An All-Ceramic Interconnect for Use in Solid-Oxide Fuel Cell Stacks

MRS Bulletin ◽  
2005 ◽  
Vol 30 (8) ◽  
pp. 596-600 ◽  
Author(s):  
Thomas A. Morris ◽  
Eric A. Barringer ◽  
Steven C. Kung ◽  
Rodger W. McKain

AbstractThis article summarizes a unique approach in which all-ceramic interconnects are used in place of metal interconnects in solid-oxide fuel cell (SOFC) stacks. The approach combines advanced SOFC materials with the manufacturing technology and infrastructure established for multilayer ceramic (MLC) packaging for the microelectronics industry. The MLC interconnect is fabricated using multiple layers of yttria-stabilized zirconia (YSZ) tape, with each layer containing conductive vias to provide for electrical current flow through the interconnect. The all-ceramic interconnect design facilitates uniform distribution of air and fuel gas to the respective electrodes of adjacent cells. The multilayer interconnects are fabricated using traditional MLC manufacturing processes. A detailed description of the processes for fabricating the all-ceramic interconnect is presented.To aid in moving from prototype fabrication to commercialization of these fuel cell systems, a detailed cost model has been used as a roadmap for commercial stack development. Cost model projections are presented for three different interconnect footprint sizes. These projections show an SOFC stack cost of less than $150 per kilowatt for the optimized SOFC stack design produced at high volume.

Author(s):  
Pei-Wen Li ◽  
Laura Schaefer ◽  
Qing-Ming Wang ◽  
Minking K. Chyu

A numerical model is presented in this work to compute the inter-dependent fields of flow, temperature and the concentrations of multiple gases in a single tubular solid oxide fuel cell (SOFC) system. It was supposed that the fuel gas supplied to the fuel cell is from a pre-reformer and thus contains hydrogen and proportions of carbon monoxide, carbon dioxide, steam, and methane. The model takes mixture gas properties of the fuel and oxidant as functions of the numerically obtained local temperature, pressure and species concentrations, which are inter-dependent and intimately related to the electrochemical reaction in the SOFC. In the iterative computation steps, local electrochemical parameters were simultaneously calculated based on the local parameters of pressure, temperature, and concentration of the species available at each step. Upon the convergence of the computation, both local details and the overall performance of the fuel cell could be obtained. The numerical results obtained are helpful for better understanding of the operation of SOFCs.


2009 ◽  
Vol 189 (2) ◽  
pp. 1127-1131 ◽  
Author(s):  
Florian P. Nagel ◽  
Tilman J. Schildhauer ◽  
Josef Sfeir ◽  
Alexander Schuler ◽  
Serge M.A. Biollaz

2008 ◽  
Vol 2008.7 (0) ◽  
pp. 1-2
Author(s):  
Shuichi SAWADA ◽  
Seiichi HARUUCHI ◽  
Shingo YOSHIDA ◽  
Masaaki IZUMI

Fuel Cells ◽  
2017 ◽  
Vol 17 (6) ◽  
pp. 825-842 ◽  
Author(s):  
R. Scataglini ◽  
M. Wei ◽  
A. Mayyas ◽  
S. H. Chan ◽  
T. Lipman ◽  
...  

2014 ◽  
Vol 33 (5) ◽  
pp. 439-445 ◽  
Author(s):  
Zhiyuan Chen ◽  
Lijun Wang ◽  
Fushen Li ◽  
Kuochih Chou

AbstractIron-based alloys are the most hopeful interconnects of intermediate temperature solid oxide fuel cell (IT-SOFC). Fe-16Cr alloy is one of the common iron-based alloys. Oxidation of the alloy is the key issue in the running process, which could be described in terms of diffusion path. Chemical potential, which is one of the primary factors to the diffusion process, is determined by the thermodynamics. The equilibrium phase in the oxidation of Fe-16Cr alloy was analyzed for better understanding of the mechanism of alloy oxidation in varied atmosphere. A novel form of thermodynamic diagram associated to the oxidation process was given. Phases in the equilibrium are changing with the quantitative increase of reacted fuel gas during the process. The diagram of Fe-16Cr alloy in atmospheres at cathode and anode sides were calculated. The diagram gives the intuitionistic phase transformation process corresponding to the practical oxidation process in the view of thermodynamics.


Author(s):  
Yuanhui Su ◽  
Tao Wei ◽  
Yining Li ◽  
Baoyi Yin ◽  
Yu Huan ◽  
...  

Methane catalytic abilities are considered to be an important and direct form of experimental evidence for evaluating the efficacy of MIEC anodes for SOFCs with CH4 as the fuel gas.


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