scholarly journals Low cloud reduction within the smoky marine boundary layer and the diurnal cycle

2019 ◽  
Author(s):  
Jianhao Zhang ◽  
Paquita Zuidema
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Cloud Cover ◽  
Marine Boundary Layer ◽  
Field Measurements ◽  
Cloud Layer ◽  
Free Troposphere ◽  
Liquid Water Path ◽  
Low Cloud ◽  
Low Cloud Cover

Abstract. Previous observational studies of the southeast Atlantic emphasize an increase in the stratocumulus cloud cover when shortwave-absorbing aerosols are present in the free-troposphere. Recent field measurements at Ascension Island (8° S, 14.5° W) reveal that smoke is also often present in the marine boundary layer, most evident in August when the smoke is highly absorbing of sunlight, the boundary layer is deeper, the cloud-top inversion is weaker, and a climatologically lower cloud fraction eases penetration of the sunlight to the surface, compared to later months. In these conditions, the low cloud cover decreases further with enhanced smoke loadings, reflecting a boundary layer semi-direct effect that is a positive feedback. The low cloud cover reduction is particularly pronounced in the afternoon, although the cloud liquid water path is more strongly reduced at night. The daily-mean surface-based mixed layer is warmer by approximately 0.5 K when more smoke is present in the boundary layer, with a warming peak in the late afternoon when the cloud cover reduction is largest. After sunset, sub-cloud moisture accumulates throughout the night, increasing the moisture stratification with the cloud layer. This increase in boundary layer decoupling is consistent with reduced turbulence. A new observation is that in the sunlit morning hours, the smokier boundary layer deepens by approximately 200 m, and both the liquid water paths and cloud top heights increase. We speculate this reflects radiatively-induced vertical ascent originating from within a well-mixed smoke-filled sub-cloud layer. Overall, the reduction in daytime low cloud decreases the top-of-atmosphere all-sky albedo, despite an increase in the top-of-atmosphere direct aerosol radiation of ~ 6.5 W m2 between the (most-least) smoky tercile composites. A convolving meteorological influence is also apparent near the cloud top, in that, although the free troposphere is also often smoky in August, the associated above-cloud potential temperatures are often cooler, rather than warmer, and better-mixed. The cooling weakens the inversion beyond that expected from the warming of the boundary layer and further encourages entrainment of more smoke into the already smoky boundary layer, increasing the longevity of the boundary layer smoke events. The free-tropospheric winds are also typically stronger and more easterly. More smoke appears to settle into the sub-cloud layer during the day than at night when it is smoky, speculated to reflect a deeper daytime sub-cloud layer facilitating entrainment, when the nighttime stratification does not.

scholarly journals The diurnal cycle of the smoky marine boundary layer observed during August in the remote southeast Atlantic

2019 ◽  
Vol 19 (23) ◽  
pp. 14493-14516 ◽  
Author(s):  
Jianhao Zhang ◽  
Paquita Zuidema
Keyword(s):  
Boundary Layer ◽  
Diurnal Cycle ◽  
Liquid Water ◽  
Marine Boundary Layer ◽  
Field Measurements ◽  
Cloud Layer ◽  
Liquid Water Path ◽  
Stratiform Cloud ◽  
Cloud Liquid Water ◽  
Cloud Models

