scholarly journals Review of “Source apportionment and impact of long-range transport on carbonaceous aerosol particles in Central Germany during HCCT-2010”

2020 ◽  
Author(s):  
Anonymous
Keyword(s):  
Source Apportionment ◽  
Long Range ◽  
Aerosol Particles ◽  
Carbonaceous Aerosol ◽  
Long Range Transport ◽  
Central Germany ◽  
Range Transport

scholarly journals Source apportionment of the organic aerosol over the Atlantic Ocean from 53° N to 53° S: significant contributions from marine emissions and long-range transport

2018 ◽  
Vol 18 (24) ◽  
pp. 18043-18062 ◽  
Author(s):  
Shan Huang ◽  
Zhijun Wu ◽  
Laurent Poulain ◽  
Manuela van Pinxteren ◽  
Maik Merkel ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
Source Apportionment ◽  
Long Range ◽  
Aerosol Particles ◽  
Organic Aerosol ◽  
Long Range Transport ◽  
Data Set ◽  
Climate Effect ◽  
Dms Oxidation ◽  
Range Transport

Abstract. Marine aerosol particles are an important part of the natural aerosol systems and might have a significant impact on the global climate and biological cycle. It is widely accepted that truly pristine marine conditions are difficult to find over the ocean. However, the influence of continental and anthropogenic emissions on the marine boundary layer (MBL) aerosol is still less understood and non-quantitative, causing uncertainties in the estimation of the climate effect of marine aerosols. This study presents a detailed chemical characterization of the MBL aerosol as well as the source apportionment of the organic aerosol (OA) composition. The data set covers the Atlantic Ocean from 53∘ N to 53∘ S, based on four open-ocean cruises in 2011 and 2012. The aerosol particle composition was measured with a high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS), which indicated that sub-micrometer aerosol particles over the Atlantic Ocean are mainly composed of sulfates (50 % of the particle mass concentration), organics (21 %) and sea salt (12 %). OA has been apportioned into five factors, including three factors linked to marine sources and two with continental and/or anthropogenic origins. The marine oxygenated OA (MOOA, 16 % of the total OA mass) and marine nitrogen-containing OA (MNOA, 16 %) are identified as marine secondary products with gaseous biogenic precursors dimethyl sulfide (DMS) or amines. Marine hydrocarbon-like OA (MHOA, 19 %) was attributed to the primary emissions from the Atlantic Ocean. The factor for the anthropogenic oxygenated OA (Anth-OOA, 19 %) is related to continental long-range transport. Represented by the combustion oxygenated OA (Comb-OOA), aged combustion emissions from maritime traffic and wild fires in Africa contributed, on average, a large fraction to the total OA mass (30 %). This study provides the important finding that long-range transport was found to contribute averagely 49 % of the submicron OA mass over the Atlantic Ocean. This is almost equal to that from marine sources (51 %). Furthermore, a detailed latitudinal distribution of OA source contributions showed that DMS oxidation contributed markedly to the OA over the South Atlantic during spring, while continental-related long-range transport largely influenced the marine atmosphere near Europe and western and central Africa (15∘ N to 15∘ S). In addition, supported by a solid correlation between marine tracer methanesulfonic acid (MSA) and the DMS-oxidation OA (MOOA, R2>0.85), this study suggests that the DMS-related secondary organic aerosol (SOA) over the Atlantic Ocean could be estimated by MSA and a scaling factor of 1.79, especially in spring.

scholarly journals Source apportionment and impact of long-range transport on carbonaceous aerosol particles in central Germany during HCCT-2010

2021 ◽  
Vol 21 (5) ◽  
pp. 3667-3684
Author(s):  
Laurent Poulain ◽  
Benjamin Fahlbusch ◽  
Gerald Spindler ◽  
Konrad Müller ◽  
Dominik van Pinxteren ◽  
...  
Keyword(s):  
Black Carbon ◽  
Long Range ◽  
Biomass Burning ◽  
Mass Concentration ◽  
Carbonaceous Aerosol ◽  
Long Range Transport ◽  
Air Masses ◽  
Central Germany ◽  
Range Transport ◽  
Local Emissions

