Akira Satoh
Keyword(s):  
Magnetic Field ◽  
Brownian Dynamics ◽  
Magnetic Particle ◽  
Colloidal Dispersion ◽  
Magnetic Interactions ◽  
Simple Shear Flow ◽  
Particle Interactions ◽  
Dynamics Simulations ◽  
Brownian Dynamics Simulations ◽  
The Magnetic Field

We have investigated aggregate structures and rheological properties of a colloidal dispersion composed of ferromagnetic spherocylinder particles with a magnetic moment along the particle axis direction, by means of Brownian dynamics simulations. In concrete, we have attempted to clarify the influences of the flow field, magnetic field strength, magnetic interactions between particles and volumetric fraction of particles. In order to discuss quantitatively the internal structures of clusters, we have concentrated our attention on the radial distribution and orientational distribution functions. The present results are compared with those of the theoretical analysis for dilute dispersions and also non-dilute dispersions; the results for the latter were obtained by means of the mean-field approximation, which magnetic particle-particle interactions can be taken into account. Some important results are summarized as follows. For the case of the magnetic field strength and magnetic interactions between particles are more dominant than the viscous forces due to a simple shear flow, chain-like like clusters are formed along the magnetic field direction, although they are slightly tilted to the flow direction. When magnetic particle-particle interactions become over a certain value, such cluster formation leads to a significant increase in the viscosity of the dispersion.

Sign in / Sign up

Export Citation Format

Share Document