Abstract. The state-of-the-science Community Multiscale Air Quality (CMAQ) Modeling System which has recently been extended for hemispheric-scale modeling applications (referred to as H-CMAQ), is applied to study the trans-Pacific transport, a phenomenon recognized as a potential source of air pollution in the U.S.A., during April 2010. The results of this analysis are presented in two parts. In the previous part 1 paper, model evaluation for tropospheric ozone (O3) was presented and an air mass characterization method was developed. Results from applying this newly established method pointed to the importance of emissions as the factor to enhance surface O3 mixing ratio over the U.S.A. In this subsequent part 2 paper, emission impacts are examined based on mathematically rigorous sensitivity analysis using the higher-order decoupled direct method (HDDM) implemented in H-CMAQ. The HDDM sensitivity coefficients indicate the presence of a NOx-sensitive regime during April 2010 over most of the northern hemisphere. By defining emission source regions over the U.S.A. and East Asia, impacts from these emission sources are examined. At the surface during April 2010, the emission impacts of the U.S.A. and East Asia are comparable over the western U.S.A. with a magnitude of about 3 ppbv impacts on a monthly mean of all hours basis whereas the impact of domestic emissions dominates over the eastern U.S.A. with a magnitude of about 10 ppbv impacts on a monthly mean basis. The positive correlation (r = 0.63) between surface O3 mixing ratios and domestic emission impacts is confirmed. In contrast, the relationship between surface O3 mixing ratios and emission impacts from East Asia exhibits a flat slope when considering the entire U.S.A. However, this relationship has strong regional differences between the western and eastern U.S.A.; the western region exhibits a positive correlation (r = 0.36–0.38) whereas the latter exhibits a flat slope (r
Supplementary material to "Modeling Trans-Pacific Transport and Stratospheric Intrusion of
Tropospheric Ozone using Hemispheric CMAQ during April 2010:
Part 2. Examination of Emission Impacts based on the Higher-order
Decoupled Direct Method"