scholarly journals Nonlinear optical response of some Graphene oxide and Graphene fluoride derivatives

2016 ◽  
Vol 3 (1) ◽  
Author(s):  
Nikolaos Liaros ◽  
Ioannis Orfanos ◽  
Ioannis Papadakis ◽  
Stelios Couris
Keyword(s):  
Graphene Oxide ◽  
Nonlinear Absorption ◽  
Nonlinear Optical ◽  
Nonlinear Refraction ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Third Order ◽  
Nonlinear Properties ◽  
Graphene Derivatives ◽  
532 Nm

AbstractThe nonlinear optical properties of two graphene derivatives, graphene oxide and graphene fluoride, are investigated by means of the Z-scan technique employing 35 ps and 4 ns, visible (532 nm) laser excitation. Both derivatives were found to exhibit significant third-order nonlinear optical response at both excitation regimes, with the nonlinear absorption being relatively stronger and concealing the presence of nonlinear refraction under ns excitation, while ps excitation reveals the presence of both nonlinear absorption and refraction. Both nonlinear properties are of great interest for several photonics, opto-fluidics, opto-electronics and nanotechnology applications.

scholarly journals Large and negative self-defocusing optical Kerr nonlinearity in Palladium di-Selenide 2D films

2021 ◽  
Author(s):  
David Moss
Keyword(s):  
High Performance ◽  
Nonlinear Optical ◽  
Laser Intensity ◽  
Nonlinear Refraction ◽  
Kerr Nonlinearity ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Closed Aperture ◽  
Third Order ◽  
Limiting Behaviour

Abstract We report a large third-order nonlinear optical response of palladium diselenide (PdSe2) films – a two-dimensional (2D) noble metal dichalcogenide material. Both open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe2 film of β = 3.26 ×10− 8 m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of n2 = -1.33×10− 15 m2/W – two orders of magnitude larger than bulk silicon. We also characterize the variation of n2 as a function of laser intensity, observing that n2 decreases in magnitude with incident laser intensity, becoming saturated at n2 = -9.96×10− 16 m2/W at high intensities. These results verify the large third-order nonlinear optical response of 2D PdSe2 as well as its strong potential for high performance nonlinear photonic devices.

scholarly journals The effects of laser intensities on nonlinear properties for Ag nanoparticles colloid

2019 ◽  
Vol 15 (34) ◽  
pp. 36-40
Author(s):  
Mazin M. Elias
Keyword(s):  
Refractive Index ◽  
Nonlinear Refractive Index ◽  
Nonlinear Optical ◽  
Ccd Camera ◽  
Optical Response ◽  
Blue Laser ◽  
Nonlinear Optical Response ◽  
Third Order ◽  
Nonlinear Properties ◽  
Nano Fluid

A huge potential from researchers was presented for enhancing the nonlinear optical response for materials that interacts by light. In this work, we study the nonlinear optical response for chemically prepared nano- fluid of silver nanoparticles in de-ionized water with TSC (Tri-sodium citrate) protecting agent. By the means of self-defocusing technique and under CW 473 nm blue laser, the reflected diffraction pattern were observed and recorded by CCD camera. The results demonstrate that, the Ag nano-fluid shows a good third order nonlinear response and the magnitude of the nonlinear refractive index was in the order of 10−7 cm2/W. We determine the maximum change of the nonlinear refractive index and the related phase shift for the material at six input laser intensities.

scholarly journals Large negative n2 and two-photon absorption in 2D PdSe2 films ACS AMI OSF

2020 ◽  
Author(s):  
David Moss
Keyword(s):  
High Performance ◽  
Nonlinear Optical ◽  
Laser Intensity ◽  
Nonlinear Refraction ◽  
Kerr Nonlinearity ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Photon Absorption ◽  
Closed Aperture ◽  
Third Order

We report a large third-order nonlinear optical response of palladium diselenide (PdSe2) films – a two-dimensional (2D) noble metal dichalcogenide material. Both open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe2 film of β = 3.26 ×10-8 m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of n2 = -1.33×10-15 m2/W – two orders of magnitude larger than bulk silicon. We also characterize the variation of n2 as a function of laser intensity, observing that n2 decreases in magnitude with incident laser intensity, becoming saturated at n2 = -9.96×10-16 m2/W at high intensities. These results verify the large third-order nonlinear optical response of 2D PdSe2 as well as its strong potential for high performance nonlinear photonic devices.

scholarly journals Large Kerr nonlinearity in PdS2 2D films

2020 ◽  
Author(s):  
linnan jia ◽  
Jiayang Wu ◽  
Baohua Jiao ◽  
Tieshan Yang ◽  
David Moss
Keyword(s):  
High Performance ◽  
Nonlinear Optical ◽  
Laser Intensity ◽  
Nonlinear Refraction ◽  
Kerr Nonlinearity ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Closed Aperture ◽  
Third Order ◽  
Limiting Behaviour