Abstract. Ascension Island (8∘ S, 14.5∘ W) is located at the northwestern edge of the south Atlantic stratocumulus deck, with most clouds in August characterized by surface observers as “stratocumulus and cumulus with bases at different levels”, and secondarily as “cumulus of limited vertical extent” and occurring within a typically decoupled boundary layer. Field measurements have previously shown that the highest amounts of sunlight-absorbing smoke occur annually within the marine boundary layer during August. On more smoke-free days, the diurnal cycle in cloudiness includes a nighttime maximum in cloud liquid water path and rain, an afternoon cloud minimum, and a secondary late-afternoon increase in cumulus and rain. The afternoon low-cloud minimum is more pronounced on days with a smokier boundary layer. The cloud liquid water paths are also reduced throughout most of the diurnal cycle when more smoke is present, with the difference from cleaner conditions most pronounced at night. Precipitation is infrequent. An exception is the mid-morning, when the boundary layer deepens and liquid water paths increase. The data support a view that a radiatively enhanced decoupling persisting throughout the night is key to understanding the changes in the cloud diurnal cycle when the boundary layer is smokier. Under these conditions, the nighttime stratiform cloud layer does not always recouple to the sub-cloud layer, and the decoupling maintains more moisture within the sub-cloud layer. After the sun rises, enhanced shortwave absorption in a smokier boundary layer can drive a vertical ascent that momentarily couples the sub-cloud layer to the cloud layer, deepening the boundary layer and ventilating moisture throughout, a process that may also be aided by a shift to smaller droplets. After noon, shortwave absorption within smokier boundary layers again reduces the upper-level stratiform cloud and the sub-cloud relative humidity, discouraging further cumulus development and again strengthening a decoupling that lasts longer into the night. The novel diurnal mechanism provides a new challenge for cloud models to emulate. The lower free troposphere above cloud is more likely to be cooler, when boundary layer smoke is present, and lower free-tropospheric winds are stronger and more northeasterly, with both (meteorological) influences supporting further smoke entrainment into the boundary layer from above.

scholarly journals Synoptic-scale controls of fog and low-cloud variability in the Namib Desert

2020 ◽  
Vol 20 (6) ◽  
pp. 3415-3438 ◽  
Author(s):  
Hendrik Andersen ◽  
Jan Cermak ◽  
Julia Fuchs ◽  
Peter Knippertz ◽  
Marco Gaetani ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Cloud Cover ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Synoptic Scale ◽  
Namib Desert ◽  
Data Set ◽  
Air Masses ◽  
Low Cloud ◽  
Low Cloud Cover

Abstract. Fog is a defining characteristic of the climate of the Namib Desert, and its water and nutrient input are important for local ecosystems. In part due to sparse observation data, the local mechanisms that lead to fog occurrence in the Namib are not yet fully understood, and to date, potential synoptic-scale controls have not been investigated. In this study, a recently established 14-year data set of satellite observations of fog and low clouds in the central Namib is analyzed in conjunction with reanalysis data in order to identify synoptic-scale patterns associated with fog and low-cloud variability in the central Namib during two seasons with different spatial fog occurrence patterns. It is found that during both seasons, mean sea level pressure and geopotential height at 500 hPa differ markedly between fog/low-cloud and clear days, with patterns indicating the presence of synoptic-scale disturbances on fog and low-cloud days. These regularly occurring disturbances increase the probability of fog and low-cloud occurrence in the central Namib in two main ways: (1) an anomalously dry free troposphere in the coastal region of the Namib leads to stronger longwave cooling of the marine boundary layer, increasing low-cloud cover, especially over the ocean where the anomaly is strongest; (2) local wind systems are modulated, leading to an onshore anomaly of marine boundary-layer air masses. This is consistent with air mass back trajectories and a principal component analysis of spatial wind patterns that point to advected marine boundary-layer air masses on fog and low-cloud days, whereas subsiding continental air masses dominate on clear days. Large-scale free-tropospheric moisture transport into southern Africa seems to be a key factor modulating the onshore advection of marine boundary-layer air masses during April, May, and June, as the associated increase in greenhouse gas warming and thus surface heating are observed to contribute to a continental heat low anomaly. A statistical model is trained to discriminate between fog/low-cloud and clear days based on information on large-scale dynamics. The model accurately predicts fog and low-cloud days, illustrating the importance of large-scale pressure modulation and advective processes. It can be concluded that regional fog in the Namib is predominantly of an advective nature and that fog and low-cloud cover is effectively maintained by increased cloud-top radiative cooling. Seasonally different manifestations of synoptic-scale disturbances act to modify its day-to-day variability and the balance of mechanisms leading to its formation and maintenance. The results are the basis for a new conceptual model of the synoptic-scale mechanisms that control fog and low-cloud variability in the Namib Desert and will guide future studies of coastal fog regimes.

scholarly journals Factors Controlling Low-Cloud Evolution over the Eastern Subtropical Oceans: A Lagrangian Perspective Using the A-Train Satellites

