Atomic precision fabrication of quantum devices down to the single atom regime

Author(s):  
Richard M. Silver ◽  
Xiqiao Wang ◽  
Fan Fei ◽  
Jon wyrick ◽  
Ranjit Kashid ◽  
...  
2020 ◽  
Vol 49 (31) ◽  
pp. 10701-10707 ◽  
Author(s):  
Xiangsha Du ◽  
Rongchao Jin

This frontier article illustrates single-atom, single-electron level engineering for tailoring the properties of metal nanoclusters using gold as a model.


2020 ◽  
Vol 12 (1) ◽  
Author(s):  
Bowen Zheng ◽  
Grace X. Gu

AbstractDefects in graphene can profoundly impact its extraordinary properties, ultimately influencing the performances of graphene-based nanodevices. Methods to detect defects with atomic resolution in graphene can be technically demanding and involve complex sample preparations. An alternative approach is to observe the thermal vibration properties of the graphene sheet, which reflects defect information but in an implicit fashion. Machine learning, an emerging data-driven approach that offers solutions to learning hidden patterns from complex data, has been extensively applied in material design and discovery problems. In this paper, we propose a machine learning-based approach to detect graphene defects by discovering the hidden correlation between defect locations and thermal vibration features. Two prediction strategies are developed: an atom-based method which constructs data by atom indices, and a domain-based method which constructs data by domain discretization. Results show that while the atom-based method is capable of detecting a single-atom vacancy, the domain-based method can detect an unknown number of multiple vacancies up to atomic precision. Both methods can achieve approximately a 90% prediction accuracy on the reserved data for testing, indicating a promising extrapolation into unseen future graphene configurations. The proposed strategy offers promising solutions for the non-destructive evaluation of nanomaterials and accelerates new material discoveries.


2014 ◽  
Vol 9 (1) ◽  
pp. 235 ◽  
Author(s):  
Chang Chen ◽  
Jinhu Zhang ◽  
Guofeng Dong ◽  
Hezhu Shao ◽  
Bo-yuan Ning ◽  
...  

Author(s):  
Shiqing He ◽  
Qingda Liu ◽  
Xun Wang

Polyoxometalates (POMs) are early transition metal oxide clusters with diverse structures and extensive functions. Due to the excellent redox property and stability, POM clusters can serve as ligands and supports...


Nanoscale ◽  
2021 ◽  
Author(s):  
SAISAI YUAN ◽  
Xiaohui Xu ◽  
Abdalghani Daaoub ◽  
Chao Fang ◽  
Wenqiang Cao ◽  
...  

The control of single atoms offers the fundamental insight for understanding the charge transport through single clusters, and the atomic precision of the clusters provides the opportunity to manipulate the...


2009 ◽  
Vol 86 (4-6) ◽  
pp. 996-998 ◽  
Author(s):  
Moh’d Rezeq ◽  
Christian Joachim ◽  
N. Chandrasekhar
Keyword(s):  

Author(s):  
Wah Chi

Resolution and contrast are the important factors to determine the feasibility of imaging single heavy atoms on a thin substrate in an electron microscope. The present report compares the atom image characteristics in different modes of fixed beam dark field microscopy including the ideal beam stop (IBS), a wire beam stop (WBS), tilted illumination (Tl) and a displaced aperture (DA). Image contrast between one Hg and a column of linearly aligned carbon atoms (representing the substrate), are also discussed. The assumptions in the present calculations are perfectly coherent illumination, atom object is represented by spherically symmetric potential derived from Relativistic Hartree Fock Slater wave functions, phase grating approximation is used to evaluate the complex scattering amplitude, inelastic scattering is ignored, phase distortion is solely due to defocus and spherical abberation, and total elastic scattering cross section is evaluated by the Optical Theorem. The atom image intensities are presented in a Z-modulation display, and the details of calculation are described elsewhere.


Author(s):  
J. J. Hren ◽  
S. D. Walck

The field ion microscope (FIM) has had the ability to routinely image the surface atoms of metals since Mueller perfected it in 1956. Since 1967, the TOF Atom Probe has had single atom sensitivity in conjunction with the FIM. “Why then hasn't the FIM enjoyed the success of the electron microscope?” The answer is closely related to the evolution of FIM/Atom Probe techniques and the available technology. This paper will review this evolution from Mueller's early discoveries, to the development of a viable commercial instrument. It will touch upon some important contributions of individuals and groups, but will not attempt to be all inclusive. Variations in instrumentation that define the class of problems for which the FIM/AP is uniquely suited and those for which it is not will be described. The influence of high electric fields inherent to the technique on the specimens studied will also be discussed. The specimen geometry as it relates to preparation, statistical sampling and compatibility with the TEM will be examined.


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