scholarly journals Calibration of the passive cavity aerosol spectrometer probe for airborne determination of the size distribution

2013 ◽  
Vol 6 (9) ◽  
pp. 2349-2358 ◽  
Author(s):  
Y. Cai ◽  
J. R. Snider ◽  
P. Wechsler

Abstract. This work describes calibration methods for the particle sizing and particle concentration systems of the passive cavity aerosol spectrometer probe (PCASP). Laboratory calibrations conducted over six years, in support of the deployment of a PCASP on a cloud physics research aircraft, are analyzed. Instead of using the many calibration sizes recommended by the PCASP manufacturer, a relationship between particle diameter and scattered light intensity is established using three sizes of mobility-selected polystyrene latex particles, one for each amplifier gain stage. In addition, studies of two factors influencing the PCASP's determination of the particle size distribution – amplifier baseline and particle shape – are conducted. It is shown that the PCASP-derived size distribution is sensitive to adjustments of the sizing system's baseline voltage, and that for aggregates of spheres, a PCASP-derived particle size and a sphere-equivalent particle size agree within uncertainty dictated by the PCASP's sizing resolution. Robust determinations of aerosol concentration, and size distribution, also require calibration of the PCASP's aerosol flowrate sensor. Sensor calibrations, calibration drift, and the sensor's non-linear response are documented.

2013 ◽  
Vol 6 (3) ◽  
pp. 4123-4152 ◽  
Author(s):  
Y. Cai ◽  
J. R. Snider ◽  
P. Wechsler

Abstract. This work describes calibration methods for the particle sizing and particle concentration systems of the passive cavity aerosol spectrometer probe (PCASP). Laboratory calibrations conducted over six years, in support of the deployment of a PCASP on a cloud physics research aircraft, are analyzed. Instead of using the many calibration sizes recommended by the PCASP manufacturer, a relationship between particle diameter and scattered light intensity is established using three sizes of mobility-selected polystyrene latex particles, one for each amplifier gain stage. In addition, studies of two factors influencing the PCASP's determination of the particle size distribution – amplifier baseline and particle shape – are conducted. It is shown that the PCASP-derived size distribution is sensitive to adjustments of the sizing system's baseline voltage, and that for aggregate spheres, a PCASP-derived particle size and a sphere-equivalent particle size agree within uncertainty dictated by the PCASP's sizing resolution. Robust determination of aerosol concentration, and size distribution, also require calibration of the PCASP's aerosol flowrate sensor. Sensor calibrations, calibration drift, and the sensor's non-linear response are documented.


Author(s):  
T. Okada ◽  
Y. Ishizu ◽  
K. Matsunuma

AbstractA new method for determining particle-size distribution of cigarette smoke particles was developed by simultaneous measurement of scattered light at three angles for a fixed wavelength. A theoretical chart useful for this purpose, which was made of the relative intensities of scattered light at the angles 45° and 135° to that at the angle 90°, was calculated on the basis of the Mie theory. The number concentration was determined from the Rayleigh ratio using the working standard method. The measurements were rapidly performed, without change of particle size during measuring time, with a device for dilution. The geometric mean diameter, the logarithmic standard deviation and the number concentration of mainstream smoke were found to be about 0.18 um, 0.4 and 3 X 10


2008 ◽  
Vol 65 (1) ◽  
pp. 189-205 ◽  
Author(s):  
Christopher P. Woods ◽  
Mark T. Stoelinga ◽  
John D. Locatelli

Abstract Particle size spectra collected by the University of Washington’s Convair-580 research aircraft at a variety of altitudes and temperatures in winter frontal and orographic precipitation systems during the Improvement of Microphysical Parameterization through Observational Verification Experiment (IMPROVE) are analyzed in this study. The particle size spectra generally appeared to conform to an exponential size distribution, with well-correlated linear fits between the log of the number concentration and particle diameter. When the particle size spectra were grouped according to the habit composition as determined from airborne imagery, significantly improved correlations between the size spectrum parameters and temperature were obtained. This result could potentially be exploited for specifying the size distribution in a single-moment bulk microphysical scheme, if particle habit is predicted by the scheme. Analyses of “spectral trajectories” suggest that the rime-splintering process was likely responsible for the presence of needle and column habit types and the positive shift in both N0s and λs at temperatures warmer than −10°C.


2015 ◽  
Vol 2015 ◽  
pp. 1-10 ◽  
Author(s):  
Benjamin Glasse ◽  
Norbert Riefler ◽  
Udo Fritsching

The continuous monitoring of the particle size distribution in particulate processes with suspensions or emulsions requires measurement techniques that can be used as in situ devices in contrast to ex situ or laboratory methods. In this context, for the evaluation of turbidimetric spectral measurements, the application of different numerical inversion algorithms is investigated with respect to the particle size distribution determination of polystyrene suspensions. A modified regularization concept consisting of a Twomey-Phillips-Regularization with an integrated nonnegative constraint and a modified L-curve criterion for the selection of the regularization parameter is used. The particle size (i.e., particle diameter) of polystyrene suspensions in the rangex=0.03–3 µm was validated via dynamic light scattering and differential centrifugal sedimentation and compared to the retrieved particle size distribution from the inverted turbidimetry measurements.


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