Assessment of influence of urban aerosol vertical profile on clear-sky diffuse radiance pattern

2021 ◽  
pp. 1-7
Author(s):  
Jaromir Petrzala

Abstract Aerosol particles spread in the atmosphere play an important role in solar light scattering and thus co-determine the sky radiance/luminance pattern as well as diffuse irradiances/illuminances at the ground. The particular influence is given by their optical properties and by their distribution in the atmosphere. The dependence of the aerosol extinction coefficient on altitude is usually described by the exponential law, which results from averaging of a large amount of aerosol realizations. This is also frequently the case of simulating of the solar diffuse radiance/luminance distribution over the sky, when it is based on solving the radiative transfer problem. However, the aerosol vertical profile can sometimes be significantly different from the exponential one. Mainly in the urban environment, the aerosol is often well-mixed within the atmospheric boundary layer, so its volume extinction coefficient is almost constant there. This work investigates how such different profiles affect the clear sky radiance pattern and consequently also the ground-based horizontal diffuse irradiance. The numerical simulations reveal that the discrepancies are negligible in practice. So it appears that the aerosol vertical distribution does not play any important role in sky radiance calculations and the standard exponential law is general enough to cover also various specific aerosol conditions.

2007 ◽  
Vol 7 (4) ◽  
pp. 9769-9793 ◽  
Author(s):  
H. Irie ◽  
Y. Kanaya ◽  
H. Akimoto ◽  
H. Iwabuchi ◽  
A. Shimizu ◽  
...  

Abstract. Ground-based Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements were performed at Tsukuba, Japan (36.1° N, 140.1° E), in November–December 2006. The measured spectra of scattered sunlight are analyzed by DOAS and optimal estimation methods to retrieve the aerosol optical depth (τ) and the vertical profile of the aerosol extinction coefficient (σ) at 476 nm in the lower troposphere. We characterize these retrieved quantities through comparisons with coincident lidar and sky radiometer measurements. The retrieved σ values for layers of 0–1 and 1–2 km agree with lidar data to within 30% and 60%, respectively, for most cases, including partly cloudy conditions. Results similar to σ at 0–1 km are obtained for the retrieved τ values, demonstrating that MAX-DOAS provides the new, unique aerosol dataset in the lower troposphere.


2020 ◽  
Author(s):  
Larry W. Thomason ◽  
Mahesh Kovilakam ◽  
Anja Schmidt ◽  
Christian von Savigny ◽  
Travis Knepp ◽  
...  

Abstract. An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption's main aerosol layer and an apparent change in aerosol size distribution that spans multiple orders of magnitude in the stratospheric impact of a volcanic event. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main aerosol layer may significantly modulate these results. Despite this limitation, these findings represent a unique opportunity to verify the performance of interactive aerosol models used in Global Climate Models and Earth System Model and may suggest an avenue for improving aerosol extinction coefficient measurements from single channel observations such the Optical Spectrograph and Infrared Imager System as they rely on a priori assumptions about particle size.


2009 ◽  
Vol 9 (5) ◽  
pp. 22177-22222
Author(s):  
L. W. Thomason ◽  
J. R. Moore ◽  
M. C. Pitts ◽  
J. M. Zawodny ◽  
E.-W. Chiou

Abstract. Herein, we provide an assessment of the data quality of Stratospheric Aerosol and Gas Experiment (SAGE III) Version 4 aerosol extinction coefficient and water vapor data products. The evaluation is based on comparisons with data from four instruments: SAGE II, the Polar Ozone and Aerosol Measurement (POAM III), the Halogen Occultation Experiment (HALOE), and the Microwave Limb Sounder (MLS). Since only about half of the SAGE III channels have a direct comparison with measurements by other instruments, we have employed some empirical techniques to evaluate measurements at some wavelengths. We find that the aerosol extinction coefficient measurements at 449, 520, 755, 869, and 1021 nm are reliable with accuracies and precisions on the order of 10% in the primary aerosol range of 15 to 25 km. We also believe this to be true of the aerosol measurements at 1545 nm though we cannot exclude some positive bias below 15 km. We recommend use of the 385 nm measurements above 16 km where the accuracy is on par with other aerosol channels. The 601 nm measurement is much noisier (~20%) than other channels and we suggest caution in the use of these data. We believe that the 676 nm data are clearly defective particularly above 20 km (accuracy as poor as 50%) and the precision is also low (~30%). We suggest excluding this channel under most circumstances. The SAGE III Version 4 water vapor data product appears to be high quality and is recommended for science applications in the stratosphere below 45 km. In this altitude range, the mean differences with all four corroborative data sets are no bigger than 15% and often less than 10% with exceptional agreement with POAM III and MLS. Above 45 km, it seems likely that SAGE III water vapor values are increasingly too large and should be used cautiously or avoided. We believe that SAGE III meets its preflight goal of 15% accuracy and 10% precision between 15 and 45 km. We do not currently recommend limiting the SAGE III water vapor data utility in the stratosphere by aerosol loading.


Author(s):  
H. L. Zhang ◽  
H. Zhao ◽  
Y. P. Liu ◽  
X. K. Wang ◽  
C. Shu

Abstract. For a long time, the research of the optical properties of atmospheric aerosols has aroused a wide concern in the field of atmospheric and environmental. Many scholars commonly use the Klett method to invert the lidar return signal of Mie scattering. However, there are always some negative values in the detection data of lidar, which have no actual meaning,and which are jump points. The jump points are also called wild value points and abnormal points. The jump points are refered to the detecting points that are significantly different from the surrounding detection points, and which are not consistent with the actual situation. As a result, when the far end point is selected as the boundary value, the inversion error is too large to successfully invert the extinction coefficient profile. These negative points are jump points, which must be removed in the inversion process. In order to solve the problem, a method of processing jump points of detection data of lidar and the inversion method of aerosol extinction coefficient is proposed in this paper. In this method, when there are few jump points, the linear interpolation method is used to process the jump points. When the number of continuous jump points is large, the function fitting method is used to process the jump points. The feasibility and reliability of this method are verified by using actual lidar data. The results show that the extinction coefficient profile can be successfully inverted when different remote boundary values are chosen. The extinction coefficient profile inverted by this method is more continuous and smoother. The effective detection range of lidar is greatly increased using this method. The extinction coefficient profile is more realistic. The extinction coefficient profile inverted by this method is more favorable to further analysis of the properties of atmospheric aerosol. Therefore, this method has great practical application and popularization value.


2021 ◽  
Vol 21 (2) ◽  
pp. 1143-1158 ◽  
Author(s):  
Larry W. Thomason ◽  
Mahesh Kovilakam ◽  
Anja Schmidt ◽  
Christian von Savigny ◽  
Travis Knepp ◽  
...  

Abstract. An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption's main aerosol layer and the wavelength dependence of that perturbation. This relationship spans multiple orders of magnitude in the aerosol extinction coefficient of stratospheric impact of volcanic events. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main sulfuric acid aerosol layer and other factors may significantly modulate these results. Despite these limitations, the findings suggest an avenue for improving aerosol extinction coefficient measurements from single-channel observations such as the Optical Spectrograph and Infrared Imager System as they rely on a prior assumptions about particle size. They may also represent a distinct avenue for the comparison of observations with interactive aerosol models used in global climate models and Earth system models.


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