scholarly journals Comparison of the aerosol optical properties and size distribution retrieved by sun photometer with in situ measurements at midlatitude

2016 ◽  
Vol 9 (9) ◽  
pp. 4569-4585 ◽  
Author(s):  
Aurélien Chauvigné ◽  
Karine Sellegri ◽  
Maxime Hervo ◽  
Nadège Montoux ◽  
Patrick Freville ◽  
...  
Keyword(s):  
Remote Sensing ◽  
High Altitude ◽  
In Situ Measurements ◽  
Aerosol Extinction ◽  
The Sun ◽  
Near Surface ◽  
Atmospheric Column ◽  
Fine Mode ◽  
Sun Photometer

Abstract. Aerosols influence the Earth radiative budget through scattering and absorption of solar radiation. Several methods are used to investigate aerosol properties and thus quantify their direct and indirect impacts on climate. At the Puy de Dôme station, continuous high-altitude near-surface in situ measurements and low-altitude ground-based remote sensing atmospheric column measurements give the opportunity to compare the aerosol extinction measured with both methods over a 1-year period. To our knowledge, it is the first time that such a comparison is realised with continuous measurements of a high-altitude site during a long-term period. This comparison addresses to which extent near-surface in situ measurements are representative of the whole atmospheric column, the aerosol mixing layer (ML) or the free troposphere (FT). In particular, the impact of multi-aerosol layers events detected using lidar backscatter profiles is analysed. A good correlation between in situ aerosol extinction coefficient and aerosol optical depth (AOD) measured by the Aerosol Robotic Network (AERONET) sun photometer is observed with a correlation coefficient around 0.80, indicating that the in situ measurements station is representative of the overall atmospheric column. After filtering for multilayer cases and correcting for each layer optical contribution (ML and FT), the atmospheric structure seems to be the main factor influencing the comparison between the two measurement techniques. When the site lies in the ML, the in situ extinction represents 45 % of the sun photometer ML extinction while when the site lies within the FT, the in situ extinction is more than 2 times higher than the FT sun photometer extinction. Moreover, the assumption of a decreasing linear vertical aerosol profile in the whole atmosphere has been tested, significantly improving the instrumental agreement. Remote sensing retrievals of the aerosol particle size distributions (PSDs) from the sun photometer observations are then compared to the near-surface in situ measurements, at dry and at ambient relative humidities. When in situ measurements are considered at dry state, the in situ fine mode diameters are 44 % higher than the sun-photometer-retrieved diameters and in situ volume concentrations are 20 % lower than those of the sun-photometer-retrieved fine mode concentration. Using a parameterised hygroscopic growth factor applied to aerosol diameters, the difference between in situ and retrieved diameters grows larger. Coarse mode in situ diameters and concentrations show a good correlation with retrieved PSDs from remote sensing.

scholarly journals Comparison of the aerosol optical properties and size distribution retrieved by Sun photometer with in-situ measurements at mid-latitude

2016 ◽  
Author(s):  
Aurélien Chauvigné ◽  
Karine Sellegri ◽  
Maxime Hervo ◽  
Nadège Montoux ◽  
Patrick Freville ◽  
...  
Keyword(s):  
Remote Sensing ◽  
In Situ Measurements ◽  
The Sun ◽  
Size Distributions ◽  
Particle Size Distributions ◽  
Near Surface ◽  
Atmospheric Column ◽  
Fine Mode ◽  
Sun Photometer