2015 ◽  
Vol 73 (1) ◽  
pp. 331-351 ◽  
Author(s):  
Ryan Eastman ◽  
Robert Wood
Keyword(s):  
Boundary Layer ◽  
Boundary Layers ◽  
Liquid Water ◽  
Cloud Cover ◽  
Liquid Water Path ◽  
Water Path ◽  
Cloud Properties ◽  
Droplet Concentration ◽  
Low Cloud ◽  
Cloud Evolution

Abstract A Lagrangian technique is developed to sample satellite data to quantify and understand factors controlling temporal changes in low-cloud properties (cloud cover, areal-mean liquid water path, and droplet concentration). Over 62 000 low-cloud scenes over the eastern subtropical/tropical oceans are sampled using the A-Train satellites. Horizontal wind fields at 925 hPa from the ERA-Interim are used to compute 24-h, two-dimensional, forward, boundary layer trajectories with trajectory locations starting on the CloudSat/CALIPSO track. Cloud properties from MODIS and AMSR-E are sampled at the trajectory start and end points, allowing for direct measurement of the temporal cloud evolution. The importance of various controls (here, boundary layer depth, lower-tropospheric stability, and precipitation) on cloud evolution is evaluated by comparing cloud evolution for different initial values of these controls. Viewing angle biases are removed and cloud anomalies (diurnal and seasonal cycles removed) are used throughout to quantify cloud evolution relative to the climatological-mean evolution. Cloud property anomalies show temporal changes similar to those expected for a stochastic red noise process, with linear relationships between initial anomalies and their mean 24-h changes. This creates a potential bias when comparing the evolutions of sets of trajectories with different initial anomalies; three methods are introduced and evaluated to account for this. Results provide statistically robust observational support for theoretical/modeling studies by showing that low clouds in deep boundary layers and under weak inversions are prone to break up. Precipitation shows a more complex and less statistically significant relationship with cloud breakup. Cloud cover in shallow precipitating boundary layers is more persistent than in deep precipitating boundary layers. Liquid water path and cloud droplet concentration decrease more rapidly for precipitating clouds and in deep boundary layers.

scholarly journals Southeast Pacific stratocumulus clouds, precipitation and boundary layer structure sampled along 20° S during VOCALS-REx

2010 ◽  
Vol 10 (21) ◽  
pp. 10639-10654 ◽  
Author(s):  
C. S. Bretherton ◽  
R. Wood ◽  
R. C. George ◽  
D. Leon ◽  
G. Allen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Vertical Structure ◽  
Layer Structure ◽  
Cloud Droplet ◽  
Free Troposphere ◽  
Liquid Water Path ◽  
Typical Structure ◽  
Southeast Pacific ◽  
Over The Top

Abstract. Multiplatform airborne, ship-based, and land-based observations from 16 October–15 November 2008 during the VOCALS Regional Experiment (REx) are used to document the typical structure of the Southeast Pacific stratocumulus-topped boundary layer and lower free troposphere on a~transect along 20° S between the coast of Northern Chile and a buoy 1500 km offshore. Strong systematic gradients in clouds, precipitation and vertical structure are modulated by synoptically and diurnally-driven variability. The boundary layer is generally capped by a strong (10–12 K), sharp inversion. In the coastal zone, the boundary layer is typically 1 km deep, fairly well mixed, and topped by thin, nondrizzling stratocumulus with accumulation-mode aerosol and cloud droplet concentrations exceeding 200 cm−3. Far offshore, the boundary layer depth is typically deeper (1600 m) and more variable, and the vertical structure is usually decoupled. The offshore stratocumulus typically have strong mesoscale organization, much higher peak liquid water paths, extensive drizzle, and cloud droplet concentrations below 100 cm−3, sometimes with embedded pockets of open cells with lower droplet concentrations. The lack of drizzle near the coast is not just a microphysical response to high droplet concentrations; smaller cloud depth and liquid water path than further offshore appear comparably important. Moist boundary layer air is heated and mixed up along the Andean slopes, then advected out over the top of the boundary layer above adjacent coastal ocean regions. Well offshore, the lower free troposphere is typically much drier. This promotes strong cloud-top radiative cooling and stronger turbulence in the clouds offshore. In conjunction with a slightly cooler free troposphere, this may promote stronger entrainment that maintains the deeper boundary layer seen offshore. Winds from ECMWF and NCEP operational analyses have an rms difference of only 1 m s−1 from collocated airborne leg-mean observations in the boundary layer and 2 m s−1 above the boundary layer. This supports the use of trajectory analysis for interpreting REx observations. Two-day back-trajectories from the 20° S transect suggest that eastward of 75° W, boundary layer (and often free-tropospheric) air has usually been exposed to South American coastal aerosol sources, while at 85° W, neither boundary-layer or free-tropospheric air has typically had such contact.

