Z-scan study of nonlinear optical standards and D-A fluorophores considering fifth-order optical nonlinearities

2018 ◽  
Vol 8 (03) ◽  
pp. 1 ◽  
Author(s):  
Yilin Zhang ◽  
Meijuan Jiang ◽  
Jie Li ◽  
Bin Hu ◽  
Ben Zhong Tang
Keyword(s):  
Nonlinear Optical ◽  
Optical Nonlinearities ◽  
Fifth Order

Few-Particle Effects in Nonlinear Optical Spectra of Semiconductor Quantum Dots

1999 ◽  
Vol 571 ◽  
Author(s):  
Ulrich Hohenesteri ◽  
Fausto Rossi ◽  
Elisa Molinari
Keyword(s):  
Quantum Dots ◽  
Density Matrix ◽  
Nonlinear Optical ◽  
Coherent Control ◽  
Optical Spectra ◽  
Carrier Dynamics ◽  
Semiconductor Quantum Dots ◽  
Nonequilibrium Carrier ◽  
Optical Nonlinearities ◽  
Matrix Approach

ABSTRACTWe present a density-matrix approach for the description of nonequilibrium carrier dynamics in optically excited semiconductor quantum dots, that explicitly accounts for exciton-exciton as well as exciton-carrier interactions. Within this framework, we analyze few-particle effects in the optical spectra and provide a consistent description of additional peaks appearing at high photoexcitation density. We discuss possible applications of such optical nonlinearities in future coherent-control experiments.

scholarly journals Electronic properties and third-order optical nonlinearities in tetragonal chalcopyrite AgInS2, AgInS2/ZnS and cubic spinel AgIn5S8, AgIn5S8/ZnS quantum dots

2017 ◽  
Vol 5 (1) ◽  
pp. 149-158 ◽  
Author(s):  
Bartłomiej Cichy ◽  
Dominika Wawrzynczyk ◽  
Marek Samoc ◽  
Wiesław Stręk
Keyword(s):  
Quantum Dots ◽  
Optical Properties ◽  
Electronic Properties ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Optical Nonlinearities ◽  
Third Order

Electronic as well as third-order nonlinear optical properties of chalcopyrite AgInS2 and non-stoichiometric spinel AgIn5S8 quantum dots compared with corresponding Zn2+ alloyed compounds are presented in this work.

Theoretical and Experimental Studies of Third-Order Nonlinear Optical Susceptibilities of New p-N,N'-Diamethylaniline Tetrathiafulvalene Derivatives

2000 ◽  
Vol 660 ◽  
Author(s):  
B. Sahraoui ◽  
K.J. Pluciński ◽  
M. Makowaska-Janusik ◽  
I. V. Kityk ◽  
M. Salle ◽  
...  
Keyword(s):  
Quantum Chemical Calculations ◽  
Quantum Chemical ◽  
Nonlinear Optical ◽  
Experimental Studies ◽  
Physical Nature ◽  
Four Wave Mixing ◽  
Wave Mixing ◽  
Electronic Contribution ◽  
Optical Nonlinearities ◽  
Third Order

ABSTRACTA study was made of third-order nonlinear optical susceptibilities of new tetrathiafulvalene (TTF) derivatives, using the degenerate four wave mixing (DFWM) method, as well as complex quantum chemical calculations. To understand the physical nature of the optical nonlinearities, we separated their electronic and nuclear contributions. We found that the electronic contribution to these nonlinearities predominated. Our investigations suggest that TTF may be a highly promising material for nonlinear optics (NLO).

