A Universal Thermally Activated Delayed Fluorescence Host with Short Triplet Lifetime for Highly Efficient Phosphorescent OLEDs with Extremely Low Efficiency Roll-off

Author(s):  
Jian Fan ◽  
Bangjin Sun ◽  
Kaining Tong ◽  
Xing Chen ◽  
Jian-Li He ◽  
...  

Triplet-involved quenching processes lead to significant efficiency roll-off in phosphorescent organic light-emitting diodes (OLEDs). Thermally activated delayed fluorescence (TADF) materials can reduce the triplet exciton density in the emitting layer...

Author(s):  
Yaxing Zhang ◽  
Yuanyuan Zheng ◽  
Changsheng Shi ◽  
Jinyan Zhang ◽  
Tao Wang ◽  
...  

The progress of orange-red thermally activated delayed fluorescence (TADF) emitters for solution-processed organic light-emitting diodes (OLEDs) is still lagged behind blue and green materials in terms of device efficiency. In...


2019 ◽  
Vol 7 (16) ◽  
pp. 4673-4680 ◽  
Author(s):  
Cheng Chen ◽  
Hai-Yan Lu ◽  
Yin-Feng Wang ◽  
Meng Li ◽  
Yi-Fan Shen ◽  
...  

1,8-Naphthyridine-based TADF molecules were utilized as a new kind of emitter for multi-color OLEDs with low efficiency roll-off.


2017 ◽  
Vol 8 (2) ◽  
pp. 1259-1268 ◽  
Author(s):  
Kunping Guo ◽  
Hedan Wang ◽  
Zixing Wang ◽  
Changfeng Si ◽  
Cuiyun Peng ◽  
...  

A bipolar host with TADF properties is realized, endowing green PhOLEDs with a twentyfold lifetime improvement.


2019 ◽  
Vol 7 (26) ◽  
pp. 8063-8069 ◽  
Author(s):  
Xiang-Long Li ◽  
Xinyi Cai ◽  
Muhammad Umair Ali ◽  
Shi-Jian Su ◽  
Hong Meng

Highly efficient TADF yellow OLEDs with an extremely low efficiency roll-off have been obtained herein via rational device engineering.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
A. Lennart Schleper ◽  
Kenichi Goushi ◽  
Christoph Bannwarth ◽  
Bastian Haehnle ◽  
Philipp J. Welscher ◽  
...  

AbstractFast emission and high color purity are essential characteristics of modern opto-electronic devices, such as organic light emitting diodes (OLEDs). These properties are currently not met by the latest generation of thermally activated delayed fluorescence (TADF) emitters. Here, we present an approach, called “hot exciplexes” that enables access to both attributes at the same time. Hot exciplexes are produced by coupling facing donor and acceptor moieties to an anthracene bridge, yielding an exciplex with large T1 to T2 spacing. The hot exciplex model is investigated using optical spectroscopy and quantum chemical simulations. Reverse intersystem crossing is found to occur preferentially from the T3 to the S1 state within only a few nanoseconds. Application and practicality of the model are shown by fabrication of organic light-emitting diodes with up to 32 % hot exciplex contribution and low efficiency roll-off.


Author(s):  
Won Jae Chung ◽  
Jun Yeob Lee

In the organic light emitting diodes (OLEDs), the achievement of high efficiency and long device lifetime has been a goal due to the short device lifetime of the high efficiency...


2017 ◽  
Vol 5 (38) ◽  
pp. 10001-10006 ◽  
Author(s):  
Xiaoqing Liao ◽  
Xin Yang ◽  
Rong Zhang ◽  
Jiang Cheng ◽  
Jie Li ◽  
...  

Solution-processed white OLEDs based on a blue TADF dendrimer host and an orange iridium complex dopant achieved a maximum EQE of 10.1% with low efficiency roll-off at high current density.


2018 ◽  
Vol 6 (35) ◽  
pp. 9510-9516 ◽  
Author(s):  
Chenyang Zhao ◽  
Tianmu Zhang ◽  
Jiangshan Chen ◽  
Donghang Yan ◽  
Dongge Ma

Highly efficient and low efficiency roll-off WOLEDs by simple insertion of multi-ultrathin phosphorescent layers within blue TADF emitters.


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