Interaction of excitons with Cherenkov radiation in WSe2 beyond the non-recoil approximation
Abstract Cherenkov radiation from electrons propagating in materials with a high refractive index have applications in particle-detection mechanisms and could be used for high-yield coherent electron beam-driven photon sources. However, the theory of the Cherenkov radiation has been treated up to now using the non-recoil approximation, which neglects the effect of electron deceleration in materials. Here, we report on the effect of electron-beam deceleration on the radiated spectrum and exciton-photon interactions in nm-thick 〖WSe〗_2 crystals. The calculation of the Cherenkov radiation is performed by simulating the kinetic energy of an electron propagating in a thick sample using the Monto Carlo method combined with the Lienard-Wiechert retarded potential. Using this approach, we numerically investigate the interaction between the excitons and generated photons (Cherenkov radiation) beyond the non-recoil approximation and are able to reproduce experimental cathodoluminescence spectra. Our findings pave the way for an accurate design of particle scintillators and detectors, based on the strong-coupling phenomenon.