Third- and Fifth-Order Nonlinear Optical Response of a TICT/Stilbene Hybrid Chromophore

2020 ◽  
Vol 124 (9) ◽  
pp. 5363-5370 ◽  
Author(s):  
Alexander J.-T. Lou ◽  
Sepehr Benis ◽  
Munan Gao ◽  
Alexander Baev ◽  
David Kim ◽  
...  
Keyword(s):  
Nonlinear Optical ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Fifth Order

scholarly journals Interaction of Pulses of Different Duration with Chemically Prepared Silver Nanoparticles: Analysis of Optical Nonlinearities

2019 ◽  
Vol 2019 ◽  
pp. 1-12 ◽  
Author(s):  
Ke Zhang ◽  
Rashid A. Ganeev ◽  
Konda Srinivasa Rao ◽  
Sandeep Kumar Maurya ◽  
Ganjaboy S. Boltaev ◽  
...  
Keyword(s):  
Silver Nanoparticles ◽  
Nonlinear Absorption ◽  
Nonlinear Optical ◽  
Reduction Method ◽  
Chemical Reduction ◽  
Nonlinear Refraction ◽  
Optical Nonlinearities ◽  
Chemical Reduction Method ◽  
Ag Nps ◽  
Picosecond Pulses

The nonlinear optical properties of the aqueous solutions of silver nanoparticles (Ag NPs) prepared by chemical reduction method are analyzed using femtosecond and picosecond pulses at different wavelengths. In the case of 800 and 400 nm, the growths of nonlinear absorption and nonlinear refraction with the increase of Ag NP concentration, as well as a change at the signs of nonlinear optical processes, are determined. The nonlinear absorption coefficient and nonlinear refractive index of Ag NP solutions measured using picosecond pulses were a few orders of magnitude larger than those in the case of femtosecond probe pulses. We also demonstrate the optical limiting properties of Ag NPs using 800 nm, 60 fs pulses.

Third- and Fifth-Order Optical Properties of Transition Metal Complexes of Benzenedithiol at 1.064 μm

1992 ◽  
Vol 247 ◽  
Author(s):  
J. R. Lindle ◽  
C. S. Weisbecker ◽  
F. J. Bartoli ◽  
R. G. S. Pong ◽  
Z. H. Kafafi
Keyword(s):  
Optical Properties ◽  
Transition Metal ◽  
Metal Complexes ◽  
Transition Metal Complexes ◽  
Nd:Yag Laser ◽  
Nonlinear Optical ◽  
Four Wave Mixing ◽  
Wave Mixing ◽  
Time Resolved ◽  
Fifth Order

ABSTRACTTime-resolved degenerate four-wave-mixing studies have been conducted on solutions of transition-metal complexes of benzenedithiol using a 35 ps Nd:YAG laser operating at 1.064 μm. The nonlinear optical properties of the first-row Co(d7), Ni(d8), and Cu(d9) and the d8 group Ni and P t transition metal complexes are discussed.

NONLINEAR RESPONSE INDUCED STRONG ABSORPTANCE OF GRAPHENE IN THE TERAHERTZ REGIME

2010 ◽  
Vol 24 (21) ◽  
pp. 2243-2249 ◽  
Author(s):  
X. G. XU ◽  
J. C. CAO
Keyword(s):  
Nonlinear Optical ◽  
Low Frequency ◽  
Single Layer ◽  
Optical Response ◽  
Optoelectronic Device ◽  
Nonlinear Optical Response ◽  
Single Layer Graphene ◽  
Dirac Fermions ◽  
Layer Graphene ◽  
Fifth Order

We have calculated the fifth-order nonlinear optical response at experimentally relevant field strengths within the model of massless Dirac fermions by coupling the massless Dirac fermions to the time-dependent electric field quantum mechanically. It demonstrates that the fifth-order nonlinear optical response plays an important role in the contribution to the optical conductivity of pristine single-layer graphene in the low frequency part of the terahertz regime. The nonlinear effect can enhance the optical activity of single-layer graphene in the terahertz regime and significantly decreases the transmittance of graphene in the regime of frequencies from 0.1 to 0.5 THz. These properties of graphene may be used for photonic and optoelectronic device in the terahertz regime.

Determination of the third- and fifth-order optical nonlinearities: the general case

2014 ◽  
Vol 116 (4) ◽  
pp. 911-917 ◽  
Author(s):  
V. Besse ◽  
G. Boudebs ◽  
H. Leblond
Keyword(s):  
Optical Nonlinearities ◽  
The Third ◽  
Fifth Order
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