Abstract. Aerosols influence the Earth radiative budget through scattering and absorption of solar radiation. Several methods are used to investigate aerosol properties and thus quantify their direct and indirect impacts on climate. At the Puy de Dôme station, continuous high altitude near surface in-situ measurements and low altitude ground-based remote sensing atmospheric column measurements give the opportunity to compare the aerosol extinction measured with both methods over a one year period. To our knowledge, it is the first time that such a comparison is realized with continuous measurements of a high altitude site during a long term period. This comparison addresses to which extend near surface in-situ measurements are representative of the whole atmospheric column, the aerosol Mixing Layer (ML), or the Free Troposphere (FT). In particular, the impact of multi aerosol layers events detected using LIDAR backscatter profiles is analysed. A good correlation between in-situ aerosol extinction coefficient and Aerosol Optical Depth (AOD) measured by the Aerosol Robotic Network (AERONET) Sun photometer is observed with a correlation coefficient around 0.80, indicating that the in-situ measurements station is representative of the overall atmospheric column. After filtering for multilayer cases and correcting for each layer optical contribution (ML and FT), the atmospheric structure seems to be the main factor influencing the comparison between the two measurement techniques. When the site lies in the ML, the in-situ extinction represents 45 % of the Sun photometer ML extinction while when the site lies within the FT, the in-situ extinction is more than two times higher than the FT Sun photometer extinction. Remote sensing retrievals of the aerosol particle size distributions (PSD) from the Sun photometer observations are then compared to the near surface in-situ measurements, at dry and at ambient relative humidities. When in-situ measurements are considered at dry state, the in-situ fine mode diameters are 44 % higher than the Sun photometer-retrieved diameters and in-situ volume concentrations are 20 % lower than of the Sun photometer-retrieved fine mode concentration. Using a parametrised hygroscopic growth factor applied to aerosol diameters, the difference between in-situ and retrieved diameters grows larger. Coarse mode in-situ diameter and concentrations show a good correlation with retrieved particle size distributions from remote sensing.

scholarly journals Description and applications of a mobile system performing on-road aerosol remote sensing and in situ measurements

2018 ◽  
Author(s):  
Ioana Elisabeta Popovici ◽  
Philippe Goloub ◽  
Thierry Podvin ◽  
Luc Blarel ◽  
Rodrigue Loisil ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Spatial Variability ◽  
Mass Concentration ◽  
In Situ Measurements ◽  
Quality Data ◽  
The Sun ◽  
Mobile System ◽  
Modis Aod ◽  
Sun Photometer

Abstract. The majority of ground-based aerosols observations are limited to fixed locations, narrowing the knowledge on their spatial variability. In order to overcome this issue, a compact Mobile Aerosol Monitoring System (MAMS) was developed to explore the aerosol vertical and spatial variability. This mobile laboratory is equipped with a micropulse lidar, a sun-photometer and an aerosol spectrometer. It is distinguished by other transportable platforms through its ability to perform on-road measurements and its unique feature lies in the sun-photometer capable to track the sun during motion. The system presents a great flexibility, being able to respond quickly in case of sudden aerosol events such as pollution episodes, dust, fire or volcano outbreaks. On-road mapping of aerosol physical parameters such as attenuated aerosol backscatter, aerosol optical depth, particle number and mass concentration and size distribution is achieved through the MAMS. The performance of remote sensing instruments on-board has been evaluated through intercomparison with instruments in reference networks (i.e. AERONET and EARLINET), showing that the system is capable of providing high quality data. This also illustrates the application of such system for instrument intercomparison field campaigns. Applications of the mobile system have been exemplified through two case studies in northern France. MODIS AOD data was compared to ground-based mobile sun-photometer data. A good correlation was observed with R2 of 0.76, showing the usefulness of the mobile system for validation of satellite-derived products. The performance of BSC-DREAM8b dust model has been tested by comparison of results from simulations to the lidar-sun-photometer derived extinction coefficient and mass concentration profiles. The comparison indicated that observations and model are in good agreement in describing the vertical variability of dust layers. Moreover, on-road measurements of PM10 were compared with modelled PM10 concentrations and with ATMO Hauts-de-France and AIRPARIF air quality in situ measurements, presenting an excellent agreement in horizontal spatial representativity of PM10. This proves a possible application of mobile platforms for evaluating the chemistry-models performances.

scholarly journals Description and applications of a mobile system performing on-road aerosol remote sensing and in situ measurements

