Influence of spin-orbit coupling on vibronic spectra of metalocomplexes porphin: Manifestation of out-of-plane vibrations

2011 ◽  
Vol 110 (2) ◽  
pp. 234-241 ◽  
Author(s):  
O. L. Gladkova ◽  
A. S. Starukhin ◽  
M. M. Kruk
2021 ◽  
Vol 7 (5) ◽  
pp. eabe2892
Author(s):  
Dmitry Shcherbakov ◽  
Petr Stepanov ◽  
Shahriar Memaran ◽  
Yaxian Wang ◽  
Yan Xin ◽  
...  

Spin-orbit coupling (SOC) is a relativistic effect, where an electron moving in an electric field experiences an effective magnetic field in its rest frame. In crystals without inversion symmetry, it lifts the spin degeneracy and leads to many magnetic, spintronic, and topological phenomena and applications. In bulk materials, SOC strength is a constant. Here, we demonstrate SOC and intrinsic spin splitting in atomically thin InSe, which can be modified over a broad range. From quantum oscillations, we establish that the SOC parameter α is thickness dependent; it can be continuously modulated by an out-of-plane electric field, achieving intrinsic spin splitting tunable between 0 and 20 meV. Unexpectedly, α could be enhanced by an order of magnitude in some devices, suggesting that SOC can be further manipulated. Our work highlights the extraordinary tunability of SOC in 2D materials, which can be harnessed for in operando spintronic and topological devices and applications.


Author(s):  
Muhammad Nauman ◽  
Tayyaba Hussain ◽  
Joonyoung Choi ◽  
Nara Lee ◽  
Young Jai Choi ◽  
...  

Abstract Magnetic anisotropy in strontium iridate (Sr2IrO4) is essential because of its strong spin–orbit coupling and crystal field effect. In this paper, we present a detailed mapping of the out-of-plane (OOP) magnetic anisotropy in Sr2IrO4 for different sample orientations using torque magnetometry measurements in the low-magnetic-field region before the isospins are completely ordered. Dominant in-plane anisotropy was identified at low fields, confirming the b axis as an easy magnetization axis. Based on the fitting analysis of the strong uniaxial magnetic anisotropy, we observed that the main anisotropic effect arises from a spin–orbit-coupled magnetic exchange interaction affecting the OOP interaction. The effect of interlayer exchange interaction results in additional anisotropic terms owing to the tilting of the isospins. The results are relevant for understanding OOP magnetic anisotropy and provide a new way to analyze the effects of spin–orbit-coupling and interlayer magnetic exchange interactions. This study provides insight into the understanding of bulk magnetic, magnetotransport, and spintronic behavior on Sr2IrO4 for future studies.


2015 ◽  
Vol 1 (8) ◽  
pp. 1500114 ◽  
Author(s):  
Kalon Gopinadhan ◽  
Anil Annadi ◽  
Younghyun Kim ◽  
Amar Srivastava ◽  
Brijesh Kumar ◽  
...  

2021 ◽  
Author(s):  
Muhammad Nauman ◽  
Tayyaba Hussain ◽  
Joonyoung Choi ◽  
Nara Lee ◽  
Young Jai Choi ◽  
...  

Abstract Magnetic anisotropy in strontium iridate (Sr2IrO4) is essential because of its strong spin-orbit coupling and crystal field effect. In this study, we investigated the detailed mapping of the out-of-plane (OOP) magnetic anisotropy in Sr2IrO4 for different sample orientations using torque magnetometry measurements in the low-magnetic-field region before the isospins are fully ordered. Dominant in-plane anisotropy was identified at low fields, confirming the b axis as an easy magnetization axis. Based on the fitting analysis of the strong uniaxial magnetic anisotropy, we observed that the main anisotropic effect arises from a spin–orbit-coupled magnetic exchange interaction that affects the OOP interaction. The interlayer exchange interaction results in additional anisotropic terms owing to the tilting of the isospins. Our results are relevant for understanding OOP magnetic anisotropy and provide a new way to analyze the effects of spin–orbit-coupling and interlayer magnetic exchange interactions. This study provides a new insight into the understanding of bulk magnetic, magneto-transport, and spintronic behavior of Sr2IrO4 for future studies.


2011 ◽  
Vol 25 (26) ◽  
pp. 3495-3502 ◽  
Author(s):  
XI FU ◽  
GUANG-HUI ZHOU

We investigate theoretically the spin accumulation of a quantum wire nonadiabatically connected to two normal leads in the presence of Rashba and Dresselhaus spin–orbit coupling (SOC). Using scattering matrix approach within the effective free-electron approximation, three components of spin polarization have been calculated. It is demonstrated that for the Dresselhaus SOC case the out-of-plane spin polarization does not form spin accumulation, and when the two SOC terms coexist the influence of Rashba SOC to the out-of-plane spin accumulation is dominant and symmetry of the spin accumulation is broken due to the existence of Dresselhaus SOC. Moreover, the formation of the out-of-plane spin accumulation is influenced by the ratio of Rashba and Dresselhaus strength, and when the ratio is very small the out-of-plane spin polarization does not show spin accumulation patterns. It is also shown that the spin accumulation for the system is an intrinsic one which can be distinguished from the extrinsic spin accumulation by changing the Rashba strength.


2005 ◽  
Vol 19 (27) ◽  
pp. 4135-4142 ◽  
Author(s):  
QIAN WANG ◽  
LI SHENG

The current induced local spin polarization due to weak Rashba spin-orbit coupling in narrow strip is studied. In the presence of longitudinal charge current, local spin polarizations appear in the sample. The spin polarization perpendicular to the plane has opposite sign near the two edges. The in-plane spin polarization in the direction perpendicular to the sample edges also appears, but does not change sign across the sample. From our scaling analysis based on increasing the strip width, the out-of-plane spin polarization is important mainly in a system of mesoscopic size, and thus appears not to be associated with the spin-Hall effect in bulk samples.


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