Spatial Variability of Liquid Water Path in Marine Low Cloud: The Importance of Mesoscale Cellular Convection

2006 ◽  
Vol 19 (9) ◽  
pp. 1748-1764 ◽  
Author(s):  
Robert Wood ◽  
Dennis L. Hartmann
Keyword(s):  
Spatial Variability ◽  
Liquid Water ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Liquid Water Path ◽  
Water Path ◽  
Geographical Regions ◽  
Low Cloud ◽  
Moderate Resolution Imaging Spectroradiometer ◽  
Subtropical Oceans

Abstract Liquid water path (LWP) mesoscale spatial variability in marine low cloud over the eastern subtropical oceans is examined using two months of daytime retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) on the NASA Terra satellite. Approximately 20 000 scenes of size 256 km × 256 km are used in the analysis. It is found that cloud fraction is strongly linked with the LWP variability in the cloudy fraction of the scene. It is shown here that in most cases LWP spatial variance is dominated by horizontal scales of 10–50 km, and increases as the variance-containing scale increases, indicating the importance of organized mesoscale cellular convection (MCC). A neural network technique is used to classify MODIS scenes by the spatial variability type (no MCC, closed MCC, open MCC, cellular but disorganized). It is shown how the different types tend to occupy distinct geographical regions and different physical regimes within the subtropics, although the results suggest considerable overlap of the large-scale meteorological conditions associated with each scene type. It is demonstrated that both the frequency of occurrence, and the variance-containing horizontal scale of the MCC increases as the marine boundary layer (MBL) depth increases. However, for the deepest MBLs, the MCC tends to be replaced by clouds containing cells but lacking organization. In regions where MCC is prevalent, a lack of sensitivity of the MCC type (open or closed) to the large-scale meteorology was found, suggesting a mechanism internal to the MBL may be important in determining MCC type. The results indicate that knowledge of the physics of MCC will be required to completely understand and predict low cloud coverage and variability in the subtropics.

scholarly journals Evaluation of stratocumulus cloud prediction in the Met Office forecast model during VOCALS-REx

2010 ◽  
Vol 10 (21) ◽  
pp. 10541-10559 ◽  
Author(s):  
S. J. Abel ◽  
D. N. Walters ◽  
G. Allen
Keyword(s):  
Boundary Layer ◽  
Diurnal Cycle ◽  
Liquid Water ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Coastal Region ◽  
Forecast Model ◽  
Good Representation ◽  
Liquid Water Path ◽  
Water Path

Abstract. Observations in the subtropical southeast Pacific obtained during the VOCALS-REx field experiment are used to evaluate the representation of stratocumulus cloud in the Met Office forecast model and to identify key areas where model biases exist. Marked variations in the large scale structure of the cloud field were observed during the experiment on both day-to-day and on diurnal timescales. In the remote maritime region the model is shown to have a good representation of synoptically induced variability in both cloud cover and marine boundary layer depth. Satellite observations show a strong diurnal cycle in cloud fraction and liquid water path in the stratocumulus with enhanced clearances of the cloud deck along the Chilean and Peruvian coasts on certain days. The model accurately simulates the phase of the diurnal cycle but is unable to capture the coastal clearing of cloud. Observations along the 20° S latitude line show a gradual increase in the depth of the boundary layer away from the coast. This trend is well captured by the model (typical low bias of 200 m) although significant errors exist at the coast where the model marine boundary layer is too shallow and moist. Drizzle in the model responds to changes in liquid water path in a manner that is consistent with previous ship-borne observations in the region although the intensity of this drizzle is likely to be too high, particularly in the more polluted coastal region where higher cloud droplet number concentrations are typical. Another mode of variability in the cloud field that the model is unable to capture are regions of pockets of open cellular convection embedded in the overcast stratocumulus deck and an example of such a feature that was sampled during VOCALS-REx is shown.

