Theory of optical tweezing of dielectric microspheres in chiral host media and its applications

We report for the first time the theory of optical tweezers of spherical dielectric particles embedded in a chiral medium. We develop a partial-wave (Mie) expansion to calculate the optical force acting on a dielectric microsphere illuminated by a circularly-polarized, highly focused laser beam. When choosing a polarization with the same handedness of the medium, the axial trap stability is improved, thus allowing for tweezing of high-refractive-index particles. When the particle is displaced off-axis by an external force, its equilibrium position is rotated around the optical axis by the mechanical effect of an optical torque. Both the optical torque and the angle of rotation are greatly enhanced in the presence of a chiral host medium when considering radii a few times larger than the wavelength. In this range, the angle of rotation depends strongly on the microsphere radius and the chirality parameter of the host medium, opening the way for a quantitative characterization of both parameters. Measurable angles are predicted even in the case of naturally occurring chiral solutes, allowing for a novel all-optical method to locally probe the chiral response at the nanoscale.

Rotation of an elliptical dielectric particle in the focus of a circularly polarized Gaussian beam

A force and a torque exerted on an elliptical dielectric particle in the focus of a spherical circularly polarized laser beam are considered. The numerical simulation is conducted using a diffraction field obtained by an FDTD method, with the force and torque derived using a Maxwell’s stress tensor. It is shown that an optical torque is exerted on the center of an elliptical particle put in the focus of a circularly polarized spherical wave, making it rotate around the optical axis. The rotation occurs when the elliptical microparticle is situated in a transverse plane to the optical axis. When shifting the ellipsoid from the optical axis, an optical trapping force appears that prevents its displacement, meaning that the particle finds itself in an optical trap on the optical axis.