<p>We report a large third-order nonlinear optical response of palladium diselenide (PdSe<sub>2</sub>) films – a two-dimensional (2D) noble metal dichalcogenide material. Both open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe<sub>2</sub> film of <i>β =</i> 3.26 × 10<sup>-8</sup> m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of <i>n</i><sub>2</sub> = -1.33×10<sup>-15</sup> m<sup>2</sup>/W – two orders of magnitude larger than bulk silicon. We also characterize the variation of <i>n</i><sub>2</sub> as a function of laser intensity, observing that <i>n</i><sub>2</sub> decreases in magnitude with incident laser intensity, becoming saturated at <i>n</i><sub>2</sub> = -9.96×10<sup>-16</sup> m<sup>2</sup>/W at high intensities. These results verify the large third-order nonlinear optical response of 2D PdSe<sub>2</sub> as well as its strong potential for high performance nonlinear photonic devices.</p>

Broadband ultrafast nonlinear absorption and nonlinear refraction of layered molybdenum dichalcogenide semiconductors

Nanoscale ◽  
2014 ◽  
Vol 6 (18) ◽  
pp. 10530-10535 ◽  
Author(s):  
Kangpeng Wang ◽  
Yanyan Feng ◽  
Chunxia Chang ◽  
Jingxin Zhan ◽  
Chengwei Wang ◽  
...  
Keyword(s):  
Nonlinear Absorption ◽  
Nonlinear Optical ◽  
Nonlinear Refraction ◽  
Optical Response ◽  
Nonlinear Optical Response

The ultrafast, broadband, nonlinear optical response of a series of layered MoX2 (X = S, Se and Te) dispersions were investigated.

scholarly journals Large Kerr nonlinearity in PdSe2 2D films

2020 ◽  
Author(s):  
linnan jia ◽  
Jiayang Wu ◽  
Baohua Jiao ◽  
Tieshan Yang ◽  
David Moss
Keyword(s):  
High Performance ◽  
Nonlinear Optical ◽  
Laser Intensity ◽  
Nonlinear Refraction ◽  
Kerr Nonlinearity ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Closed Aperture ◽  
Third Order ◽  
Limiting Behaviour

<p>We report a large third-order nonlinear optical response of palladium diselenide (PdSe<sub>2</sub>) films – a two-dimensional (2D) noble metal dichalcogenide material. Both open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe<sub>2</sub> film of <i>β =</i> 3.26 × 10<sup>-8</sup> m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of <i>n</i><sub>2</sub> = -1.33×10<sup>-15</sup> m<sup>2</sup>/W – two orders of magnitude larger than bulk silicon. We also characterize the variation of <i>n</i><sub>2</sub> as a function of laser intensity, observing that <i>n</i><sub>2</sub> decreases in magnitude with incident laser intensity, becoming saturated at <i>n</i><sub>2</sub> = -9.96×10<sup>-16</sup> m<sup>2</sup>/W at high intensities. These results verify the large third-order nonlinear optical response of 2D PdSe<sub>2</sub> as well as its strong potential for high performance nonlinear photonic devices.</p>

scholarly journals Large Kerr nonlinearity in PdSe2 2D films

2020 ◽  
Author(s):  
linnan jia ◽  
Jiayang Wu ◽  
Baohua Jiao ◽  
Tieshan Yang ◽  
David Moss
Keyword(s):  
High Performance ◽  
Nonlinear Optical ◽  
Laser Intensity ◽  
Nonlinear Refraction ◽  
Kerr Nonlinearity ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Closed Aperture ◽  
Third Order ◽  
Limiting Behaviour

<p>We report a large third-order nonlinear optical response of palladium diselenide (PdSe<sub>2</sub>) films – a two-dimensional (2D) noble metal dichalcogenide material. Both open-aperture (OA) and closed-aperture (CA) Z-scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe<sub>2</sub> film of <i>β =</i> 3.26 × 10<sup>-8</sup> m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of <i>n</i><sub>2</sub> = -1.33×10<sup>-15</sup> m<sup>2</sup>/W – two orders of magnitude larger than bulk silicon. We also characterize the variation of <i>n</i><sub>2</sub> as a function of laser intensity, observing that <i>n</i><sub>2</sub> decreases in magnitude with incident laser intensity, becoming saturated at <i>n</i><sub>2</sub> = -9.96×10<sup>-16</sup> m<sup>2</sup>/W at high intensities. These results verify the large third-order nonlinear optical response of 2D PdSe<sub>2</sub> as well as its strong potential for high performance nonlinear photonic devices.</p>

Third-order nonlinear optical response of some tetrasubstituted cumulenes

1993 ◽  
Vol 5 (3) ◽  
pp. 357-360 ◽  
Author(s):  
Ivan Kminek ◽  
Josef Klimovic ◽  
Paras N. Prasad
Keyword(s):  
Nonlinear Optical ◽  
Optical Response ◽  
Nonlinear Optical Response ◽  
Third Order
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