Amplification of Elliptically Polarized Sub-Femtosecond Pulses in Neon-Like X-Ray Laser Modulated By An IR Field

Amplification of attosecond pulses produced via high harmonic generation is a formidable problem since none of the amplifiers can support the corresponding PHz bandwidth. Producing the well defined polarization state common for a set of harmonics required for formation of the circularly/elliptically polarized attosecond pulses (which are on demand for dynamical imaging and coherent control of the spin flip processes) is another big challenge. In this work we show how both problems can be tackled simultaneously on the basis of the same platform, namely, the plasma-based X-ray amplifier whose resonant transition frequency is modulated by an infrared field.

Polarization control of attosecond pulses using bi-chromatic elliptically polarized laser

We study the high harmonic generation (HHG) using elliptically polarized two-color driving fields. The HHG via bi-chromatic counter-rotating laser fields is a promising source of circularly polarized ultrashort XUV radiation at the attosecond time scale. The ellipticity or the polarization of the attosecond pulses can be tweaked by modifying the emitted harmonics' ellipticity, which can be controlled by varying the driver fields. A simple setup is used to control the polarization of the driving fields, which eventually changes the ellipticity of the attosecond pulses. A well-defined scaling for the ellipticity of the attosecond pulse as a function of the rotation angle of the quarter-wave plate is also deduced by solving the time-dependent Schr\"odinger equation (TDSE) in two dimensions. The scaling can further be explored to obtain the attosecond pulses of the desired degree of polarization, ranging from linear to elliptical to circular polarization.

Strong-field coherent control of isolated attosecond pulse generation

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: improved spectral tunability (allowing selectivity in addressing electronic transitions) and higher photon flux (permitting to measure low cross-section processes). New developments come through parametric waveform synthesis, which provides control over the shape of field transients, enabling the creation of highly-tunable isolated attosecond pulses via high-harmonic generation. Here we demonstrate that the first goal is fulfilled since central energy, spectral bandwidth/shape and temporal duration of isolated attosecond pulses can be controlled by shaping the laser waveform via two key parameters: the relative-phase between two halves of the multi-octave spanning spectrum, and the overall carrier-envelope phase. These results not only promise to expand the experimental possibilities in attosecond science, but also demonstrate coherent strong-field control of free-electron trajectories using tailored optical waveforms.