Effect of Interlayer Coupling and Symmetry on High-Order Harmonic Generation from Monolayer and Bilayer Hexagonal Boron Nitride

High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich information concerning the electron structure and dynamics of matter, for instance, gases, solids and liquids. Moreover, the HHG from solids has recently attracted the attention of both attosecond science and condensed matter physicists, since the HHG spectra can carry information of electron-hole dynamics in bands and inter- and intra-band current dynamics. In this paper, we study the effect of interlayer coupling and symmetry in two-dimensional (2D) material by analyzing high-order harmonic generation from monolayer and two differently stacked bilayer hexagonal boron nitrides (hBNs). These simulations reveal that high-order harmonic emission patterns strongly depend on crystal inversion symmetry (IS), rotation symmetry and interlayer coupling.

Extended model for optimizing high-order harmonic generation in absorbing gases

We report on an extended version of the one-dimensional model proposed by Constant et al. [Phys. Rev. Lett 82(8), 1668 (1999)] to study phase matching of high-order harmonic generation in absorbing and dispersive medium. The model - expanded from zeroth to first order - can be used with media having a pressure profile varying linearly with propagation length. Based on the new formulas, the importance of having a generation medium that ends abruptly with a steep pressure gradient for achieving high flux is highlighted. In addition to further rule-of-thumb guidelines for harmonic-flux optimization, it is shown that having a steep increase of pressure in the beginning of the medium increases harmonic flux, while it also decreases the required medium length to reach the absorption-limited maximum.

Retrieval of Angle-Dependent Strong-Field Ionization by Using High Harmonics Generated from Aligned N2 Molecules

We propose a method to retrieve the angle-dependent strong-field ionization of highest occupied molecular orbital (HOMO) from high-order harmonic generation (HHG) of aligned molecules. This method is based on the single-molecule quantitative rescattering model with known alignment distribution and photo-recombination cross sections of fixed-in-space molecules. With the macroscopic HHG of aligned N2 molecules, we show that angle-dependent ionization of HOMO can be successfully retrieved at both low and high degrees of alignment. We then show that the error in the retrieved angular dependence of ionization becomes larger if the uncertainty in the alignment distribution is introduced in the retrieval procedure. We also examine that the retrieved ionization of HOMO is much deviated from the accurate one if the intensity of probe laser becomes higher such that inner HOMO-1 can contribute to HHG.

Orientation and Ellipticity Dependence of High-order Harmonic Generation in Nanowires

It has been predicted that high-order harmonic generation (HHG) in nanowires has the potential to scale up photon energy and harmonic yield. However, studies on HHG in nanowires are still theoretical and no relevant experimental results have been reported as yet. Our experimental observation of the high-order harmonic in cadmium sulfide nanowires (CdS NWs) excited by a mid-infrared laser is, to our knowledge, the first such study, and it verifies some of the theoretical results. Our experimental results show that the observed harmonics are strongest when a pump laser is parallel to the nanowires. Therefore, the theoretical prediction that harmonics are strongest under the nanowires parallel to the laser field is confirmed experimentally; this can be used to determine the orientation of the nanowire. In addition, harmonics are sensitive to the variation of pump light ellipticities. This orientation dependence opens new opportunities to access ultrafast and strong-field physics of nanowires.