scholarly journals Магнитные структуры и магнитные фазовые переходы в редкоземельных интерметаллидах RMn-=SUB=-2-=/SUB=-Si-=SUB=-2-=/SUB=- (R=Sm, Tb)

2018 ◽  
Vol 60 (6) ◽  
pp. 1071
Author(s):  
Н.В. Мушников ◽  
Е.Г. Герасимов ◽  
В.С. Гавико ◽  
П.Б. Терентьев ◽  
К.А. Язовских ◽  
...  

AbstractThe magnetic structures that form in La_1– x R_ x Mn_2Si_2 ( R = Sm, Tb) layered compounds with various concentrations x have been determined by magnetic neutron diffraction and magnetic measurements, and the magnetic phase diagrams have been built. It is shown that the formation of the magnetic structures is dependent not only on exchange interactions, but also on the type of the magnetic anisotropy of a rare-earth atom. It is found that, in La_1– x Tb_ x Mn_2Si_2 compounds with 0.2 < x < 0.5, the competition of the Tb–Mn and Mn–Mn interlayer exchange interactions and the existence of a strong uniaxial magnetic anisotropy in the Mn and Tb sublattices leads to the frustrated magnetic state and prevents the formation of the long-range magnetic order in the Tb sublattice.

2021 ◽  
Vol 6 (1) ◽  
Author(s):  
Margaret M. Kane ◽  
Arturas Vailionis ◽  
Lauren J. Riddiford ◽  
Apurva Mehta ◽  
Alpha T. N’Diaye ◽  
...  

AbstractThe emergence of ferromagnetism in materials where the bulk phase does not show any magnetic order demonstrates that atomically precise films can stabilize distinct ground states and expands the phase space for the discovery of materials. Here, the emergence of long-range magnetic order is reported in ultrathin (111) LaNiO3 (LNO) films, where bulk LNO is paramagnetic, and the origins of this phase are explained. Transport and structural studies of LNO(111) films indicate that NiO6 octahedral distortions stabilize a magnetic insulating phase at the film/substrate interface and result in a thickness-dependent metal–insulator transition at t = 8 unit cells. Away from this interface, distortions relax and bulk-like conduction is regained. Synchrotron x-ray diffraction and dynamical x-ray diffraction simulations confirm a corresponding out-of-plane unit-cell expansion at the interface of all films. X-ray absorption spectroscopy reveals that distortion stabilizes an increased concentration of Ni2+ ions. Evidence of long-range magnetic order is found in anomalous Hall effect and magnetoresistance measurements, likely due to ferromagnetic superexchange interactions among Ni2+–Ni3+ ions. Together, these results indicate that long-range magnetic ordering and metallicity in LNO(111) films emerges from a balance among the spin, charge, lattice, and orbital degrees of freedom.


2005 ◽  
Vol 71 (21) ◽  
Author(s):  
Zahirul Islam ◽  
D. Haskel ◽  
J. C. Lang ◽  
G. Srajer ◽  
X. Liu ◽  
...  

2000 ◽  
Vol 658 ◽  
Author(s):  
J. E. L. Waldron ◽  
M. A. Green

ABSTRACTThe synthesis, structure and magnetic properties of monoclinic Nb12O29 are described. The synthesis of a pure bulk sample is difficult due to the large number of other similar phases. It is achieved by rapid reduction of H-Nb2O5 with Nb metal. The compound is shown to undergo a charge ordering transition at low temperature which provokes long range magnetic order in an intriguing one dimensional arrangement.


1995 ◽  
Vol 7 (3) ◽  
pp. 597-610 ◽  
Author(s):  
E Gratz ◽  
R Hauser ◽  
A Lindbaum ◽  
M Maikis ◽  
R Resel ◽  
...  

2000 ◽  
Vol 61 (2) ◽  
pp. 1199-1205 ◽  
Author(s):  
Vishal Mehra ◽  
Jayme De Luca

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