scholarly journals The remote-controlled spectrometric system for searching and characterization of high-level radioactive waste

2020 ◽  
Vol 225 ◽  
pp. 06002
Author(s):  
Alexey Danilovich ◽  
Victor Potapov ◽  
Sergey Smirnov

In 2003, the work on environmental rehabilitation of the former coastal technical base of the Russian Navy in Gremikha town, with technical and financial support of the State Atomic Energy Corporation “Rosatom” and the French Alternative Energies and Atomic Energy Commission had begun. In 2017, the task of searching, characterization and packaging in transport containers for export to the long-term storage of high-level waste containing 152Eu was set as part of this program. These wastes were presented as fragments of reactor control and safety system rods of first generation nuclear submarine reactors and were placed in temporary storage containers mixed with other radioactive waste and construction garbage on the territory of the Gremikha branch of the North-West Center “SevRAO”. To accomplish the task, the spectrometric system “Gamma-Pioneer” was developed and made at National Research Center “Kurchatov Institute”. The system consist of a collimated spectrometric gamma-ray CdZnTe detector 500 mm3 volume, a dosimeter for continuous measurement of ambient equivalent dose rate at the instrument location and a color video camera with zoom lens. The device is placed in a protective frame and installed as an attachment implements on robot Brokk-90. Communication between the measuring system and the control computer is carried out using USB extender and 100 meters cable. The video camera is connected to the control computer via Ethernet. To search for the most active sources of gamma radiation, an equivalent dose rate calculation program using the results of measured instrumental spectra was developed. The characterization of the extracted fragments was carried out by activity evaluation of the main radionuclides polluting the samples under investigation. The paper describes design and operating principles of the system, as well as methods for the equivalent dose rate calculation and the activity evaluation of the fragments of reactor control and safety system rods based on spectral measurements obtained using the developed radiometric system

Author(s):  
J. A. Mason ◽  
W. Hage ◽  
R. Price ◽  
A. C. Tolchard ◽  
A. C. N. Towner

The paper describes an automated non-destructive assay (NDA) system for the measurement and characterization of radioactive waste. The Waste Characterisation System (WCS) can be adapted to measure a variety of drum sizes: 60, 220 (55 gallon) and 440 liter, the latter with a maximum weight of 1500 kg (1.5 tonnes). The NDA system includes a Tomographic Segmented Gamma Scanner (TSGS) and an active/passive neutron Differential Die-away (DDA or DDT). The system can assay a wide variety of waste types in a range of waste matrices. The assay stations are linked by a heavy duty roller conveyor which incorporates a 20 drum buffer store, a load cell (built into the conveyor), bar code readers and a dose rate measurement station. The Tomographic Segmented Gamma Scanner (TSGS) combines conventional high resolution gamma spectrometry and a tranission source to interrogate a waste drum in vertical slices (segments) as for Segmented Gamma Scanner (SGS) measurements. However, in the case of the TSGS, while the drum is rotated, it is also moved in the horizontal direction leading to an enhanced ability to correct the gamma ray energies, from the nuclides of interest, for the attenuation of the matrix. The TSGS can also be operated as a conventional SGS for the measurement of homogeneous waste drums. The DDA is a very sensitive active neutron interrogation method that uses thermalised neutrons from a pulsed source within the chamber to irradiate a waste drum. Prompt neutrons from fissile material present in the waste (e. g. 239Pu, 235U) are detected and provide a measure of the fissile content in the drum. In passive mode, the DDA determines the even Pu nuclides exhibiting significant spontaneous fission (e.g. 240Pu). Measurement accuracy depends on correction algorithms to compensate for self-shielding and matrix effects in waste drums containing hydrogenous materials. In addition, the DDA will be provided with the Fission-Fission Neutron Correlation Analysis System (FFnC) which is an absolute technique eliminating the need for matrix dependent mass calibrations, and allowing separate U and Pu determination using delayed neutron counting. The FFnC technique will be tested for the first time on the WCS. The NDA system incorporates integrated stations to determine the weight and dose rate of each drum, the former built into the conveyor the latter as part of the TSGS. Six Geiger Muller tubes measure the surface dose at three positions on the drum side, one at 1 metre from the drum and one each measuring the surface dose of the top and bottom of the drum. The assay instruments are linked to a heavy duty conveyor system onto which up to 20 waste drums can be loaded for delivery to the various measurement stations, thus permitting unattended, automated operation. Once measured, the drums remain on the conveyer in a holding system waiting to be unloaded. Automation is provided using a programmable logic controller (PLC) and associated computers. A central computer and associated software is used for data acquisition and management.


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