Abstract. The identification of different sources of the carbonaceous aerosol (organics and black carbon) was investigated at a mountain forest site located in central Germany from September to October 2010 to characterize incoming air masses during the Hill Cap Cloud Thuringia 2010 (HCCT-2010) experiment. The near-PM1 chemical composition, as measured by a high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS), was dominated by organic aerosol (OA; 41 %) followed by sulfate (19 %) and nitrate (18 %). Source apportionment of the OA fraction was performed using the multilinear engine (ME-2) approach, resulting in the identification of the following five factors: hydrocarbon-like OA (HOA; 3 % of OA mass), biomass burning OA (BBOA; 13 %), semi-volatile-like OA (SV-OOA; 19 %), and two oxygenated OA (OOA) factors. The more oxidized OOA (MO-OOA, 28 %) was interpreted as being influenced by aged, polluted continental air masses, whereas the less oxidized OOA (LO-OOA, 37 %) was found to be more linked to aged biogenic sources. Equivalent black carbon (eBC), measured by a multi-angle absorption photometer (MAAP) represented 10 % of the total particulate matter (PM). The eBC was clearly associated with HOA, BBOA, and MO-OOA factors (all together R2=0.83). Therefore, eBC's contribution to each factor was achieved using a multi-linear regression model. More than half of the eBC (52 %) was associated with long-range transport (i.e., MO-OOA), whereas liquid fuel eBC (35 %) and biomass burning eBC (13 %) were associated with local emissions, leading to a complete apportionment of the carbonaceous aerosol. The separation between local and transported eBC was well supported by the mass size distribution of elemental carbon (EC) from Berner impactor samples. Air masses with the strongest marine influence, based on back trajectory analysis, corresponded with a low particle mass concentration (6.4–7.5 µg m−3) and organic fraction (≈30 %). However, they also had the largest contribution of primary OA (HOA ≈ 4 % and BBOA 15 %–20 %), which was associated with local emissions. Continental air masses had the highest mass concentration (11.4–12.6 µg m−3), and a larger fraction of oxygenated OA (≈45 %) indicated highly processed OA. The present results emphasize the key role played by long-range transport processes not only in the OA fraction but also in the eBC mass concentration and the importance of improving our knowledge on the identification of eBC sources.

scholarly journals Source apportionment and impact of long-range transport on carbonaceous aerosol particles in Central Germany during HCCT-2010

2020 ◽  
Author(s):  
Laurent Poulain ◽  
Benjamin Fahlbusch ◽  
Gerald Spindler ◽  
Konrad Müller ◽  
Dominik van Pinxteren ◽  
...  
Keyword(s):  
Black Carbon ◽  
Long Range ◽  
Biomass Burning ◽  
Mass Concentration ◽  
Carbonaceous Aerosol ◽  
Long Range Transport ◽  
Air Masses ◽  
Central Germany ◽  
Range Transport ◽  
Local Emissions

Abstract. The identification of different sources of the carbonaceous aerosol (organics and black carbon) was investigated at a mountain forest site located in central Germany from September to October 2010 to characterize incoming air masses during the Hill Cap Cloud Thuringia 2010 (HCCT-2010) experiment. The near-PM1 chemical composition, as measured by an Aerosol Mass Spectrometer (HR-ToF-AMS), was dominated by organics (OA, 41 %), followed by sulfate (19 %) and nitrate (18 %). Source apportionment of the OA fraction was performed using the Multilinear Engine approach (ME-2), resulting in the identification of five factors: Hydrocarbon-like OA (HOA, 3 % of OA mass), biomass burning OA (BBOA, 13 %), semi-volatile-like OA (SVOOA, 19 %), and two oxygenated OA (OOA) factors. The more-oxidized OOA (MO-OOA, 28 %) was interpreted as being influenced by aged polluted continental air masses, whereas the less-oxidized OOA (LO-OOA, 37 %) was found to be more linked to aged biogenic sources. Equivalent black carbon (eBC) measured by a multi-angle absorption photometer, MAAP, represented 10 % of the total PM. The eBC was clearly associated with the three factors HOA, BBOA, and MO-OOA (all together R2 = 0.83). Therefore, eBC's contribution to each factor was achieved using a multi-linear regression model. More than half of the eBC (52 %) was associated with long-range transport (i.e. MO-OOA), whereas liquid fuel eBC (35 %) and biomass burning eBC (13 %) were associated with local emissions leading to a complete apportionment of the carbonaceous aerosol. The separation between local and transported eBC was well supported by the mass size distribution of elemental carbon (EC) from Berner-impactor samples. Air masses with the strongest marine influence based on back trajectory analysis corresponded with a low particle mass concentration (6.4–7.5 µg m−3) and organic fraction (≈ 30 %). However, they also had the largest contribution of primary OA (HOA ≈ 4 % and BBOA 15–20 %), which was associated with local emissions. Continental air masses had the highest mass concentration (11.4–12.6 µg m−3) and a larger fraction of oxygenated OA (≈ 45 %) indicated highly processed OA. The present results emphasize the key role played by long-range transport processes not only on the OA fraction but also on the eBC mass concentration and the importance of improving our knowledge on the identification of eBC sources.