On the Relationship between Stratiform Low Cloud Cover and Lower-Tropospheric Stability

2006 ◽  
Vol 19 (24) ◽  
pp. 6425-6432 ◽  
Author(s):  
Robert Wood ◽  
Christopher S. Bretherton
Keyword(s):  
Boundary Layer ◽  
Temperature Profile ◽  
Cloud Cover ◽  
Cloud Amount ◽  
Lapse Rate ◽  
Stratus Cloud ◽  
Low Clouds ◽  
Wide Range ◽  
Low Cloud ◽  
Low Cloud Cover

Abstract Observations in subtropical regions show that stratiform low cloud cover is well correlated with the lower-troposphere stability (LTS), defined as the difference in potential temperature θ between the 700-hPa level and the surface. The LTS can be regarded as a measure of the strength of the inversion that caps the planetary boundary layer (PBL). A stronger inversion is more effective at trapping moisture within the marine boundary layer (MBL), permitting greater cloud cover. This paper presents a new formulation, called the estimated inversion strength (EIS), to estimate the strength of the PBL inversion given the temperatures at 700 hPa and at the surface. The EIS accounts for the general observation that the free-tropospheric temperature profile is often close to a moist adiabat and its lapse rate is strongly temperature dependent. Therefore, for a given LTS, the EIS is greater at colder temperatures. It is demonstrated that while the seasonal cycles of LTS and low cloud cover fraction (CF) are strongly correlated in many regions, no single relationship between LTS and CF can be found that encompasses the wide range of temperatures occurring in the Tropics, subtropics, and midlatitudes. However, a single linear relationship between CF and EIS explains 83% of the regional/seasonal variance in stratus cloud amount, suggesting that EIS is a more regime-independent predictor of stratus cloud amount than is LTS under a wide range of climatological conditions. The result has some potentially important implications for how low clouds might behave in a changed climate. In contrast to Miller’s thermostat hypothesis that a reduction in the lapse rate (Clausius–Clapeyron) will lead to increased LTS and increased tropical low cloud cover in a warmer climate, the results here suggest that low clouds may be much less sensitive to changes in the temperature profile if the vertical profile of tropospheric warming follows a moist adiabat.

scholarly journals Manipulating marine stratocumulus cloud amount and albedo: a process-modelling study of aerosol-cloud-precipitation interactions in response to injection of cloud condensation nuclei

2011 ◽  
Vol 11 (1) ◽  
pp. 885-916 ◽  
Author(s):  
H. Wang ◽  
P. J. Rasch ◽  
G. Feingold
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Marine Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Cloud Amount ◽  
Number Concentration ◽  
Condensation Nuclei ◽  
Liquid Water Path ◽  
Water Path ◽  
Injection Method

Abstract. We use a cloud-system-resolving model to study marine-cloud brightening. We examine how injected aerosol particles that act as cloud condensation nuclei (CCN) are transported within the marine boundary layer and how the additional particles in clouds impact cloud microphysical processes, and feedback on dynamics. Results show that the effectiveness of cloud brightening depends strongly on meteorological and background aerosol conditions. Cloud albedo enhancement is very effective in a weakly precipitating boundary layer and in CCN-limited conditions preceded by heavy and/or persistent precipitation. The additional CCN help sustain cloud water by weakening the precipitation substantially in the former case and preventing the boundary layer from collapse in the latter. For a given amount of injected CCN, the injection method (i.e., number and distribution of sprayers) is critical to the spatial distribution of these CCN. Both the areal coverage and the number concentration of injected particles are key players but neither one always emerges as more important than the other. The same amount of injected material is much less effective in either strongly precipitating clouds or polluted clouds, and it is ineffective in a relatively dry boundary layer that supports clouds of low liquid water path. In the polluted case and "dry" case, the CCN injection increases drop number concentration but lowers supersaturation and liquid water path. As a result, the cloud experiences very weak albedo enhancement, regardless of the injection method.

scholarly journals The Role of Precipitation in Controlling the Transition from Stratocumulus to Cumulus Clouds in a Northern Hemisphere Cold-Air Outbreak

