A three-dimensional numerical study of the effect of pulsating flow on conversion efficiency inside a catalytic converter

Author(s):  
S.-J. Jeong ◽  
W. S. Kim
Author(s):  
M. H. Akbari ◽  
R. Roohi ◽  
S. A. Asaee

A three-dimensional model is developed to simulate the behavior of a single-channel three-way catalytic converter. The flow regime is assumed to be steady and laminar, and the channel walls are considered as isothermal. A multi-step, global heterogeneous reaction mechanism with 16 reactions and 11 species is used in this investigation to enhance the accuracy of the results. The chemical reactions are assumed to occur only on the reactor walls. The developed model is validated against available experimental data for stoichiometric operating conditions. The effect of the feed temperature on the conversion efficiency of the main pollutant components is studied. The light-off temperature for the stoichiometric A/F is found to be about 530 K for CO, NO and UHC, and 425 K for H2 conversion. The model is also applied to predict the effect of reactor length and inlet mixture space velocity on the conversion efficiency at two different temperatures. By using the same kinetics a well-stirred, unsteady model is also developed to identify the sensitivity of the multi-step kinetic mechanism to the mixture composition. The effect of mole fraction variation of each species on the conversion of other mixture components is investigated.


Author(s):  
Bassem H. Ramadan ◽  
Russel L. Richmond

This study involves a numerical and experimental investigation of fluid flow in automotive catalytic converters. The numerical work involves using computational fluid dynamics (CFD) to perform three-dimensional calculations of turbulent flow in an inlet pipe, inlet cone, catalyst substrate (porous medium), outlet cone, and outlet pipe. The experimental work includes using hot-wire anemometry to measure the velocity profile at the outlet of the catalyst substrate, and pressure drop measurements across the system. Very often, the designer may have to resort to offset inlet and outlet cones, or angled inlet pipes due to space limitations. Hence, it is very difficult to achieve a good flow distribution at the inlet cross section of the catalyst substrate. Therefore, it is important to study the effect of the geometry of the catalytic converter on flow uniformity in the substrate. The analysis involved determining back pressure (BP) across the converter system for different monolith cell densities, mass flow rates, converter aspect ratio, inlet cone angle, and inlet pipe offset. The numerical results were used to study the velocity profile at the inlet to the substrate, and were verified with experimental measurements of velocity and BP.


Author(s):  
Bassem H. Ramadan

Recently, the new regulations on emission standards have prompted a reconsideration of the design of automotive catalytic converters in order to reduce the light-off period of the catalyst. The catalytic converter light-off period is very Important since almost 80% of the emissions from vehicles occur within the first three minutes after cold start in the FTP-75 test. In order to meet these new regulations, current studies have suggested that the catalyst should be “close-coupled”; that is fitted close to the engine exhaust manifold. In order to design “close-coupled” converters, the designer may have to resort to truncated inlet and outlet cones, or distorted inlet pipes due to space limitations. Hence, it is very difficult to achieve good mixing of the exhaust gas, and a good flow distribution at the inlet cross section of the monolith. Based on such a current status in the study of the catalytic converter, the present work focuses on the time-dependent flow patterns, both in the exhaust manifold and the catalytic converter using Computational Fluid Dynamics (CFD). A three-dimensional grid model of an engine exhaust manifold and a close-coupled catalytic converter was developed and analyzed. The flow simulations were performed using KIVA-3 for non-reacting flow fields. These simulations were performed with transient boundary conditions applied at the inlet to the exhaust runners to simulate the opening and closing of exhaust valves. The CFD results were used to study flow uniformity under different operating conditions and to identify the best location of the oxygen sensor.


Author(s):  
C. Abegg ◽  
Graham de Vahl Davis ◽  
W.J. Hiller ◽  
St. Koch ◽  
Tomasz A. Kowalewski ◽  
...  

2012 ◽  
Vol 9 (1) ◽  
pp. 94-97
Author(s):  
Yu.A. Itkulova

In the present work creeping three-dimensional flows of a viscous liquid in a cylindrical tube and a channel of variable cross-section are studied. A qualitative triangulation of the surface of a cylindrical tube, a smoothed and experimental channel of a variable cross section is constructed. The problem is solved numerically using boundary element method in several modifications for a periodic and non-periodic flows. The obtained numerical results are compared with the analytical solution for the Poiseuille flow.


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