2018 ◽  
Vol 11 (8) ◽  
pp. 4671-4691 ◽  
Author(s):  
Ioana Elisabeta Popovici ◽  
Philippe Goloub ◽  
Thierry Podvin ◽  
Luc Blarel ◽  
Rodrigue Loisil ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Spatial Variability ◽  
Mass Concentration ◽  
In Situ Measurements ◽  
Quality Data ◽  
The Sun ◽  
Mobile System ◽  
Modis Aod ◽  
Sun Photometer

Abstract. The majority of ground-based aerosols observations are limited to fixed locations, narrowing the knowledge on their spatial variability. In order to overcome this issue, a compact Mobile Aerosol Monitoring System (MAMS) was developed to explore the aerosol vertical and spatial variability. This mobile laboratory is equipped with a micropulse lidar, a sun photometer and an aerosol spectrometer. It is distinguished from other transportable platforms through its ability to perform on-road measurements and its unique feature lies in the sun photometer's capacity for tracking the sun during motion. The system presents a great flexibility, being able to respond quickly in case of sudden aerosol events such as pollution episodes, dust, fire or volcano outbreaks. On-road mapping of aerosol physical parameters such as attenuated aerosol backscatter, aerosol optical depth, particle number and mass concentration and size distribution is achieved through the MAMS. The performance of remote sensing instruments on-board has been evaluated through intercomparison with instruments in reference networks (i.e. AERONET and EARLINET), showing that the system is capable of providing high quality data. This also illustrates the application of such a system for instrument intercomparison field campaigns. Applications of the mobile system have been exemplified through two case studies in northern France. MODIS AOD data was compared to ground-based mobile sun photometer data. A good correlation was observed with R2 of 0.76, showing the usefulness of the mobile system for validation of satellite-derived products. The performance of BSC-DREAM8b dust model has been tested by comparison of results from simulations for the lidar–sun-photometer derived extinction coefficient and mass concentration profiles. The comparison indicated that observations and the model are in good agreement in describing the vertical variability of dust layers. Moreover, on-road measurements of PM10 were compared with modelled PM10 concentrations and with ATMO Hauts-de-France and AIRPARIF air quality in situ measurements, presenting an excellent agreement in horizontal spatial representativity of PM10. This proves a possible application of mobile platforms for evaluating the chemistry-models performances.

scholarly journals Intercomparison of aerosol extinction profiles retrieved from MAX-DOAS measurements

2016 ◽  
Author(s):  
U. Frieß ◽  
H. Klein Baltink ◽  
S. Beirle ◽  
K. Clèmer ◽  
F. Hendrick ◽  
...  
Keyword(s):  
Optimal Estimation ◽  
Optical Absorption Spectroscopy ◽  
Measuring Instruments ◽  
Aerosol Extinction ◽  
Vertical Profiles ◽  
Near Surface ◽  
Aerosol Absorption ◽  
Sun Photometer ◽  
Absorption Measurements

Abstract. A first direct intercomparison of aerosol vertical profiles from Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations, performed during the Cabauw Intercomparison Campaign of Nitrogen Dioxide measuring Instruments (CINDI) in summer 2009, is presented. Five out of 14 participants of the CINDI campaign reported aerosol extinction profiles and aerosol optical thickness (AOT) as deduced from observations of differential slant column densities of the oxygen collision complex (O4) at different elevation angles. Aerosol vertical profiles and AOT are compared to backscatter profiles from a ceilometer instrument and to sun photometer measurements, respectively. Furthermore, the near-surface aerosol extinction coefficient is compared to in-situ measurements of a humidity controlled nephelometer and dry aerosol absorption measurements. The participants of this intercomparison exercise use different approaches for the retrieval of aerosol information, including the retrieval of the full vertical profile using optimal estimation and a parametrised approach with a prescribed profile shape. Despite these large conceptual differences, and also differences in the wavelength of the observed O4 absorption band, good agreement in terms of the vertical structure of aerosols within the boundary layer is achieved between the aerosol extinction profiles retrieved by the different groups and the backscatter profiles observed by the ceilometer instrument. AOT from MAX-DOAS and sun photometer show a good correlation (R > 0.8), but all participants systematically underestimate the AOT. Substantial differences between the near-surface aerosol extinction from MAX-DOAS and from the humidified nephelometer remain largely unresolved.