2017 ◽  
Vol 74 (7) ◽  
pp. 2293-2314 ◽  
Author(s):  
Steven J. Abel ◽  
Ian A. Boutle ◽  
Kirk Waite ◽  
Stuart Fox ◽  
Philip R. A. Brown ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Rapid Change ◽  
Supercooled Liquid ◽  
Cloud Layer ◽  
Liquid Water Path ◽  
Cumulus Clouds ◽  
Cold Air ◽  
Stratiform Region ◽  
Cold Air Outbreak

Abstract Aircraft observations in a cold-air outbreak to the north of the United Kingdom are used to examine the boundary layer and cloud properties in an overcast mixed-phase stratocumulus cloud layer and across the transition to more broken open-cellular convection. The stratocumulus cloud is primarily composed of liquid drops with small concentrations of ice particles and there is a switch to more glaciated conditions in the shallow cumulus clouds downwind. The rapid change in cloud morphology is accompanied by enhanced precipitation with secondary ice processes becoming active and greater thermodynamic gradients in the subcloud layer. The measurements also show a removal of boundary layer accumulation mode aerosols via precipitation processes across the transition that are similar to those observed in the subtropics in pockets of open cells. Simulations using a convection-permitting (1.5-km grid spacing) regional version of the Met Office Unified Model were able to reproduce many of the salient features of the cloud field although the liquid water path in the stratiform region was too low. Sensitivity studies showed that ice was too active at removing supercooled liquid water from the cloud layer and that improvements could be made by limiting the overlap between the liquid water and ice phases. Precipitation appears to be the key mechanism responsible for initiating the transition from closed- to open-cellular convection by decoupling the boundary layer and depleting liquid water from the stratiform cloud.

scholarly journals Ultra-clean and smoky marine boundary layers frequently occur in the same season over the southeast Atlantic

2020 ◽  
Vol 20 (4) ◽  
pp. 2341-2351 ◽  
Author(s):  
Sam Pennypacker ◽  
Michael Diamond ◽  
Robert Wood
Keyword(s):  
Boundary Layer ◽  
Boundary Layers ◽  
Biomass Burning ◽  
Liquid Water ◽  
Marine Boundary Layer ◽  
Liquid Water Path ◽  
Accumulation Mode ◽  
Water Path ◽  
Aerosol Cloud ◽  
Ascension Island

Abstract. We study 41 d with daily median surface accumulation mode aerosol particle concentrations below 50 cm−3 (ultra-clean conditions) observed at Ascension Island (ASI; 7.9∘ S, 14.4∘ W) between June 2016 and October 2017 as part of the Layered Atlantic Smoke Interactions with Clouds (LASIC) campaign. Interestingly, these days occur during a period of great relevance for aerosol–cloud–radiation interactions, the southeast Atlantic (SEATL) biomass-burning season (approximately June–October). That means that these critical months can feature both the highest surface aerosol numbers, from smoke intrusion into the marine boundary layer, as well as the lowest. While carbon monoxide and refractory black carbon concentrations on ultra-clean days do not approach those on days with heavy smoke, they also frequently exceed background concentrations calculated in the non-burning season from December 2016 to April 2017. This is evidence that even what become ultra-clean boundary layers can make contact with and entrain from an overlying SEATL smoke layer before undergoing a process of rapid aerosol removal. Because many ultra-clean and polluted boundary layers observed at Ascension Island during the biomass burning season follow similar isobaric back trajectories, the variability in this entrainment is likely more closely tied to the variability in the overlying smoke rather than large-scale horizontal circulation through the boundary layer. Since exceptionally low accumulation mode aerosol numbers at ASI do not necessarily indicate the relative lack of other trace pollutants, this suggests the importance of regional variations in what constitutes an “ultra-clean” marine boundary layer. Finally, surface drizzle rates, frequencies and accumulation – as well as retrievals of liquid water path – all consistently tend toward higher values on ultra-clean days. This implicates enhanced coalescence scavenging in low clouds as the key driver of ultra-clean events in the southeast Atlantic marine boundary layer. These enhancements occur against and are likely mediated by the backdrop of a seasonal increase in daily mean cloud fraction and daily median liquid water path over ASI, peaking in September and October in both LASIC years. Therefore the seasonality in ultra-clean day occurrence seems directly linked to the seasonality in SEATL cloud properties. These results highlight the importance of two-way aerosol–cloud interactions in the region.

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