Evidence for long range transport of biological and anthropogenic aerosol particles in the atmosphere

Grana ◽  
1984 ◽  
Vol 23 (1) ◽  
pp. 43-53 ◽  
Author(s):  
Paolo Mandrioli ◽  
Maria Grazia Negrini ◽  
Giulio Cesari ◽  
Griffith Morgan
Keyword(s):  
Long Range ◽  
Aerosol Particles ◽  
Long Range Transport ◽  
Anthropogenic Aerosol ◽  
Range Transport

scholarly journals Statistical aerosol properties associated with fire events from 2002 to 2019 along with a case analysis in 2019 over Australia

2020 ◽  
Author(s):  
Xingchuan Yang ◽  
Chuanfeng Zhao ◽  
Yikun Yang ◽  
Xing Yan ◽  
Hao Fan
Keyword(s):  
Long Range ◽  
Biomass Burning ◽  
Case Analysis ◽  
Carbonaceous Aerosol ◽  
Long Range Transport ◽  
Southeastern Australia ◽  
Range Transport ◽  
Central Australia ◽  
Aerosol Properties ◽  
Aerosol Type

Abstract. Wildfires are an important contributor to atmospheric aerosols in Australia and could significantly affect regional and even global climate. This study investigates the impact of fire events on aerosol properties along with the long-range transport of biomass burning aerosols over Australia using multi-year measurements from Aerosol Robotic Network (AERONET) at ten sites over Australia, satellite dataset derived from the Moderate Resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), reanalysis data from Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), and back-trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT). Strong correlation (0.62) was found between fire radiative power (FRP) and aerosol optical depth (AOD) over Australia, suggesting the significant contribution to aerosols from fires. The fire count, FRP, and AOD showed distinct and consistent interannual variations with high values during September–February (Biomass Burning period, BB period) and low values during March–August (non-Biomass Burning period, non-BB period) every year. The annual average contribution of carbonaceous, dust, sulfate and sea salt aerosols to total aerosol were 26.24 %, 23.38 %, 26.36 % and 24.02 %, respectively. The results from AERONET, MODIS, and MERRA-2 showed that AOD values significantly increased with fine mode aerosol dominated during BB period, especially in northern and southeastern Australia. Further, Carbonaceous aerosol was the main contributor to total aerosols during BB period, especially in September–December when carbonaceous aerosol contributed the most (30.08–42.91 %). The great fires during the BB period of 2019/2020 further demonstrated significant impact on aerosol properties, such as the extreme increase in AOD for most southeastern Australia, the dominance of fine particle aerosols, and the significant increase in carbonaceous and dust aerosols in southeastern and central Australia, respectively. Moreover, smoke was found as the dominant aerosol type detected at heights 2.5–12 km in southeastern Australia in December 2019 and at heights roughly from 6.2 to 12 km in January 2020. In contrast, dust was detected more frequently at heights from 2 to 5 km in November 2019, January, and February 2020. A case analysis revealed that significant changes in aerosol properties including aerosol loading, aerosol particle size, aerosol type in central Australia could be caused during the BB period of 2019/2020 due to the long-range transport of biomass burning aerosols from eastern and southern Australia.

scholarly journals Vertical profiling of aerosol particles and trace gases over the central Arctic Ocean during summer

2013 ◽  
Vol 13 (24) ◽  
pp. 12405-12431 ◽  
Author(s):  
P. Kupiszewski ◽  
C. Leck ◽  
M. Tjernström ◽  
S. Sjogren ◽  
J. Sedlar ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Long Range ◽  
Aerosol Particles ◽  
High Arctic ◽  
Long Range Transport ◽  
Low Level ◽  
Pack Ice ◽  
Range Transport ◽  
Formation And Evolution ◽  
Arctic Summer

Abstract. Unique measurements of vertical size-resolved aerosol particle concentrations, trace gas concentrations and meteorological data were obtained during the Arctic Summer Cloud Ocean Study (ASCOS, www.ascos.se), an International Polar Year project aimed at establishing the processes responsible for formation and evolution of low-level clouds over the high Arctic summer pack ice. The experiment was conducted from on board the Swedish icebreaker Oden, and provided both ship- and helicopter-based measurements. This study focuses on the vertical helicopter profiles and onboard measurements obtained during a three-week period when Oden was anchored to a drifting ice floe, and sheds light on the characteristics of Arctic aerosol particles and their distribution throughout the lower atmosphere. Distinct differences in aerosol particle characteristics within defined atmospheric layers are identified. Within the lowermost couple hundred metres, transport from the marginal ice zone (MIZ), condensational growth and cloud processing develop the aerosol population. During two of the four representative periods defined in this study, such influence is shown. At altitudes above about 1 km, long-range transport occurs frequently. However, only infrequently does large-scale subsidence descend such air masses to become entrained into the mixed layer in the high Arctic, and therefore long-range transport plumes are unlikely to directly influence low-level stratiform cloud formation. Nonetheless, such plumes can influence the radiative balance of the planetary boundary layer (PBL) by influencing formation and evolution of higher clouds, as well as through precipitation transport of particles downwards. New particle formation was occasionally observed, particularly in the near-surface layer. We hypothesize that the origin of these ultrafine particles could be in biological processes, both primary and secondary, within the open leads between the pack ice and/or along the MIZ. In general, local sources, in combination with upstream boundary-layer transport of precursor gases from the MIZ, are considered to constitute the origin of cloud condensation nuclei (CCN) particles and thus be of importance for the formation of interior Arctic low-level clouds during summer, and subsequently, through cloud influences, for the melting and freezing of sea ice.

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