scholarly journals Aerosol absorption profiling from the synergy of lidar and sun-photometry: the ACTRIS-2 campaigns in Germany, Greece and Cyprus

2018 ◽  
Vol 176 ◽  
pp. 08005 ◽  
Author(s):  
Alexandra Tsekeri ◽  
Vassilis Amiridis ◽  
Anton Lopatin ◽  
Eleni Marinou ◽  
Eleni Giannakaki ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Radiative Transfer ◽  
Absorption Coefficient ◽  
Single Scattering ◽  
In Situ Measurements ◽  
Climate Modelling ◽  
Aerosol Absorption ◽  
Sun Photometer ◽  
Remote Sensing Techniques

Aerosol absorption profiling is crucial for radiative transfer calculations and climate modelling. Here, we utilize the synergy of lidar with sun-photometer measurements to derive the absorption coefficient and single scattering albedo profiles during the ACTRIS-2 campaigns held in Germany, Greece and Cyprus. The remote sensing techniques are compared with in situ measurements in order to harmonize and validate the different methodologies and reduce the absorption profiling uncertainties.

scholarly journals Intercomparison of aerosol extinction profiles retrieved from MAX-DOAS measurements

2016 ◽  
Vol 9 (7) ◽  
pp. 3205-3222 ◽  
Author(s):  
U. Frieß ◽  
H. Klein Baltink ◽  
S. Beirle ◽  
K. Clémer ◽  
F. Hendrick ◽  
...  
Keyword(s):  
Optimal Estimation ◽  
Optical Absorption Spectroscopy ◽  
Measuring Instruments ◽  
Aerosol Extinction ◽  
Vertical Profiles ◽  
Near Surface ◽  
Aerosol Absorption ◽  
Sun Photometer ◽  
Absorption Measurements

Abstract. A first direct intercomparison of aerosol vertical profiles from Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations, performed during the Cabauw Intercomparison Campaign of Nitrogen Dioxide measuring Instruments (CINDI) in summer 2009, is presented. Five out of 14 participants of the CINDI campaign reported aerosol extinction profiles and aerosol optical thickness (AOT) as deduced from observations of differential slant column densities of the oxygen collision complex (O4) at different elevation angles. Aerosol extinction vertical profiles and AOT are compared to backscatter profiles from a ceilometer instrument and to sun photometer measurements, respectively. Furthermore, the near-surface aerosol extinction coefficient is compared to in situ measurements of a humidity-controlled nephelometer and dry aerosol absorption measurements. The participants of this intercomparison exercise use different approaches for the retrieval of aerosol information, including the retrieval of the full vertical profile using optimal estimation and a parametrised approach with a prescribed profile shape. Despite these large conceptual differences, and also differences in the wavelength of the observed O4 absorption band, good agreement in terms of the vertical structure of aerosols within the boundary layer is achieved between the aerosol extinction profiles retrieved by the different groups and the backscatter profiles observed by the ceilometer instrument. AOTs from MAX-DOAS and sun photometer show a good correlation (R>0.8), but all participants systematically underestimate the AOT. Substantial differences between the near-surface aerosol extinction from MAX-DOAS and from the humidified nephelometer remain largely unresolved.

Particulate matter variability in Kathmandu based on in-situ measurements, remote sensing, and reanalysis data

2021 ◽  
pp. 105623
Author(s):  
Stefan Becker ◽  
Ramesh Prasad Sapkota ◽  
Binod Pokharel ◽  
Loknath Adhikari ◽  
Rudra Prasad Pokhrel ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Particulate Matter ◽  
Reanalysis Data ◽  
In Situ Measurements
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